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In this study, we synthesized single crystals of Na$_{x}$CoO$_{2}$ with $x\sim0.8$ using the optical floating zone technique. A thorough electrochemical treatment of the samples permitted us to control the de-intercalation of Na to obtain…

强关联电子 · 物理学 2018-06-18 I. F. Gilmutdinov , I. R. Mukhamedshin , F. Rullier-Albenque , H. Alloul

We have investigated the influence of Ca ions substitution on the structural and superconducting properties of (Nd1-xCax)(Ba1.6La0.4)Cu3Oz system. Magnetization, X-ray diffraction and neutron diffraction studies have been carried out on a…

超导电性 · 物理学 2010-05-14 Amish G. Joshi , R. G. Kulkarni , W. B. Yelon , Ram Prasad , M. R. Gonal

We have successfully grown single crystalline NaFeAs with cobalt or phosphor doping. Bulk superconductivity occurs in NaFe$_{0.95}$Co$_{0.05}$As at 19 K while much higher transition temperature is observed in NaFeAs$_{0.8}$P$_{0.2}$, in…

超导电性 · 物理学 2010-02-03 T. -L. Xia , J. B. He , D. M. Wang , G. F. Chen

We report the synthesis and superconducting properties of a metastable form of the known superconductor NaxCoO2*yH2O (x ~ 1/3, y ~ 4x). Instead of using the conventional bromine-acetonitrile mixture for sodium deintercalation, we use an…

材料科学 · 物理学 2009-11-11 P. W. Barnes , M. Avdeev , J. D. Jorgensen , D. G. Hinks , H. Claus , S. Short

We report the electrical, magnetic and thermal measurements on a layered cobalt oxyhydrate Na$_{0.31}$CoO$_{2}\cdot$1.3H$_{2}$O. Bulk superconductivity at 4.3 K has been confirmed, however, the measured superconducting fraction is…

超导电性 · 物理学 2009-11-10 Guanghan Cao , Chunmu Feng , Yi Xu , Wen Lu , Jingqin Shen , Minghu Fang , Zhu'an Xu

A systematic study of NaxCoO2 (x=0.50 - 0.90) and NaxCoO2 yH(D)2O (x=0.26 - 0.42, y=1.3) has been performed to determine phase stability and the effect of hydration on the structural and superconducting properties of this system. We show…

超导电性 · 物理学 2009-11-10 D. P. Chen , H. C. Chen , A. Maljuk , A. Kulakov , H. Zhang , P. Lemmens , C. T. Lin

Soda-lime-silica is a glassy system of strong industrial interest. In order to characterize its liquid state properties, we performed molecular dynamics simulations employing an aspherical ion model that includes atomic polarization and…

We have carried out systematic temperature-dependent neutron diffraction measurements in conjunction with dielectric spectroscopy from 6 to 300 K for sodium niobate based compounds (1-x) NaNbO3 -xBaTiO3 (NNBTx). The dielectric constant is…

材料科学 · 物理学 2018-05-23 S. K. Mishra , Mrinal Jauhari , R. Mittal , P. S. R. Krishna , V. R. Reddy , S. L. Chaplot

By tuning the physical and chemical pressures of layered perovskite materials we can realize the quantum states of both superconductors and insulators. By reducing the thickness of a layered crystal to a nanometer level, a nanofilm crystal…

Poly- and single-crystalline Na$_x$CoO$_2$ has been successfully intercalated with H$_2$O and D$_2$O as confirmed by X-ray diffraction and thermogravimetric analysis. Resistivity, magnetic susceptibility, and specific heat measurements show…

超导电性 · 物理学 2009-11-10 R. Jin , B. C. Sales , P. Khalifah , D. Mandrus

A single crystal of GdBaCo2O5.47(2) has been studied by means of X-ray diffraction. Appearance of superstructure reflections at T = 341.5(7) K gives an evidence of continuous transition to the phase with unit cell doubled along the shortest…

We report the presence of a correlation between the bulk and interfacial properties of electrostatic coacervate complexes. Complexes were obtained by co-assembly between cationic-neutral diblocks and oppositely charged surfactant micelles…

软凝聚态物质 · 物理学 2007-10-12 Ling Qi , Jean-Paul Chapel , Jean-Christophe Castaing , Jerome Fresnais , Jean-Francois Berret

A series of CaxCoO2 (0.15 <= x <= 0.40) materials have been prepared by means of ion exchange reaction from NaxCoO2. Transmission electron microscopy (TEM) measurements revealed a rich variety of structural phenomena resulting from cation…

强关联电子 · 物理学 2009-11-11 H. X. Yang , Y. G. Shi , X. Liu , R. J. Xiao , H. F. Tian , J. Q. Li

The crystal structure of Na0.5CoO2, determined by powder neutron diffraction, is reported. The structure consists of layers of edge-shared CoO6 octahedra in a triangular lattice, with Na ions occupying ordered positions in the interleaving…

强关联电子 · 物理学 2009-11-10 Q. Huang , M. L. Foo , J. W. Lynn , H. W. Zandbergen , G. Lawes , Yayu Wang , B. H. Toby , A. P. Ramirez , N. P. Ong , R. J. Cava

$Na_xCoO_2$ that comprises of alternating Na and $CoO_2$ layers has exotic magnetic and thermoelectric properties that could favorably be manipulated by adding dopants or varying Na concentration. In this work, we investigated the…

材料科学 · 物理学 2019-02-27 M. H. N. Assadi , H. Katayama-Yoshida

Doping is considered to be the main method for improving the thermoelectric performance of layered sodium cobaltate (Na$_{1-x}$CoO$_2$). However, in the vast majority of past reports, the equilibrium location of the dopant in the…

材料科学 · 物理学 2021-06-25 M. Hussein N. Assadi

We present high energy X-ray diffraction studies on the structural phases of an optimal high-$T_c$ superconductor La$_{2-x}$Sr$_x$CuO$_{4+y}$ tailored by co-hole-doping. This is specifically done by varying the content of two very different…

X-ray diffraction experiments were performed on polycrystalline and single-crystal specimens of Ce$_{2}$Fe$_{17}$ at temperatures between 10 K and 300 K. Below $T_{\mathrm{t}}$ = 118$\pm$2 K, additional weak superstructure reflections were…

We theoretically investigate the possibility of achieving a superconducting state in transition-metal dichalcogenide bilayers through intercalation, a process previously and widely used to achieve metallization and superconducting states in…

超导电性 · 物理学 2017-09-20 R. Szczesniak , A. P. Durajski , M. W. Jarosik

The NaNO$_{2}$ nanocomposite ferroelectric material in porous glass was studied by neutron diffraction. For the first time the details of the crystal structure including positions and anisotropic thermal parameters were determined for the…