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Gas phase density-functional theory (DFT) and time-dependent DFT (TD-DFT) calculations are reported for a data base of 98 ruthenium(II) polypyridine complexes. Comparison with X-ray crystal geometries and with experimental absorption…

化学物理 · 物理学 2023-11-06 Denis Magero , Mark E. Casida , George Amolo , Nicholas Makau , Lusweti Kituyi

We review theories of phosphorescence in cyclometalated complexes. We focus primarily on pseudooctahedrally coordinated $t_{2g}^6$ metals (e.g., [Os(II)(bpy)$_3$]$^{2+}$, Ir(III)(ppy)$_3$ and Ir(III)(ptz)$_3$) as, for reasons that are…

化学物理 · 物理学 2015-04-02 B. J. Powell

The dominant majority of the hundreds of available spin-crossover compounds, including the technologically most promising ones, are based on the Earth-abundant metal iron, making these switches particularly appealing in terms of sustainable…

其他凝聚态物理 · 物理学 2020-07-24 Latévi Max Lawson Daku , Mark Earl Casida

Iridium-based photosensitizers have attracted significant attention in photodynamic therapy (PDT) due to their exceptional photophysical properties and chemical stability, as well as tunable phosphorescence emission spectrum and high…

化学物理 · 物理学 2026-05-08 Aynur Matyusup , Jia-ying Zhao , Yu-dan Zhang , Qi Zhaoa , Ai-min Ren , Jing-fu Guo

The development of photonic integrated circuits would benefit from a wider selection of materials that can strongly-control near-infrared (NIR) light. Transition metal dichalcogenides (TMDs) have been explored extensively for visible…

介观与纳米尺度物理 · 物理学 2019-10-18 Akshay Singh , Yifei Li , Balint Fodor , Laszlo Makai , Jian Zhou , Haowei Xu , Austin Akey , Ju Li , R. Jaramillo

In transition-metal compounds, the transition-metal d electrons play an important role in their physical properties; however, the effects of the electron correlation between the ligand p electrons have not been clear yet. In this Letter,…

Pyrene-functionalized materials are extensively employed in photoluminescent applications, owing to their extended {\pi}-conjugation and favorable photophysical properties. However, their luminescent performance is often attenuated by…

化学物理 · 物理学 2025-12-01 Wenlong Li , Stephen Awuku , Jenna N. Merk , Marc R. MacKinnon , Amy L. Stevens

The scientific community has witnessed tremendous expansion of research on layered (i.e. two-dimensional, 2D) materials, with increasing recent focus on applications to photonics. Layered materials are particularly exciting for manipulating…

材料科学 · 物理学 2020-11-17 Akshay Singh , Seong Soon Jo , Yifei Li , Changming Wu , Mo Li , R. Jaramillo

Density functional theory (DFT) based modeling of electronic excited states is of importance for investigation of the photophysical/photochemical properties and spectroscopic characterization of large systems. The widely used linear…

化学物理 · 物理学 2021-05-11 Diptarka Hait , Martin Head-Gordon

The nonlinear optics and optical limiting properties of materials based on multifunctional fullerenol and poly(styrene-co-4-vinylpyridine) matrix were studied using 7 ns pulses of nanosecond laser operating at 532 nm wavelength. The…

可精确求解与可积系统 · 物理学 2009-11-07 Hendry Izaac Elim , Wei Ji , Gwee Chen Meng , Jianying Ouyang , Suat Hong Goh

In recent years, enhanced light-matter interactions through a plethora of dipole-type polaritonic excitations have been observed in two-dimensional (2D) layered materials. In graphene, electrically tunable and highly confined…

Strong optical pulses at mid-infrared and terahertz frequencies have recently emerged as a powerful tool to manipulate and control the solid state and especially complex condensed matter systems with strongly correlated electrons. The…

强关联电子 · 物理学 2016-08-22 Daniele Nicoletti , Andrea Cavalleri

The systematic trends in structural and electronic properties of perylene diimide (PDI) derived dye molecules have been investigated by DFT calculations based on projector augmented wave (PAW) method including gradient corrected…

材料科学 · 物理学 2008-01-15 E. Mete , D. Uner , M. Cakmak , O. Gulseren , S. Ellialtioglu

Long-lived emissive materials based on room temperature phosphorescence (RTP) and thermally activated delayed fluorescence (TADF) are considered as the cornerstone of the development of optical sensors, security systems and solid-state…

材料科学 · 物理学 2021-10-26 Mario Gutiérrez , Cristina Martín , Johan Hofkens , Jin-Chong Tan

Organic--inorganic complexes are promising materials for light-emitting applications. Here, we report a new organometallic complex, cis-[Cd(Tz)$_2$(py)$_2$], featuring a distorted octahedral Cd(II) coordination environment. IR and Raman…

Lanthanide-based emitters are attracting increasing interest for their potential in high-performance OLEDs due to their narrow emission bands, high photostability, and functional versatility. However, their low radiative rates and poor…

Condensed-matter provides attractive platforms to realize exotic particles, originally proposed in high-energy physics. Weyl semimetal (WSM) is a material in which low-energy collective excitations are governed by massless Weyl fermions,…

介观与纳米尺度物理 · 物理学 2025-01-20 Amar Bharti

In recent years, the need for high-power laser is of great interest for different applications ranging from direct-laser processing, light detection, medicine, and lighting. However, high-power lasers with high intensities give rise to…

光学 · 物理学 2021-01-06 Liyi Hsu , Abdoulaye Ndao

Thermally stable polymers have attracted a lot of interest due to their potential use as the active component in electronic, optical and optoelectronic applications, such as light-emitting diodes, light emitting electrochemical cells,…

其他凝聚态物理 · 物理学 2007-05-23 O. S. Prelipceanu , M. Prelipceanu , O. G. Tudose , B. Grimm , S. Schrader

Two dimensional materials such as graphene and transition metal dichalcogenides (TMDs) are promising for optical modulation, detection, and light emission since their material properties can be tuned on-demand via electrostatic doping. The…

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