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CoO has an odd number of electrons in its unit cell, and therefore is expected to be metallic. Yet, CoO is strongly insulating owing to significant electronic correlations, thus classifying it as a Mott insulator. We investigate the…

Following previous works reporting an anomalous behavior of several zone-center optical phonons across the magnetic transition of square lattice iridates Sr2IrO4 and Sr3Ir2O7, we have investigated the lattice dynamics as a function of…

强关联电子 · 物理学 2022-02-02 K. Sen , R. Heid , S. M. Souliou , D. Boll , A. Bosak , N. H. Sung , J. Bertinshaw , H. Gretarsson , B. J. Kim , F. Weber , M. Le Tacon

MnV$_2$O$_4$ in the spinel structure is known to exhibit coupled orbital and spin ordering, and its Raman spectra show interesting anomalies in its low-temperature phase. With a goal to explain this behavior involving coupled spins and…

材料科学 · 物理学 2020-05-27 Dibyendu Dey , T. Maitra , U. V. Waghmare , A. Taraphder

Sr2IrO4 exhibits a novel insulating state driven by spin-orbit interactions. We report two novel phenomena, namely a large magnetoresistivity in Sr2IrO4 that is extremely sensitive to the orientation of magnetic field but exhibits no…

强关联电子 · 物理学 2015-05-28 M. Ge , T. F. Qi , O. B. Korneta , D. E. De Long , P. Schlottmann , W. P. Crummett , G. Cao

The frustrated magnet Bi2Fe4O9 has been reported to exhibit complex spin dynamics coexisting with conventional spin wave excitations. The magnetic Fe3+ (S = 5/2) ions are arranged into a distorted two-dimensional Cairo pentagonal lattice…

We report neutron inelastic scattering measurements and analysis of the spectrum of magnons propagating within the Fe2O4 bilayers of LuFe2O4. The observed spectrum is consistent with six magnetic modes and a single prominent gap, which is…

Quasi-2D van der Waals ferromagnet Fe$_4$GeTe$_2$, featuring the simultaneous presence of high Curie temperature ($T_\mathrm{C}$ $\sim 270$ K) and a spin-reorientation transition at $T_\mathrm{SR}$ $\sim 110$ K, is a rare system where…

The low-dimensional s=1/2 compound (NO)[Cu(NO3)3] has recently been suggested to follow the Nersesyan-Tsvelik model of coupled spin chains. Such a system shows unbound spinon excitations and a resonating valence bond ground state due spin…

强关联电子 · 物理学 2022-06-08 V. Gnezdilov , P. Lemmens , Yu. G. Pashkevich , D. Wulferding , I. V. Morozov , O. S. Volkova , A. Vasiliev

Here we report on the low-energy excitations within the paramagnetic spin-orbit insulator Sr$_3$Ir$_2$O$_7$F$_2$ studied via resonant inelastic X-ray scattering, \textit{ab initio} quantum chemical calculations, and model-Hamiltonian…

强关联电子 · 物理学 2022-09-26 Zach Porter , Paul M. Sarte , Thorben Petersen , Mary H. Upton , Liviu Hozoi , Stephen D. Wilson

Spin-phonon coupling, the interaction of spins with surrounding lattice is a key parameter to understand the underlying physics of multiferroics and engineer their magnetization dynamics. Elementary excitations in multiferroic materials are…

材料科学 · 物理学 2020-11-05 Bommareddy Poojitha , Anjali Rathore , Ankit Kumar , Surajit Saha

We have performed polarized Raman scattering measurements on the newly discovered superconductor Ba$_{2}$Ti$_{2}$Fe$_{2}$As$_{4}$O$_{2}$ ($T_c = 21$ K). We observe seven out of eight Raman active modes, with frequencies in good accordance…

超导电性 · 物理学 2014-05-07 S. -F. Wu , P. Richard , W. -L. Zhang , C. -S. Lian , Y. -L. Sun , G. -H. Cao , J. -T. Wang , H. Ding

Dynamical correlations of Jeff = 1/2 isospins in the paramagnetic state of spin-orbital Mott insu- lator Sr2IrO4 was revealed by resonant magnetic x-ray diffuse scattering. We found two-dimensional antiferromagnetic fluctuation with a large…

强关联电子 · 物理学 2015-06-04 S. Fujiyama , H. Ohsumi , T. Komesu , J. Matsuno , B. J. Kim , M. Takata , T. Arima , H. Takagi

The magnetic critical scattering in Sr$_2$IrO$_4$ has been characterized using X-ray resonant magnetic scattering (XRMS) both below and above the 3D antiferromagnetic ordering temperature, T$_{\text{N}}$. The order parameter critical…

The polarized Raman scattering spectra from freshly cleaved $ab$, $ac$, and $bc$ surfaces of high quality twin free YBa$_2$Cu$_3$O$_{6.5}$ (Ortho-II) single crystals ($T_c$=57.5 K and $\Delta T = 0.6$ K) were studied between 80 and 300 K.…

超导电性 · 物理学 2008-03-14 M. N. Iliev , V. G. Hadjiev , S. Jandl , D. Le Boeuf , V. N. Popov , D. Bonn , R. Liang , W. N. Hardy

Spin and lattice are two fundamental degrees of freedom in a solid, and their fluctuations about the equilibrium values in a magnetic ordered crystalline lattice form quasiparticles termed magnons (spin waves) and phonons (lattice waves),…

We present inelastic neutron scattering measurements of the antiferromagnetic insulator CaMn$_2$Sb$_2$, which consists of corrugated honeycomb layers of Mn. The dispersion of magnetic excitations has been measured along the H and L…

We calculate the Raman spectrum of the two-dimensional (2D) spin-1/2 Heisenberg antiferromagnet by exact diagonalization and quantum Monte Carlo techniques on clusters of up to 144 sites and, on a 16-site cluster, by considering the…

超导电性 · 物理学 2016-08-31 Franco Nori , Roberto Merlin , Stephan Haas , Anders Sandvik , Elbio Dagotto

An intriguing idea of spin-orbit Mott insulator has been proposed to explain magnetic insulating behavior in various iridates. This scenario relies on the strength of the spin-orbit coupling being comparable to electronic correlations, and…

强关联电子 · 物理学 2013-05-30 Jean-Michel Carter , Hae-Young Kee

Two--magnon Raman scattering is a useful tool to verify recent suggestions concerning the value of the interplanar exchange constant in antiferromagnetic two--layer systems, such as $YBa_2Cu_3O_{6+x}$. We present a theory for Raman…

凝聚态物理 · 物理学 2009-10-28 Dirk K. Morr , Andrey V. Chubukov , Arno P. Kampf , G. Blumberg

We investigate the interplay between lattice symmetry, phonons, and magnetism in the quasi-one-dimensional ladder compound BaFe$_2$S$_3$ by combining polarized synchrotron infrared spectroscopy, hybrid-functional density functional theory…