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We present time-of-flight inelastic neutron scattering measurements at low temperature on powder samples of the magnetic pyrochlore oxides Tb2Ti2O7 and Tb2Sn2O7. These two materials possess related, but different ground states, with…

Pyrochlores offer an ideal playground to investigate the magnetic ground state of frustrated magnetic systems. In this class of materials, competition between various magnetic interactions remains frustrated and prevents an ordered magnetic…

强关联电子 · 物理学 2022-10-06 Karan Singh , Dheeraj Ranaut , G. Sharma , K. Mukherjee

A quantum spin liquid is a novel state of matter characterized by quantum entanglement and the absence of any broken symmetry. In condensed matter, the frustrated rare-earth pyrochlore magnets Ho$_2$Ti$_2$O$_7$ and Dy$_2$Ti$_2$O$_7$,…

强关联电子 · 物理学 2017-04-05 E. Kermarrec , J. Gaudet , K. Fritsch , R. Khasanov , Z. Guguchia , C. Ritter , K. A. Ross , H. A. Dabkowska , B. D. Gaulin

The pyrochlore magnet $\rm Yb_2Ti_2O_7$ has been proposed as a quantum spin ice candidate, a spin liquid state expected to display emergent quantum electrodynamics with gauge photons among its elementary excitations. However, $\rm…

强关联电子 · 物理学 2018-06-20 Gabriele Sala , Dalini D. Maharaj , Matthew B. Stone , Hanna A. Dabkowska , Bruce D. Gaulin

Magnetic-rare-earth pyrochlore iridates exhibit a rich variety of unconventional phases, driven by the complex interactions within and between the rare-earth and the iridium sublattices. In this study, we investigate the peculiar magnetic…

We present an interpretation of zero field diffuse neutron scattering and of high field magnetisation data at very low temperature in the frustrated pyrochlore system Tb2Ti2O7. This material has antiferromagnetic exchange interactions and…

强关联电子 · 物理学 2013-12-16 P. Bonville , A. Gukasov , I. Mirebeau , S. Petit

We report detailed measurements of the low temperature magnetic phase diagram of Er$_2$Ti$_2$O$_7$. Heat capacity and time-of-flight neutron scattering studies of single crystals, subject to magnetic fields applied along the…

We present a model which accounts for the high field magnetisation at very low temperature in two pyrochlore frustrated systems, Er2Ti2O7 and Tb2Ti2O7. The two compounds present very different ground states: Er2Ti2O7, which has a planar…

强关联电子 · 物理学 2015-06-15 Pierre Bonville , Sylvain Petit , Isabelle Mirebeau , Julien Robert , Elsa Lhotel , Carley Paulsen

We report an analysis of neutron diffraction from single crystals of the spin-liquid pyrochlore Tb2Ti2O7 under the application of magnetic fields along the crystallographic $[110]$ direction. Such a perturbation has been shown to destroy…

强关联电子 · 物理学 2009-11-17 J. P. C. Ruff , B. D. Gaulin , K. C. Rule , J. S. Gardner

Neutron scattering experiments on a polycrystalline sample of the frustrated pyrochlore magnet Tb2Ti2O7, which does not show any magnetic order down to 50 mK, have revealed that it shows condensation behavior below 0.4 K from a thermally…

无序系统与神经网络 · 物理学 2011-12-13 Hiroshi Takatsu , Hiroaki Kadowaki , Taku J. Sato , Jeffrey W. Lynn , Yoshikazu Tabata , Teruo Yamazaki , Kazuyuki Matsuhira

Magnetic pyrochlores with non-Kramers rare-earth ions provide a platform for exploring emergent gauge physics and quantum spin-ice behavior, yet the influence of structural disorder on their ground states remains insufficiently understood.…

We report the low temperature magnetic properties of the pyrochlore Pr$_2$Hf$_2$O$_7$. Polycrystalline and single-crystal samples are investigated using time-of-flight neutron spectroscopy and macroscopic measurements, respectively. The…

The Tb$_2$Ti$_2$O$_7$ pyrochlore magnetic material is attracting much attention for its {\em spin liquid} state, failing to develop long range order down to 50 mK despite a Curie-Weiss temperature $\theta_{\rm CW} \sim -14$ K. In this paper…

统计力学 · 物理学 2007-05-23 Hamid R. Molavian , Michel J. P. Gingras , Benjamin Canals

The low-temperature thermodynamic properties of the frustrated pyrochlore Tb$_{2+x}$Ti$_{2-x}$O$_{7+y}$ have been studied using the single crystal of $x=0.005$ sitting in a long range ordered phase in the $x$-$T$ phase diagram. We observed…

强关联电子 · 物理学 2017-04-25 H. Takatsu , T. Taniguchi , S. Kittaka , T. Sakakibara , H. Kadowaki

Static and dynamical properties of the magnetic moment system of pyrochlore compound Tb2Ti2O7 with strong magnetic frustration, have been investigated down to the temperature T=0.4 K by neutron scattering on a single crystal sample. The…

We report an extensive study on the zero field ground state of a powder sample of the pyrochlore $\mathrm{Yb_2Ti_2O_7}$. A sharp heat capacity anomaly that labels a low temperature phase transition in this material is observed at 280 mK.…

We report time-of-flight neutron scattering measurements of the magnetic spectrum of Tb3+ in Tb2Ti2O7. The data, which extend up to 120 meV and have calibrated intensity, enable us to consolidate and extend previous studies of the…

强关联电子 · 物理学 2015-09-04 A. J. Princep , H. C. Walker , D. T. Adroja , D. Prabhakaran , A. T. Boothroyd

By means of ac magnetic-susceptibility measurements, we find evidence for a new magnetic phase of Tb$_2$Ti$_2$O$_7$ below about 140 mK in zero magnetic field. In magnetic fields parallel to [111], this phase---exhibiting frequency- and…

强关联电子 · 物理学 2015-06-05 L. Yin , J. S. Xia , Y. Takano , N. S. Sullivan , Q. J. Li , X. F. Sun

The low temperature magnetic properties of pyrochlore compound Dy2Ti2O7 in magnetic fields applied along the [111] direction are reported. Below 1 K, a clear plateau has been observed in the magnetization process in the field range 2~9 kOe,…

材料科学 · 物理学 2009-11-07 Kazuyuki Matsuhira , Zenji Hiroi , Takashi Tayama , Seishi Takagi , Toshiro Sakakibara

Neutron scattering measurements on the pyrochlore magnet Ce$_2$Zr$_2$O$_7$ reveal an unusual crystal field splitting of its lowest $J$=5/2 multiplet, such that its ground state doublet is composed of m$_J$=$\pm$3/2, giving these doublets a…

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