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相关论文: Ultralong-Range Rb-KRb Rydberg Molecules: Selected…

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We investigate the electronic structure of a triatomic Rydberg molecule formed by a Rydberg atom and two neutral ground-state atoms. Taking into account the $s$-wave and $p$-wave interactions we perform electronic structure calculations and…

原子物理 · 物理学 2016-06-22 Javier Aguilera Fernández , Peter Schmelcher , Rosario González-Férez

We explore the electronic structure and rovibrational properties of an ultralong-range triatomic Rydberg molecule formed by a Rydberg atom and a ground state heteronuclear diatomic molecule. We focus here on interaction of Rb($27s$) Rydberg…

原子物理 · 物理学 2015-06-22 Rosario González-Férez , H. R. Sadeghpour , Peter Schmelcher

We explore the electronic structure of ultralong-range pentaatomic Rydberg molecules from a merger of a Rydberg atom and two ground state heteronuclear diatomic molecules. Our focus is on the interaction of Rb($23s$) and Rb($n=20$, $l\ge…

We investigate polyatomic ultralong-range Rydberg molecules consisting of three ground state atoms bound to a Rydberg atom via $s$- and $p$-wave interactions. By employing the finite basis set representation of the unperturbed Rydberg…

原子物理 · 物理学 2016-08-03 Christian Fey , Markus Kurz , Peter Schmelcher

We investigate properties of ultralong-range polyatomic molecules formed with a Rb Rydberg atom and several ground-state atoms whose distance from the Rydberg atom is of the order of n^2a_0, where n is the principle quantum number of the…

原子物理 · 物理学 2007-05-23 Ivan C. H. Liu , Jan M. Rost

Rydberg molecule, formed by one or more Rydberg atoms, exhibits remarkable properties, including an exceptionally large spatial extent, rich rovibrational level structures, permanent electric dipole moments, and a pronounced sensitivity to…

原子物理 · 物理学 2026-03-11 Jingxu Bai , Yuechun Jiao , Xiao-Qiang Shao , Weibin Li , Jianming Zhao

We propose an experimentally realizable scheme to produce triatomic ultralong-range Rydberg molecules (TURM), formed in ultracold KRb traps. A near resonant coupling of the non-zero quantum defect Rydberg levels with the KRb molecule in N=0…

We consider ultralong-range polyatomic Rydberg molecules formed by combining a Rydberg cesium atom and a ground-state RbCs molecule. We explore the regime where the charge-dipole interaction due to the Rydberg electron with the diatomic…

We explore the external electric field control of a species of ultralong-range molecules that emerge from the interaction of a ground state polar molecule with a Rydberg atom. The external field mixes the Rydberg electronic states and…

原子物理 · 物理学 2012-06-01 M. Mayle , S. T. Rittenhouse , P. Schmelcher , H. R. Sadeghpour

Ultralong-range Rydberg molecules, composed of an excited Rydberg atom and a ground-state atom, are characterized by large bond lengths, dipole moments, sensitivity to external fields, and an unusual binding mechanism based on low-energy…

原子物理 · 物理学 2025-05-13 Agata Wojciechowska , Michał Tomza , Matthew T. Eiles

The internal electric field of a Rydberg atom electron can bind a polar molecule to form a giant ultralong-range stable polyatomic molecule. Such molecules not only share their properties with Rydberg atoms, they possess huge permanent…

原子物理 · 物理学 2015-05-27 Seth T. Rittenhouse , M. Mayle , P. Schmelcher , H. R. Sadeghpour

This Ph.D. tutorial discusses ultra-long-range Rydberg molecules, the exotic bound states of a Rydberg atom and one or more ground state atoms immersed in the Rydberg electron's wave function. This novel chemical bond is distinct from an…

原子物理 · 物理学 2019-09-04 Matthew T Eiles

We introduce a computational method developed for study of long-range molecular Rydberg states of such systems that can be approximated by two electrons in a model potential of the atomic cores. Only diatomic molecules are considered. The…

化学物理 · 物理学 2016-01-26 Michal Tarana , Roman Čurík

Ultralong-range Rydberg molecules provide an exciting testbed for molecular physics at exaggerated scales. In the so-called trilobite and butterfly Rydberg molecules, the Born-Oppenheimer approximation can fail due to strong non-adiabatic…

原子物理 · 物理学 2023-02-23 Frederic Hummel , Peter Schmelcher , Matthew T. Eiles

We investigate the impact of combined electric and magnetic fields on the structure of ultralong-range polar Rydberg molecules. Our focus is hereby on the parallel as well as the crossed field configuration taking into account both the…

原子物理 · 物理学 2014-09-11 Markus Kurz , Peter Schmelcher

We investigate triatomic molecules that consist of two ground state atoms and a highly excited Rydberg atom, bound at large internuclear distances of thousands of \AA ngstroms. In the molecular state the Rydberg electron is in a…

原子物理 · 物理学 2019-02-27 Christian Fey , Frederic Hummel , Peter Schmelcher

Ultra-long-range Rydberg molecules (ULRMs) have attracted significant interest due to their unique electronic properties and potential applications in quantum technologies. We theoretically investigate the formation and characteristics of…

The adiabatic potential energy curves of Rb$_2$ in the long-range Rydberg electronic states are calculated using the two-electron \textit{R}-matrix method [M. Tarana, R. \v{C}ur\'{i}k, Phys. Rev. A \textbf{93}, 012515 (2016)] for the…

原子物理 · 物理学 2020-12-03 Michal Tarana

Trilobite molecules are ultralong-range Rydberg molecules formed when a high angular momentum Rydberg electron scatters off of a ground-state atom. Their unique electronic structure and highly oscillatory potential energy curves support a…

原子物理 · 物理学 2024-12-31 Rohan Srikumar , Seth T. Rittenhouse , Peter Schmelcher

A generalized class of ultra-long-range Rydberg molecules is proposed which consist of a multichannel Rydberg atom whose outermost electron creates a chemical bond with a distant ground state atom. Such multichannel Rydberg molecules…

原子物理 · 物理学 2015-11-11 Matthew T. Eiles , Chris H. Greene
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