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High frequency electron spin resonance (ESR) spectroscopy is an invaluable tool for identification and characterization of spin systems. Nanoscale ESR using the nitrogen-vacancy (NV) center has been demonstrated down to the level of a…

介观与纳米尺度物理 · 物理学 2020-05-05 Benjamin Fortman , Junior Pena , Karoly Holczer , Susumu Takahashi

An interacting spin system is an excellent testbed for fundamental quantum physics and applications in quantum sensing and quantum simulation. For these investigations, detailed information of the interactions, e.g., the number of spins and…

量子物理 · 物理学 2024-11-12 Yuhang Ren , Susumu Takahashi

Spectral analysis of electron spin resonance (ESR) is a powerful technique for various investigations including characterization of spin systems, measurements of spin concentration, and probing spin dynamics. The nitrogen-vacancy (NV)…

介观与纳米尺度物理 · 物理学 2019-07-19 Benjamin Fortman , Susumu Takahashi

Using an optical tweezers apparatus, we demonstrate three-dimensional control of nanodiamonds in solution with simultaneous readout of ground-state electron-spin resonance (ESR) transitions in an ensemble of diamond nitrogen-vacancy (NV)…

The application of magnetic resonance (MR) spectroscopy at progressively smaller length scales may eventually permit "chemical imaging" of spins at the surfaces of materials and biological complexes. In particular, the negatively charged…

介观与纳米尺度物理 · 物理学 2015-06-18 Hai-Jing Wang , Chang S. Shin , Scott J. Seltzer , Claudia E. Avalos , Alexander Pines , Vikram S. Bajaj

Substitutional nitrogen atoms in a diamond crystal (P1 centers) are, on one hand, a resource for creation of nitrogen-vacancy (NV) centers, that have been widely employed as nanoscale quantum sensors. On the other hand, P1's electron spin…

Paramagnetic magnetic resonance, a powerful technique for characterizing and identifying chemical targets, is increasingly used for imaging; however, low spin polarization at room temperature and moderate magnetic fields poses challenges…

介观与纳米尺度物理 · 物理学 2019-09-04 C. M. Purser , V. P. Bhallamudi , C. S. Wolfe , H. Yusuf , B. A. McCullian , C. Jayaprakash , M. E. Flatté , P. C. Hammel

Near-surface nitrogen-vacancy (NV) centers have been created in diamond through low energy implantation of 15N to sense electron spins that are external to the diamond. By performing double resonance experiments, we have verified the…

介观与纳米尺度物理 · 物理学 2015-06-11 H. J. Mamin , M. H. Sherwood , D. Rugar

Electron Spin Resonance (ESR) describes a suite of techniques for characterising electronic systems, with applications in physics, materials science, chemistry, and biology. However, the requirement for large electron spin ensembles in…

量子物理 · 物理学 2015-03-04 L. T. Hall , P. Kehayias , D. A. Simpson , A. Jarmola , A. Stacey , D. Budker , L. C. L. Hollenberg

We report observations of the Electron Spin Resonance (ESR) of Nitrogen Vacancy (NV) centers in diamonds that are levitating in an ion trap. Using a needle Paul trap operating under ambient conditions, we demonstrate efficient microwave…

量子物理 · 物理学 2017-07-10 Tom Delord , Louis Nicolas , Lucien Schwab , Gabriel Hétet

We report an experimental study of the longitudinal relaxation time ($T_1$) of the electron spin associated with single nitrogen-vacancy (NV) defects hosted in nanodiamonds (ND). We first show that $T_1$ decreases over three orders of…

介观与纳米尺度物理 · 物理学 2015-06-15 J. -P. Tetienne , T. Hingant , L. Rondin , A. Cavailles , L. Mayer , G. Dantelle , T. Gacoin , J. Wrachtrup , J. -F. Roch , V. Jacques

Electron paramagnetic resonance spectroscopy (EPR) is among the most important analytical tools in physics, chemistry, and biology. The emergence of nitrogen-vacancy (NV) centers in diamond, serving as an atomic-sized magnetometer, has…

Diamond has been extensively investigated recently due to a wide range of potential applications of nitrogen-vacancy (NV) defect centers existing in a diamond lattice. The applications include magnetometry and quantum information…

介观与纳米尺度物理 · 物理学 2016-03-25 Viktor Stepanov , Susumu Takahashi

The nitrogen-vacancy (NV) center can serve as a magnetic sensor for electron paramagnetic resonance (EPR) measurements. Benefiting from its atomic size, the diamond chip can integrate a tremendous amount of NV centers to improve the…

In diamond, nitrogen defects like the substitutional nitrogen defect (Ns) or the nitrogen-vacancy-hydrogen complex (NVH) outnumber the nitrogen vacancy (NV) defect by at least one order of magnitude creating a dense spin bath. While neutral…

We present an experimental and theoretical study of electronic spin decoherence in ensembles of nitrogen-vacancy (NV) color centers in bulk high-purity diamond at room temperature. Under appropriate conditions, we find ensemble NV spin…

介观与纳米尺度物理 · 物理学 2011-01-25 P. L. Stanwix , L. M. Pham , J. R. Maze , D. Le Sage , T. K. Yeung , P. Cappellaro , P. R. Hemmer , A. Yacoby , M. D. Lukin , R. L. Walsworth

High concentration of negatively charged nitrogen-vacancy ($\text{NV}^{-}$) centers was created in diamond single crystals containing approximately 100 ppm nitrogen using electron and neutron irradiation and subsequent thermal annealing in…

Pulsed ESR experiments are reported for ensembles of negatively-charged nitrogen-vacancy centers (NV$^-$) in diamonds at X-band magnetic fields (280-400 mT) and low temperatures (2-70 K). The NV$^-$ centers in synthetic type IIb diamonds…

量子物理 · 物理学 2016-12-22 B. C. Rose , C. D. Weis , A. M. Tyryshkin , T. Schenkel , S. A. Lyon

Nitrogen-vacancy (NV) center in diamond is a promising quantum sensor with remarkably versatile sensing capabilities. While scanning NV magnetometry is well-established, NV electrometry has been so far limited to bulk diamonds. Here we…

量子物理 · 物理学 2022-10-12 Ziwei Qiu , Assaf Hamo , Uri Vool , Tony X. Zhou , Amir Yacoby

The negatively charged nitrogen-vacancy (NV$^-$) center in diamond is a model quantum system for university teaching labs due to its room-temperature compatibility and cost-effective operation. Based on the low-cost experimental setup that…

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