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Anisotropic open shell 4f ions have magnetic moments that can be read and written as atomic bits. If it comes to qbits where the phase of the wave function has to be written, controlled and read, it is of advantage to rely on more than one…

量子物理 · 物理学 2024-03-14 Thomas Greber

A Mn4 single-molecule magnet (SMM) is used to show that quantum tunneling of magnetization (QTM) is not suppressed by moderate three dimensional exchange coupling between molecules. Instead, it leads to an exchange bias of the quantum…

介观与纳米尺度物理 · 物理学 2009-11-10 R. Tiron , W. Wernsdorfer , N. Aliaga-Alcalde , D. N. Hendrickson , G. Christou

The quantum tunneling of the magnetization vector between excited levels are studied theoretically in single-domain ferromagnetic nanoparticles with biaxial crystal symmetry placed in an external magnetic field at an arbitarily directed…

介观与纳米尺度物理 · 物理学 2009-10-31 Rong Lu , Su-Peng Kou , Jia-Lin Zhu , Lee Chang , Bing-Lin Gu

We Have developed the concept of a new kind of single-electron transistor in which the transport of the electron through a quantum wire is controlled by charged quantum rings. Using a 2D harmonic potential as the transverse constraint, we…

介观与纳米尺度物理 · 物理学 2016-10-24 Ali Hosseinzadeh , Shahpoor Saeidian

We theoretically investigate quantum transport through single-molecule magnet (SMM) junctions with ferromagnetic and normal-metal leads in the sequential regime. The current obtained by means of the rate-equation gives rise to the tunneling…

介观与纳米尺度物理 · 物理学 2015-06-05 Haiqing Xie , Qiang Wang , Hujun Jiao , J. -Q. Liang

We demonstrate that in a single molecule magnet (SMM) strongly coupled to electrodes the Kondo effect involves all magnetic excitations. This Kondo effect is induced by the quantum tunneling of the magnetic moment (QTM). Importantly, the…

强关联电子 · 物理学 2009-11-11 C. Romeike , M. R. Wegewijs , W. Hofstetter , H. Schoeller

Inspired by cotunneling spectroscopy of spin-states in a single OPE5-based molecule, we investigate the prospects for electric control of magnetism in purely organic molecules contacted in a three-terminal geometry. Using the gate…

介观与纳米尺度物理 · 物理学 2012-12-21 J. Fock , M. Leijnse , K. Jennum , A. S. Zyazin , J. Paaske , P. Hedegård , M. Brøndsted Nielsen , H. S. J. van der Zant

We theoretically study the spin-polarized transport through a single-molecule magnet, which is weakly coupled to ferromagnetic leads, by means of the rate-equation approach. We consider both the ferromagnetic and antiferromagnetic…

介观与纳米尺度物理 · 物理学 2012-03-22 Haiqing Xie , Qiang Wang , Bo Chang , Hujun Jiao , J. -Q. Liang

One of the long-standing goals of quantum transport is to use the noise, rather than the average current, for information processing. However, achieving this requires on-demand control of quantum fluctuations in the electric current. In…

介观与纳米尺度物理 · 物理学 2021-05-12 Nicholas S. Davis , Samuel L. Rudge , Daniel S. Kosov

A new family of supramolecular, antiferromagnetically exchange-coupled dimers of single-molecule magnets (SMMs) has recently been reported [W. Wernsdorfer, N. Aliaga-Alcalde, D.N. Hendrickson, and G. Christou, Nature 416, 406 (2002)]. Each…

介观与纳米尺度物理 · 物理学 2009-11-10 R. Tiron , W. Wernsdorfer , D. Foguet-Albiol , N. Aliaga-Alcalde , G. Christou

By measuring electron tunneling between a ferromagnet and individual energy levels in an aluminum quantum dot, we show how spin-resolved quantum states can be used as filters to determine spin-dependent tunneling rates. We also observe…

介观与纳米尺度物理 · 物理学 2009-11-07 Mandar M. Deshmukh , D. C. Ralph

The effects of a turnstile operation on the current-induced vibron dynamics in nanoelectromechanical systems (NEMS) are analyzed in the framework of the generalized master equation. In our simulations each turnstile cycle allows the pumping…

介观与纳米尺度物理 · 物理学 2020-05-22 R. Dragomir , V. Moldoveanu , S. Stanciu , B. Tanatar

Electron transport is theoretically investigated in a molecular device made of anthracene molecule attached to the electrodes by thiol end groups in two different configurations (para and meta, respectively). Molecular system is described…

介观与纳米尺度物理 · 物理学 2007-05-23 Kamil Walczak

We explore theoretically the spin transport in nanostructures consisting of a gold quantum dot bridging nonmagnetic electrodes and two Mn12-Ph single molecule magnets (SMMs) that are thiol-bonded to the dot but are not in direct contact…

介观与纳米尺度物理 · 物理学 2015-06-15 Fatemeh Rostamzadeh Renani , George Kirczenow

We demonstrate that transport spectroscopy of single molecular magnets shows signatures of quantum tunneling at low temperatures. We find current and noise oscillations as function of bias voltage due to a weak violation of spin selection…

强关联电子 · 物理学 2009-11-11 C. Romeike , M. R. Wegewijs , H. Schoeller

Controlling electronic transport through a single-molecule junction is crucial for molecular electronics or spintronics. In magnetic molecular devices, the spin degree-of-freedom can be used to this end since the magnetic properties of the…

The electric control of quantum spin chains has been an outstanding goal for the few last years due to its potential use in technologies related to quantum information processing. In this work, we show the feasibility of the different steps…

量子物理 · 物理学 2024-08-14 Diego Acosta Coden , Omar Osenda , Alejandro Ferrón

Tunneling of electrons through rotor-stator anthracene aldehyde molecular interfaces is studied with a combined ab initio and model approach. Molecular electronic structure calculated from first principles is utilized to model different…

化学物理 · 物理学 2016-05-27 Irina Petreska , Vladimir Ohanesjan , Ljupco Pejov , Ljupco Kocarev

We study single-electron transport in a three-ion molecule with strong uniaxial anisotropy and in the presence of a transverse magnetic field. Two magnetic ions are connected to each other through a third, nonmagnetic ion. The magnetic ions…

介观与纳米尺度物理 · 物理学 2014-05-12 Javier I. Romero , Eduardo R. Mucciolo

Spin-ordered states close to metal-insulator transitions are poorly understood theoretically and challenging to probe in experiments. Here, we propose that the quantum twisting microscope, which provides direct access to the energy-momentum…

强关联电子 · 物理学 2024-07-11 Fabian Pichler , Wilhelm Kadow , Clemens Kuhlenkamp , Michael Knap