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We report a combined experimental and theoretical investigation of the magnetic structure of the honeycomb lattice magnet Na$_2$IrO$_3$, a strong candidate for a realization of a gapless spin-liquid. Using resonant x-ray magnetic scattering…

In this work, we investigate the microscopic nature of the magnetism in honeycomb iridium-based systems by performing a systematic study of how the effective magnetic interactions in these compounds depend on various electronic microscopic…

强关联电子 · 物理学 2015-06-22 Yuriy Sizyuk , Craig Price , Peter Wölfle , Natalia B. Perkins

We report the structure, magnetic, and thermal property measurements on single crystalline and polycrystalline samples of Ru substituted honeycomb lattice iridate Na$_2$Ir$_x$Ru$_{1-x}$O$_3$ (x = 0, 0.05, 0.1, 0.15, 0.2, 0.3, 0.5). The…

强关联电子 · 物理学 2015-10-20 Kavita Mehlawat , Yogesh Singh

We have combined single crystal neutron and x-ray diffractions to investigate the magnetic and crystal structures of the honeycomb lattice $\rm Na_2IrO_3$. The system orders magnetically below $18.1(2)$ K with Ir$^{4+}$ ions forming zigzag…

Honeycomb iridate Na2IrO3, a Jeff=1/2 magnet, is a potential platform for realizing the quantum spin liquid. Many experiments have shown that its magnetic ground state has a zigzag antiferromagnetic (AFM) order. However, there is still a…

强关联电子 · 物理学 2018-09-05 Y. S. Hou , J. H. Yang , H. J. Xiang , X. G. Gong

We report inelastic neutron scattering measurements on Na2IrO3, a candidate for the Kitaev spin model on the honeycomb lattice. We observe spin-wave excitations below 5 meV with a dispersion that can be accounted for by including…

We have synthesized single crystals of Na$_3$Co$_2$SbO$_6$ and characterized the structure and magnetic order by measuring anisotropic magnetic properties, heat capacity, x-ray and neutron single crystal diffraction. Magnetic properties and…

强关联电子 · 物理学 2019-07-17 J. -Q. Yan , S. Okamoto , Y. Wu , Q. Zheng , H. D. Zhou , H. B. Cao , M. A. McGuire

The magnetic orders in Na$_2$IrO$_3$ and $\alpha-$RuCl$_3$, honeycomb systems with strong spin-orbit coupling and correlations, have been recently described by models with the dominant Kitaev interactions. In this work we discuss how the…

强关联电子 · 物理学 2017-02-10 Yuriy Sizyuk , Peter Woelfle , Natalia B. Perkins

We explore the phase diagram of spin-orbit Mott insulators on a honeycomb lattice, within the Kitaev-Heisenberg model extended to its full parameter space. Zigzag-type magnetic order is found to occupy a large part of the phase diagram of…

强关联电子 · 物理学 2013-03-19 Jiří Chaloupka , George Jackeli , Giniyat Khaliullin

The honeycomb iridates A2IrO3 (A=Na, Li) constitute promising candidate materials to realize the Heisenberg-Kitaev model (HKM) in nature, hosting unconventional magnetic as well as spin liquid phases. Recent experiments suggest, however,…

强关联电子 · 物理学 2015-06-19 Johannes Reuther , Ronny Thomale , Stephan Rachel

The layered honeycomb magnet $\alpha$-Li$_2$IrO$_3$ has been theoretically proposed as a candidate to display novel magnetic behaviour associated with Kitaev interactions between spin-orbit entangled $j_{\rm eff}=1/2$ magnetic moments on a…

The nature of magnetism in the intercalated honeycomb iridate Ag$_3$LiIr$_2$O$_6$ has been a subject of recent intensive debate, where the absence or presence of antiferromagnetic order has been reported to be related to possible structural…

强关联电子 · 物理学 2022-03-28 Ying Li , Roser Valenti

The magnetic field response of the Mott-insulating honeycomb iridate Na$_{2}$IrO$_{3}$ is investigated using torque magnetometry measurements in magnetic fields up to 60 tesla. A peak-dip structure is observed in the torque response at…

Materials that realize Kitaev spin models with bond-dependent anisotropic interactions have long been searched for, as the resulting frustration effects are predicted to stabilize novel forms of magnetic order or quantum spin liquids. Here…

强关联电子 · 物理学 2014-11-11 A. Biffin , R. D. Johnson , I. Kimchi , R. Morris , A. Bombardi , J. G. Analytis , A. Vishwanath , R. Coldea

The crystal structure, magnetic ground state, and the temperature dependent microscopic spin-spin correlations of the frustrated honeycomb lattice antiferromagnet Na2Co2TeO6 have been investigated by powder neutron diffraction. A three…

强关联电子 · 物理学 2017-03-29 A. K. Bera , S. M. Yusuf , Amit Kumar , C. Ritter

We have successfully synthesized the novel antiferromagnets with Ir$^{4+}$ honeycomb lattice ZnIrO$_3$ and MgIrO$_3$ and investigated their magnetic and thermodynamic properties. The two iridates are isomorphic but exhibit qualitatively…

We report the successful synthesis of single-crystals of the layered iridate, (Na$_{1-x}$Li$_{x}$)$_2$IrO$_3$, $0\leq x \leq 0.9$, and a thorough study of its structural, magnetic, thermal and transport properties. The new compound allows a…

强关联电子 · 物理学 2014-01-07 G. Cao , T. F. Qi , L. Li , J. Terzic , V. S. Cao , S. J. Yuan , M. Tovar , G. Murthy , R. K. Kaul

We report the magnetic structure and properties of a thiocyanate-based honeycomb magnet [Na(OH$_2$)$_3$]Mn(NCS)$_3$ which crystallises in the unusual low-symmetry trigonal space group $P\overline{3}$. Magnetic measurements on powder samples…

Na$_2$IrO$_3$, a honeycomb 5$d^5$ oxide, has been recently identified as a potential realization of the Kitaev spin lattice. The basic feature of this spin model is that for each of the three metal-metal links emerging out of a metal site,…

We report magnetization and neutron diffraction studies on crystal and magnetic structures of Ir- and Rh-substituted honeycomb lattice $\alpha$-RuCl$_3$. The iridium or rhodium atoms are distributed at the Ru site with little structural…

材料科学 · 物理学 2023-10-05 Zachary Morgan , Iris Ye , Colin L. Sarkis , Xiaoping Wang , Stephen Nagler , Jiaqiang Yan
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