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A colloidal particle placed in an inhomogeneous solution of smaller non-adsorbing polymers will move towards regions of lower polymer concentration, in order to reduce the free energy of the interface between the surface of the particle and…

软凝聚态物质 · 物理学 2017-12-13 Richard P. Sear , Patrick B. Warren

We investigate coarse-grained models of suspended self-thermophoretic microswimmers. Upon heating, the Janus spheres, with hemispheres made of different materials, induce a heterogeneous local solvent temperature that causes the…

软凝聚态物质 · 物理学 2021-08-09 Sven Auschra , Dipanjan Chakraborty , Gianmaria Falasco , Richard Pfaller , Klaus Kroy

In this Account, we describe how synthetic motors that operate by self-diffusiophoresis make use of a self-generated concentration gradient to drive motor motion. A description of propulsion by self-diffusiophoresis is presented for Janus…

软凝聚态物质 · 物理学 2015-01-21 Peter H. Colberg , Shang Yik Reigh , Bryan Robertson , Raymond Kapral

Active particles driven by a chemical reaction are the subject of intense research to date due to their rich physics, being intrinsically far from equilibrium, and their multiple technological applications. Recent attention in the field is…

软凝聚态物质 · 物理学 2023-10-02 Dolachai Boniface , Sergi G. Leyva , Ignacio Pagonabarraga , Pietro Tierno

Micron-sized particles moving through solution in response to self-generated chemical gradients serve as model systems for studying active matter. Their far-reaching potential applications will require the particles to sense and respond to…

软凝聚态物质 · 物理学 2016-03-09 W. E. Uspal , M. N. Popescu , S. Dietrich , M. Tasinkevych

Phoretic colloids self-propel thanks to surface flows generated in response to surface gradients (thermal, electrical, or chemical), that are self-induced and/or generated by other particles. Here we present a scalable and versatile…

软凝聚态物质 · 物理学 2024-07-29 Blaise Delmotte , Florencio Balboa Usabiaga

We study numerically and analytically a model of self-propelled polar disks on a substrate in two dimensions. The particles interact via isotropic repulsive forces and are subject to rotational noise, but there is no aligning interaction.…

软凝聚态物质 · 物理学 2014-02-24 Yaouen Fily , M. Cristina Marchetti

This paper investigates the problem of electrophoretic motion of a polyelectrolyte capsule with a porous arbitrary charged conducting shell in an electrolyte under the action of an external electric field. The corresponding boundary value…

流体动力学 · 物理学 2021-08-11 Anatoly N. Filippov , Daria Yu. Khanukaeva , Petr A. Aleksandrov

We study the mobility of a charged colloidal particle in a constant homogeneous electric field by means of computer simulations. The simulation method combines a lattice Boltzmann scheme for the fluid with standard Langevin dynamics for the…

软凝聚态物质 · 物理学 2007-06-20 Vladimir Lobaskin , Burkhard Duenweg , Christian Holm

When a floating body is internally or externally vibrated, its self-generated wavefield can lead to steady propulsion along the interface. In this article, we review several related and recently discovered systems that leverage this…

流体动力学 · 物理学 2025-09-09 Daniel M. Harris , Jack-William Barotta

The thermophoretic motion of a charged spherical colloidal particle and its accompanying cloud of counterions and co-ions in a temperature gradient is studied theoretically. Using the Debye-Huckel approximation, the Soret drift velocity of…

软凝聚态物质 · 物理学 2008-08-05 Seyyed Nader Rasuli , Ramin Golestanian

We suppose that a rigid spherical particle is put into a binary fluid mixture with the critical composition in the homogeneous phase near the demixing critical point. A short-range interaction is assumed between each component and the…

流体动力学 · 物理学 2022-05-26 Youhei Fujitani

Surface bound catalytic chemical reactions self-propel chemically active Janus particles. In the vicinity of boundaries, these particles exhibit rich behavior, such as the occurrence of wall-bound steady states of "sliding". Most active…

Janus phoretic colloids (JPs) self-propel as a result of self-generated chemical gradients and exhibit spontaneous nontrivial dynamics within phoretic suspensions, on length scales much larger than the microscopic swimmer size. Such…

流体动力学 · 物理学 2021-11-29 Tullio Traverso , Sebastien Michelin

Phoretic particles self-propel using self-generated physico-chemical gradients at their surface. Within a suspension, they interact hydrodynamically by setting the fluid around them into motion, and chemically by modifying the chemical…

流体动力学 · 物理学 2019-02-20 Eva Kanso , Sebastien Michelin

A highly-charged spherical colloid in a salt-free environment exerts such a powerful attraction on its counterions that a certain fraction condenses onto the surface of a particle. The degree of condensation depends on the curvature of the…

Colloidal motors without moving parts can be propelled by self-diffusiophoresis, coupling molecular concentration gradients generated by surface chemical reactions to the velocity slip between solid Janus particles and the surrounding fluid…

统计力学 · 物理学 2021-02-08 Pierre Gaspard , Raymond Kapral

We present the diffusiophoresis of ellipsoidal particles induced by ionic solute gradients. Contrary to the common expectation that diffusiophoresis is shape independent, here we show experimentally that this assumption breaks down when the…

软凝聚态物质 · 物理学 2023-05-31 Viet Sang Doan , Dong-Ook Kim , Craig Snoeyink , Ying Sun , Sangwoo Shin

The stochastic dynamics of colloidal particles with surface activity--in the form of catalytic reaction or particle release--and self-phoretic effects is studied analytically. Three different time scales corresponding to inertial effects,…

软凝聚态物质 · 物理学 2015-05-13 Ramin Golestanian

We consider a 2D model of an autophoretic particle in which the particle has a circular shape and emits/absorbs a solute that diffuses and is advected by the suspending fluid. Beyond a certain emission/absorption rate (characterized by a…

软凝聚态物质 · 物理学 2022-11-30 A. Farutin , M. S. Rizvi , W. -F. Hu , T. S. Lin , S. Rafaï , C. Misbah