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We discuss photo-luminescence characteristics of CdSe core/shell quantum dots at cryogenic temperatures using a hybrid system of a single quantum dot and an optical nanofiber. The key point is to control the emission species of quantum dot…

介观与纳米尺度物理 · 物理学 2022-06-27 K. Muhammed Shafi , Kazunori Iida , Emi Tsutsumi , Akiharu Miyanaga , Kohzo Hakuta

By performing spectroscopic single-particle measurements at cryogenic temperatures over the course of hours we study %By performing spectroscopic longtime single-particle measurements at cryogenic temperatures we study both the spectral…

介观与纳米尺度物理 · 物理学 2017-11-13 Sven-Hendrik Lohmann , Christian Strelow , Alf Mews , Tobias Kipp

Electron transfer to an individual quantum dot promotes the formation of charged excitons with enhanced recombination pathways and reduced lifetimes. Excitons with only one or two extra charges have been observed and exploited for very…

The blinking dynamics of colloidal core-shell CdSe/CdS dot-in-rods is studied in detail at the single particle level. Analyzing the autocorrelation function of the fluorescence intensity, we demonstrate that these nanoemitters are…

Upon photo- or electrical-excitation, colloidal quantum dots (QDs) are often found in multi-carrier states due to multi-photon absorption and photo-charging of the QDs. While many of these multi-carrier states are observed in single-dot…

Correlation between the rectilinear polarisations of the photons emitted from the biexciton decay in a single quantum dot is investigated in a device which allows the charge-state of the dot to be controlled. Optimising emission from the…

We have observed strong photoluminescence from a single CdSe quantum dot embedded in a ZnSe nanowire. Exciton, biexciton and charged exciton lines have been identified unambiguously using photon correlation spectroscopy. This technique has…

We report semi-empirical pseudopotential calculations of emission spectra of charged excitons and biexcitons in CdSe nanocrystals. We find that the main emission peak of charged multiexcitons - originating from the recombination of an…

材料科学 · 物理学 2009-11-11 M. C. Troparevsky , A. Franceschetti

We employ the quantum-jump approach to study single scatterings in single semiconductor quantum dots. Two prototypical situations are investigated. First, we analyze two-photon emissions from the cascade biexciton decay of a dot where the…

介观与纳米尺度物理 · 物理学 2009-11-10 Ulrich Hohenester , Claudia Sifel , Pekka Koskinen

Exciton-phonon coupling limits the homogeneous emission linewidth of nanocrystals. Hence, a full understanding of it is crucial. In this work, we statistically investigate exciton-phonon coupling by performing single-particle spectroscopy…

The optical spectra of CdSe nanocrystals up to 55 A in diameter are analyzed in a wide range of energies from the fine structure of the low-energy excitations to the so-called high-energy transitions. We apply a symmetry-based method in two…

介观与纳米尺度物理 · 物理学 2009-11-07 J. Perez-Conde , A. K. Bhattacharjee

Quantum dots acting as single photon emitters in the blue-green range are fabricated and characterized at cryogenic temperature. They consist in CdSe dots inserted in (Zn,Mg)Se nanowires with a thick shell. Photoluminescence spectra, decay…

We investigate the emission of single photons from CdSe/CdS dot-in-rods which are optically trapped in the focus of a deep parabolic mirror. Thanks to this mirror, we are able to image almost the full 4$\pi$ emission pattern of…

The exciton spin dynamics and polarization properties of the related emission are investigated in colloidal CdSe/CdS dot-in-rod (DiR) and spherical core/shell nanocrystal (NC) ensembles by magneto-optical photoluminescence (PL) spectroscopy…

介观与纳米尺度物理 · 物理学 2015-06-23 B. Siebers , L. Biadala , D. R. Yakovlev , A. V. Rodina , T. Aubert , Z. Hens , M. Bayer

The optical creation and recombination of charged biexciton and trion complexes in an (In,Ga)As/GaAs quantum dot is investigated by micro-photoluminescence spectroscopy. Photon cross-correlation measurements demonstrate the temporally…

其他凝聚态物理 · 物理学 2009-11-10 S. M. Ulrich , M. Benyoucef , P. Michler , N. Baer , P. Gartner , F. Jahnke , M. Schwab , H. Kurtze , M. Bayer , S. Fafard , Z. Wasilewski

We investigate the photon statistics of the light emitted by single self-assembled hybrid gold-CdSe/CdS/CdZnS colloidal nanocrystal supraparticles through the detailed analysis of the intensity autocorrelation function $g^{(2)}(\tau)$. We…

介观与纳米尺度物理 · 物理学 2023-02-16 V. Blondot , D. Gérard , G. Quibeuf , C. Arnold , A. Delteil , A. Bogicevic , T. Pons , N. Lequeux , S. Buil , J-P. Hermier

We study the emission of individual quantum dots in CdTe/ZnTe samples doped with a low concentration of Cr. In addition to dots with a photoluminescence (PL) split by the exchange interaction with a magnetic Cr atom, we observe another type…

介观与纳米尺度物理 · 物理学 2019-11-27 L. Besombes , H. Boukari , V. Tiwari , A. Lafuente-Sampietro , M. Sunaga , K. Makita , S. Kuroda

Spin dynamics of a single electron and an exciton confined in CdTe/ZnTe quantum dot is investigated by polarization-resolved correlation spectroscopy. Spin memory effects extending over at least a few tens of nanoseconds have been directly…

其他凝聚态物理 · 物理学 2008-06-07 J. Suffczynski , K. Kowalik , T. Kazimierczuk , A. Trajnerowicz , M. Goryca , P. Kossacki , A. Golnik , M. Nawrocki , J. A. Gaj

We have theoretically shown that optical properties of semiconductor nanorods are controlled by 1D excitons. The theory, which takes into account anisotropy of spacial and dielectric confinement, describes size dependence of interband…

材料科学 · 物理学 2007-05-23 A. Shabaev , Al. L. Efros

Images of semiconductor `dot in rods' and their small clusters are studied by measuring the second-order correlation function with a spatially resolving ICCD camera. This measurement allows one to distinguish between a single dot and a…

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