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We report low-temperature powder X-ray and neutron diffraction studies on breathing pyrochlore magnets Cu$M$Cr$_{4}$S$_{8}$ ($M$ = Al, Ga), which undergo a magnetic transition at $T_{\rm N} \approx$ 21 and 31 K for {$M$ = Al and Ga,…

材料科学 · 物理学 2024-05-09 Masaki Gen , Taro Nakajima , Hiraku Saito , Yusuke Tokunaga , Taka-hisa Arima

We report the crystal growth and structural and magnetic properties of quasi two-dimensional $S=1/2$ quantum magnet Cu[C$_6$H$_2$(COO)$_4$][H$_3$N-(CH$_2$)$_2$-NH$_3$]$\cdot$3H$_2$O. It is found to crystallize in a monoclinic structure with…

材料科学 · 物理学 2021-05-26 S. Guchhait , S. Baby , M. Padmanabhan , A. Medhi , R. Nath

InMnO$_3$ is a peculiar member of the hexagonal manganites h-RMnO$_3$ (where R is a rare earth metal element), showing crystalline, electronic and magnetic properties at variance with the other compounds of the family. We have studied high…

材料科学 · 物理学 2015-03-19 X. Fabrèges , I. Mirebeau , S. Petit , P. Bonville , A. A. Belik

We have observed enhancement and shift in the spin reorientation transition temperature as a consequence of coexistence of orthorhombic and hexagonal phases and higher aspect ratio in nanoscale LuFeO3. Nanoparticles and nanofibers of LuFeO3…

The crystal structure and the magnetism of BaMn$_2$O$_3$ have been studied by thermodynamic and by diffraction techniques using large single crystals and powders. BaMn$_2$O$_3$ is a realization of a $S = 5/2$ spin ladder as the magnetic…

强关联电子 · 物理学 2015-05-20 M. Valldor , O. Heyer , A. C. Komarek , A. Senyshyn , M. Braden , T. Lorenz

The magnetic properties of a series of YBa2Cu3O7-x/La2/3Ca1/3MnO3 (YBCO/LC1/3MO) superlattices grown by dc sputtering at high oxygen pressures (3.5 mbar) show the expected ferromagnetic behaviour. However, field cooled hysteresis loops at…

材料科学 · 物理学 2009-11-10 N. Haberkorn , J. Guimpel , M. Sirena , L. B. Steren , W. Saldarriaga , E. Baca , M. E. Gómez

We report the observation of weak magnetism in superlattices of LaAlO3/SrTiO3 using beta-detected nuclear magnetic resonance. The spin lattice relaxation rate of 8 Li in superlattices with a spacer layers of 8 and 6 unit cells of LaAlO3…

Magnetic structure of single crystalline TmB4 has been studied by magnetization, magnetoresistivity and specific heat measurements. A complex phase diagram with different antiferromagnetic (AF) phases was observed below TN1 = 11.7 K.…

强关联电子 · 物理学 2007-12-05 S. Gabani , S. Matas , P. Priputen , K. Flachbart , K. Siemensmeyer , E. Wulf , A. Evdokimova , N. Shitsevalova

HoNiSi$_{3}$ is an intermetallic compound characterized by two successive antiferromagnetic transitions at $T_{N1} = 6.3$ K and $T_{N2} = 10.4$ K. Here, its zero-field microscopic magnetic structure is inferred from resonant x-ray magnetic…

We report single crystal growth and magnetic susceptibility and neutron diffraction studies of the S=1/2 quasi-1D antiferromagnet CaCu2O3. The structure of this material is similar to that of the prototype two-leg spin-ladder compound…

凝聚态物理 · 物理学 2009-10-31 V. Kiryukhin , Y. J. Kim , K. J. Thomas , F. C. Chow , R. W. Erwin , Q. Huang , M. A. Kastner , R. J. Birgeneau

To study the relationship between the properties of low-dimensional spin systems with weakly coupled Cu-triangles and their crystal structure, single crystals of $Cs_3Cu_3Cl_8OH$ (1) and the new $Cs_3Cu_3Cl_{7.6}Br_{0.4}OH$ (2) were grown.…

Frustrated magnetism continues to attract significant attention due to its potential to host novel quantum many-body phenomena and associated exotic excitations that transcend existing paradigms. Herein, we present our reply to the comment…

The crystal structure and magnetic correlations in triangular antiferromagnet FeGa$_2$S$_4$ are studied by x-ray diffraction, magnetic susceptibility, neutron diffraction and neutron inelastic scattering. We report significant mixing at the…

Neutron diffraction on the double perovskite Sr2YRuO6 with a quasi-face-centered cubic (FCC) lattice of Ru moments reveals planar magnetic correlations that condense into a partial long-range ordered state with coupled alternate…

强关联电子 · 物理学 2015-06-11 E. Granado , J. W. Lynn , R. F. Jardim , M. S. Torikachvili

We report a comprehensive study of the low-level substitution of Mn$^{3+}$ by Fe$^{3+}$ effect on the static and dynamic magnetoelectric coupling in TbMn$_{1-x}$Fe$_x$O$_3$ ($x=0$, 0.02 and 0.04). The cationic substitution has a large…

In the R$\_{3}$Ga$\_{5}$SiO$\_{14}$ compounds, the network R of rare earth cations form well separated planes of corner sharing triangles topologically equivalent to a kagom\'e lattice. Powder samples and single crystals with R = Nd and Pr…

强关联电子 · 物理学 2007-05-23 P. Bordet , I. Gelard , K. Marty , A. Ibanez , J. Robert , V. Simonet , B. Canals , R. Ballou , P. Lejay

FeVO$_4$ has been studied by heat capacity, magnetic susceptibility, electric polarization and single crystal neutron diffraction experiments. The triclinic crystal structure is made of \emph{S}-shaped clusters of six Fe$^{3+}$ ions, linked…

超导电性 · 物理学 2015-05-13 A. Daoud-Aladine , B. Kundys , C. Martin , P. G. Radaelli , P. J. Brown , C. Simon , L. C. Chapon

We use ultrafast x-ray and electron diffraction to disentangle spin-lattice coupling of granular FePt in the time domain. The reduced dimensionality of single-crystalline FePt nanoparticles leads to strong coupling of magnetic order and a…

We have used soft x-ray magnetic diffraction at the Fe3+ L2,3 edges to examine to what extent the Dzyaloshinsky-Moriya interaction in Ba3NbFe3Si2O14 influences its low temperature magnetic structure. A modulated component of the moments…

强关联电子 · 物理学 2013-09-26 V. Scagnoli , S. W. Huang , M. Garganourakis , R. A. de Souza , U. Staub , V. Simonet , P. Lejay , R. Ballou

In this work, we report on the thermomagnetic characterization and crystalline-electric field (CEF) energy scheme of the disordered defect-fluorite Ho2Zr2O7. This structural phase is distinguished by the coexistence of magnetic frustration…

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