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Monte Carlo simulation on the crystallization of double crystalline diblock copolymer unravels an intrinsic relationship between block asymmetry and crystallization behaviour. We model crystalline A-B diblock copolymer, wherein the melting…

软凝聚态物质 · 物理学 2015-06-19 Chitrita Kundu , Ashok Kumar Dasmahapatra

Polymer blends offer an exciting material for various potential applications due to their tunable properties by varying constituting components and their relative composition. Our simulation results unravel an intrinsic relationship between…

软凝聚态物质 · 物理学 2016-10-13 Ashok Kumar Dasmahapatra

Diblock copolymers by virtue of the chemical dissimilarity between the constituting blocks exhibit microphase separation in the melt state. The phase separated melt can successfully be exploited to control the morphology of the final semi…

软凝聚态物质 · 物理学 2018-02-19 Chitrita Kundu , Nikhil S. Joshi , Ashok Kumar Dasmahapatra

Based upon kinetic Monte Carlo simulations of crystallization in a simple polymer model we present a new picture of the mechanism by which the thickness of lamellar polymer crystals is constrained to a value close to the minimum…

凝聚态物理 · 物理学 2007-05-23 Jonathan Doye , Daan Frenkel

Crystallization within the discrete spheres of a block copolymer mesophase was studied by time-resolved x-ray scattering. The cubic packing of microdomains, established by self-assembly in the melt, is preserved throughout crystallization…

软凝聚态物质 · 物理学 2009-10-31 Yueh-Lin Loo , Richard A. Register , Anthony J. Ryan

In the present work, crystallization in melts and poor-solvent solutions of semiflexible polymers with different concentration was studied by means of dissipative particle dynamics simulation technique. We use a coarse-grained polymer model…

化学物理 · 物理学 2020-01-30 P. I. Kos , V. A. Ivanov , A. V. Chertovich

Experimental and modeling/simulation studies of phase equilibrium and growth morphologies of novel polymer-dispersed liquid crystal (PDLC) mixtures of PS (polystyrene) and liquid crystals that exhibit a direct isotropic/smectic-A (lamellar)…

软凝聚态物质 · 物理学 2015-05-13 Ezequiel R. Soule , Nasser Mohieddin Abukhdeir , Alejandro D. Rey

We present a kinetic model of crystal growth of polymers of finite molecular weight. Experiments help to classify polymer crystallization broadly into two kinetic regimes. One is observed in melts or in high molar mass polymer solutions and…

软凝聚态物质 · 物理学 2009-11-11 Arindam Kundagrami , M. Muthukumar

Investigating thermodynamic properties of liquid-solid transitions of flexible homopolymers with elastic bonds by means of multicanonical Monte Carlo simulations, we find crystalline conformations that resemble ground-state structures of…

软凝聚态物质 · 物理学 2010-02-11 Stefan Schnabel , Thomas Vogel , Michael Bachmann , Wolfhard Janke

The crystallization of a metastable melt is one of the most important non equilibrium phenomena in condensed matter physics, and hard sphere colloidal model systems have been used for several decades to investigate this process by…

软凝聚态物质 · 物理学 2015-05-20 Tanja Schilling , Sven Dorosz , Hans Joachim Schoepe , George Opletal

We perform molecular dynamics (MD) simulations of the crystallization process in binary Lennard-Jones systems during heating and cooling to investigate atomic-scale crystallization kinetics in glass-forming materials. For the cooling…

软凝聚态物质 · 物理学 2015-06-23 Minglei Wang , Kai Zhang , Zhusong Li , Yanhui Liu , Jan Schroers , Mark D. Shattuck , Corey S. O'Hern

We investigate the phase behavior of symmetric AB diblock copolymers confined into a thin film. The film boundaries are parallel, impenetrable and attract the A component of the diblock copolymer. Using a self-consistent field technique…

统计力学 · 物理学 2009-10-31 Thorsten Geisinger , Marcus Mueller , Kurt Binder

Using Monte Carlo simulations we study crystallization in the three-dimensional Ising model with four-spin interaction. We monitor the morphology of crystals which grow after placing crystallization seeds in a supercooled liquid. Defects in…

材料科学 · 物理学 2009-11-07 A. Lipowski , D. Johnston

We investigate the finite-temperature phase diagram of polar molecules confined in a quasi-two-dimensional geometry by a harmonic potential along the polarization axis. We employ Quantum Monte Carlo simulations to explore the strongly…

量子气体 · 物理学 2026-05-19 Vinicius Zampronio , Matteo Ciardi , Fabio Cinti

The coil-globule transition has been studied for A-B copolymer chains both by means of lattice Monte Carlo simulations using bond fluctuation algorithm and by a numerical self-consistent field method. Copolymer chains of fixed length with A…

The process of homogeneous crystal nucleation has been considered in a model liquid, where the interparticle interaction is described by a short-range spherical oscillatory potential. Mechanisms of initiating structural ordering in the…

材料科学 · 物理学 2018-12-18 Bulat N. Galimzyanov , Dinar T. Yarullin , Anatolii V. Mokshin

It has been revealed by mean-field theories and computer simulations that the nature of the collapse transition of a polymer is influenced by its bending stiffness $\epsilon_{\rm b}$. In two dimensions, a recent analytical work demonstrated…

软凝聚态物质 · 物理学 2009-11-13 Jie Zhou , Zhong-Can Ou-Yang , Haijun Zhou

Kinetic barriers cause polymers to crystallize incompletely, into nanoscale lamellae interleaved with amorphous regions. As a result, crystalline polymers are full of crystal-melt interfaces, which dominate their physical properties. The…

软凝聚态物质 · 物理学 2010-09-23 Scott T. Milner

Polymers with both soluble and insoluble blocks typically self-assemble into micelles, aggregates of a finite number of polymers where the soluble blocks shield the insoluble ones from contact with the solvent. Upon increasing…

软凝聚态物质 · 物理学 2009-11-13 J. A. Anderson , C. D. Lorenz , A. Travesset

We systematically study the relationship between equilibrium and non-equilibrium phase diagrams of a system of short-ranged attractive colloids. Using Monte Carlo and Brownian dynamics simulations we find a window of enhanced…

软凝聚态物质 · 物理学 2009-11-13 Andrea Fortini , Eduardo Sanz , Marjolein Dijkstra
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