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We study the statistical properties of charge and energy transport in electron conducting junctions with electron-phonon interactions, specifically, the thermoelectric efficiency and its fluctuations. The system comprises donor and acceptor…

统计力学 · 物理学 2016-01-20 Bijay Kumar Agarwalla , Jian-Hua Jiang , Dvira Segal

We show that the radiative heat transfer between two solid surfaces at short separation may increase by many order of magnitude when the surfaces are covered by adsorbates. In this case the heat transfer is determined by resonant photon…

材料科学 · 物理学 2009-11-11 A. I. Volokitin , B. N. J. Persson

Recent experiments have demonstrated that vibrational strong coupling (VSC) between molecular vibrations and the optical cavity field can modify vibrational energy transfer (VET) processes in molecular systems. However, the underlying…

化学物理 · 物理学 2024-11-25 Qi Yu , Dong H. Zhang , Joel M. Bowman

Based on the reduced density matrix method, we compare two different approaches to calculate the dynamics of the electron transfer in systems with donor, bridge, and acceptor. In the first approach a vibrational substructure is taken into…

量子物理 · 物理学 2009-10-31 M. Schreiber , D. Kilin , U. Kleinekathoefer

The coherent evolution of the atom-cavity state in bimodal (cavity) experiments has been analyzed for a realistic time-dependence in detuning the atomic transition frequency. Apart from a `smooth switch' of the atomic resonance from one to…

量子物理 · 物理学 2009-11-13 D. Gonta , S. Fritzsche

Vibrationally inelastic electron transport through a molecular bridge that is connected to two leads is investigated. The study is based on a generic model of vibrational excitation in resonant transmission of electrons through a molecular…

介观与纳米尺度物理 · 物理学 2009-11-10 Martin Cizek , Michael Thoss , Wolfgang Domcke

The two-dimensional spectroscopy has recently revealed oscillatory behavior of excitation dynamics in molecular systems. However, in the majority of cases it is strongly debated if excitonic or vibrational wavepackets, or evidences of…

化学物理 · 物理学 2012-11-27 Vytautas Butkus , Donatas Zigmantas , Leonas Valkunas , Darius Abramavicius

We investigate the interplay of quantum interference effects and electronic-vibrational coupling in electron transport through single-molecule junctions, employing a nonequilibrium Green's function approach. Our findings show that inelastic…

介观与纳米尺度物理 · 物理学 2013-02-18 R. Härtle , M. Butzin , M. Thoss

The influence of fast vibrations on energy transfer and conversion in natural molecular aggregates is an issue of central interest. This article shows the important role of high-energy quantized vibrations and their non-equilibrium dynamics…

生物物理 · 物理学 2013-01-30 Avinash Kolli , Edward J. O'Reilly , Gregory D. Scholes , Alexandra Olaya-Castro

Waveguides subject to spatiotemporal modulations are known to exhibit nonreciprocal vibration transmission, whereby interchanging the locations of the source and receiver change the end-to-end transmission characteristics. The scenario of…

应用物理 · 物理学 2025-10-20 Jiuda Wu , Behrooz Yousefzadeh

We consider quantum many body systems as quantum channels and study the relation between the transfer quality and the size of the spectral gap between the system's ground and excited states. In our setup two ancillas are weakly coupled to…

量子物理 · 物理学 2009-11-11 Michael J. Hartmann , Moritz E. Reuter , Martin B. Plenio

The excitation of vibrational modes in molecules affects the outcome of chemical reactions, for example by providing molecules with sufficient energy to overcome activation barriers. In this work, we introduce a quantum algorithm for…

量子物理 · 物理学 2021-12-01 Soran Jahangiri , Juan Miguel Arrazola , Nicolás Quesada , Alain Delgado

It is discussed how vibrationally excited molecules in their electronic ground state can transfer their vibrational energy to the electronic motion of neighbors and ionize them. Based on explicit examples of vibrationally excited molecules…

化学物理 · 物理学 2018-12-05 Lorenz S. Cederbaum

We explore the classical dynamics of two interacting rotating dipoles that are fixed in the space and exposed to an external homogeneous electric field. Kinetic energy transfer mechanisms between the dipoles are investigated varying both…

混沌动力学 · 物理学 2017-01-25 Rosario González-Férez , Manuel Iñarrea , J. Pablo Salas , Peter Schmelcher

A general rate theory for resonance energy transfer is formulated to incorporate any degrees of freedom (e.g., rotation, vibration, exciton, and polariton) as well as coherently-coupled composite states. The compact rate expression allows…

化学物理 · 物理学 2022-01-31 Jianshu Cao

When two solids are separated by a vacuum gap of thickness smaller than the wavelength of acoustic phonons, the latter can tunnel across the gap thanks to van der Waals forces or electrostatic interactions. Here we show that these…

介观与纳米尺度物理 · 物理学 2023-11-27 Mauricio Gómez Viloria , Yangyu Guo , Samy Merabia , Riccardo Messina , Philippe Ben-Abdallah

We investigate the energy transfer dynamics in a donor-acceptor model by developing a time-local master equation technique based on a variational transformation of the underlying Hamiltonian. The variational transformation allows a…

量子物理 · 物理学 2011-09-19 Dara P. S. McCutcheon , Ahsan Nazir

We present analytical expressions and numerical results for the rates of energy exchange between oscillators and with the environment in a heterogeneous ensemble of globally coupled mechanical phase oscillators. The system is in stationary…

适应与自组织系统 · 物理学 2022-01-19 Raúl I. Sosa , Damián H. Zanette

Electronic and vibrational degrees of freedom in atom-cluster collisions are treated simultaneously and self-consistently by combining time-dependent density functional theory with classical molecular dynamics. The gradual change of the…

原子与分子团簇 · 物理学 2009-10-30 U. Saalmann , R. Schmidt

Decoherence for a one-dimensional coupled-resonator waveguide with a two-level system inside one of resonators, induced by their interaction with corresponding environments, is investigated. Each environment is modeled as a continuum of…

量子物理 · 物理学 2015-05-19 Jing Lu , Lan Zhou , H. C. Fu , Le-Man Kuang