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Studies of ultrafast dynamics along with femtosecond-pulse metrology rely on non-linear processes, induced solely by the exciting/probing pulses or the pulses to be characterized. Extension of these approaches to the extreme-ultraviolet…

原子物理 · 物理学 2015-05-27 P. Tzallas , E. Skantzakis , L. A. A. Nikolopoulos , G. D. Tsakiris , D. Charalambidis

Attosecond light pulses in the extreme ultraviolet have drawn a great deal of attention due to their ability to interrogate electronic dynamics in real time. Nevertheless, to follow charge dynamics and excitations in materials, element…

原子物理 · 物理学 2016-06-08 S. M. Teichmann , F. Silva , S. L. Cousin , M. Hemmer , J. Biegert

We propose a new scenario to apply IR-pump-XUV-probe schemes to resolving strong field ionization induced and attosecond pulse driven electron-hole dynamics and coherence in real time. The coherent driving of both the infrared laser and the…

原子物理 · 物理学 2016-02-26 Jing Zhao , Jianmin Yuan , Zengxiu Zhao

Attosecond laser pulses open the door to resolve microscopic electron dynamics in time. Experiments performed include the decay of a core hole, the time-resolved measurement of photo ionization and electron tunneling. The processes…

原子与分子团簇 · 物理学 2011-11-09 Ionut Georgescu , Ulf Saalmann , Jan M. Rost

Modern intense ultrafast pulsed lasers generate an electric field of sufficient strength to permit tunnel ionization of the valence electrons in atoms. This process is usually treated as a rapid succession of isolated events, in which the…

The development of attosecond technology has enabled the real-time observation of coherent electron motion in atoms, molecules and condensed phases. Experimentally, it is now possible to generate laser pulses of durations of only a few tens…

化学物理 · 物理学 2017-05-18 David Ayuso

High harmonic generation driven by femtosecond lasers makes it possible to capture the fastest dynamics in molecules and materials. However, to date the shortest attosecond (as) pulses have been produced only in the extreme ultraviolet…

Measuring the delay for an electron to emerge from different states is one of the major achievements of attosecond science. This delay can have two origins - the electron wave packet is reshaped during departure by the electrostatic field…

原子物理 · 物理学 2020-10-14 Graham G. Brown , Dong Hyuk Ko , Chunmei Zhang , P. B. Corkum

The basic properties of atoms, molecules and solids are governed by electron dynamics which take place on extremely short time scales. To measure and control these dynamics therefore requires ultrafast sources of radiation combined with…

原子物理 · 物理学 2008-02-27 J. Mauritsson , P. Johnsson , E. Gustafsson , M. Swoboda , T. Ruchon , A. LHuillier , K. J. Schafer

We consider an electron in an atom driven by an infrared (IR) elliptically polarized laser field after its ionization by an ultrashort extreme ultraviolet (XUV) pulse. We find that, regardless of the atom species and the laser ellipticity,…

原子物理 · 物理学 2021-11-24 Jonathan Dubois , Angel Jorba

Attosecond science is based on steering of electrons with the electric field of well-controlled femtosecond laser pulses. It has led to, for example, the generation of XUV light pulses with a duration in the sub-100-attosecond regime, to…

量子物理 · 物理学 2011-07-11 Michael Krüger , Markus Schenk , Peter Hommelhoff

Laser-plasma electron accelerators can be used to produce high-intensity X-rays, as electrons accelerated in wakefields emit radiation due to betatron oscillations.Such X-ray sources inherit the features of the electron beam;…

等离子体物理 · 物理学 2021-04-07 Julien Ferri , Vojtech Horný , Tünde Fülöp

Nonsequential multiple ionization of atoms in intense laser fields is initiated by a recollision between an electron, freed by tunneling, and its parent ion. Following recollision, the initial electron shares its energy with several bound…

原子物理 · 物理学 2009-11-11 X. Liu , C. Figueira de Morisson Faria , W Becker , P. B. Corkum

Infrared femtosecond laser pulses are important tools both in strong-field physics, driving X-ray high-harmonic generation, and as the basis for widely tuneable, if inefficient, ultrafast sources in the visible and ultraviolet. Although…

光学 · 物理学 2020-10-14 Christian Brahms , Federico Belli , John C. Travers

The photoelectric effect is not truly instantaneous, but exhibits attosecond delays that can reveal complex molecular dynamics. Sub-femtosecond duration light pulses provide the requisite tools to resolve the dynamics of photoionization.…

It is shown that the energy absorption of a rare-gas cluster from a vacuum-ultraviolet (VUV) pulse can be traced with time-delayed extreme-ultraviolet (XUV) attosecond probe pulses by measuring the kinetic energy of the electrons detached…

原子与分子团簇 · 物理学 2008-04-07 Ulf Saalmann , Ionuţ Georgescu , Jan M. Rost

A coherent vibrational wavepacket is launched and manipulated in the symmetric stretch (a$_1$) mode of CBr$_4$, by impulsive stimulated Raman scattering from non-resonant 400 nm laser pump pulses with various peak intensities on the order…

Multiphoton-ionized electrons are born into a strong light field that will determine their short-term future. By controlling the infrared beam, we enable atoms or molecules to generate extreme ultraviolet (XUV) pulses and synthesize…

原子物理 · 物理学 2020-10-13 Dong Hyuk Ko , Graham G. Brown , Chunmei Zhang , P. B. Corkum
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