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The phase separation in lipid bilayers that include negatively charged lipids is examined experimentally. We observed phase-separated structures and determined the membrane miscibility temperatures in several binary and ternary lipid…

软凝聚态物质 · 物理学 2014-10-16 Hiroki Himeno , Naofumi Shimokawa , Shigeyuki Komura , David Andelman , Tsutomu Hamada , Masahiro Takagi

We investigated the phase separation of dioleoylphosphatidylserine (DOPS) and dipalmitoylphosphatidylcholine (DPPC) in giant unilamellar vesicles in hypotonic solution using fluorescence and confocal laser scanning microscopy. Although…

软凝聚态物质 · 物理学 2021-09-02 Jingyu Guo , Hiroaki Ito , Yuji Higuchi , Klemen Bohinc , Naofumi Shimokawa , Masahiro Takagi

Cholesterol (CHOL) is one of the most important components of plasma membranes of higher cells and one of the main factors for the formation of (nano)domains. In this work, molecular dynamics simulations of mixtures of CHOL with DPPC…

生物物理 · 物理学 2022-08-11 Fabian Keller , Andreas Heuer

Many ternary mixtures composed of saturated and unsaturated lipids with cholesterol (Chol) exhibit a region of coexistence between liquid-disordered $(L_d)$ and liquid-ordered $(L_o)$ domains, bearing some similarities to lipid rafts in…

软凝聚态物质 · 物理学 2024-11-26 Subhadip Basu , Oded Farago

Water contained within biological membranes plays a critical role in maintaining the separation between intracellular and extracellular environments and facilitating biochemical processes. Variations in membrane composition and temperature…

We summarize and compare recent Molecular Dynamics simulations on the interactions of dipalmitoylphosphatidylcholine (DPPC) bilayers in the liquid crystalline phase with a number of small molecules including trehalose, a disaccharide of…

We report on atomistic simulations of DPPC lipid monolayers using the CHARMM36 lipid force field and four-point OPC water model. The entire two-phase region where domains of the `liquid-condensed' (LC) phase coexist with domains of the…

软凝聚态物质 · 物理学 2019-03-18 S. Panzuela , D. P. Tieleman , L. Mederos , E. Velasco

We study the effect of cholesterol on the structure of dipalmitoylphosphatidylcholine (DPPC) phospholipid bilayers. Using extensive molecular dynamics computer simulations at atomistic resolution we observe and quantify several structural…

生物物理 · 物理学 2018-12-26 Felix Leeb , Lutz Maibaum

The presence and the properties of lipid bilayer nanometer-scale domains might be important for understanding the membranes of living cells. We used molecular dynamics (MD) simulations to investigate perturbations of a small patch of…

软凝聚态物质 · 物理学 2011-06-01 Frederick A. Heberle , David G. Ackerman , Gerald W. Feigenson

The widespread interest in phase recognition of lipid membranes has led to the use of different optical techniques to enable differentiation of healthy and not fully functional cells. In this work, we show how the combination of different…

The molecular arrangement of lipids and proteins within biomembranes and monolayers gives rise to complex film morphologies as well as regions of distinct electrical surface potential, topographical and electrostatic nanoscale domains. To…

软凝聚态物质 · 物理学 2016-11-28 Elizabeth Drolle , W. F. D. Bennett , K. Hammond , Edward Lyman , Mikko Karttunen , Zoya Leonenko

Monolayer spontaneous curvatures for cholesterol, DOPE, POPE, DOPC, DPPC, DSPC, POPC, SOPC, and egg sphingomyelin were obtained using small-angle X-ray scattering (SAXS) on inverted hexagonal phases (HII). Spontaneous curvatures of bilayer…

软凝聚态物质 · 物理学 2013-10-08 Benjamin Kollmitzer , Peter Heftberger , Michael Rappolt , Georg Pabst

We report a new and facile method for measuring edge tensions of lipid membranes. The approach is based on electroporation of giant unilamellar vesicles and analysis of the pore closure dynamics. We applied this method to evaluate the edge…

生物物理 · 物理学 2011-02-11 Thomas Portet , Rumiana Dimova

The influence of dimethyl sulfoxide (DMSO) on membrane thickness, multilamellar repeat distance, and phase transitions of 1,2-dipalmitoyl-sn-glycero-3-phosphatidylcholine (DPPC) was investigated by X-ray diffraction and small-angle neutron…

生物物理 · 物理学 2007-05-23 M. A. Kiselev , P. Lesieur , A. M. Kisselev , C. Grabielle-Madelmond , M. Ollivon

The molecular dynamics in the ambient-pressure solid phase of (1,1,2)-trichloroethane is studied by means of broadband dielectric spectroscopy and molecular dynamics simulations. The dielectric spectra of polycrystalline samples obtained by…

The low sliding friction of articular cartilage in the major joints , which is crucial for its homeostasis and for joint health, has been attributed to lipid bilayers forming lubricious boundary layers at its surface. The robustness of such…

软凝聚态物质 · 物理学 2023-09-06 Salome Mielke , Raya Sorkin , Jacob Klein

By means of atomistic molecular dynamics simulations, we study cholesterol-DPPC (dipalmitoyl phosphatidylcholine) bilayers of different composition, from pure DPPC bilayers to a 1:1 mixture of DPPC and cholesterol. The lateral-pressure…

软凝聚态物质 · 物理学 2007-05-23 Michael Patra

Hypothesis. Isoniazid is one of the primary drugs used in tuberculosis treatment. Isoniazid encapsulation in liposomal vesicles can improve drug therapeutic index and minimize toxic and side effects. In this work, we consider mixtures of…

A molecular model is proposed of a bilayer consisting of fully saturated DPPC and mono unsaturated DOPC. The model not only encompasses the constant density within the hydrophobic core of the bilayer, but also the tendency of chain segments…

生物物理 · 物理学 2009-11-10 R. Elliott , K. Katsov , M. Schick , I. Szleifer

Salt, glycerol and dimethyl sulfoxide (DMSO) are used to modify the properties of protein solutions. We experimentally determined the effect of these additives on the phase behavior of lysozyme solutions. Upon the addition of glycerol and…

软凝聚态物质 · 物理学 2012-03-27 Christoph Gögelein , Dana Wagner , Frédéric Cardinaux , Gerhard Nägele , Stefan U. Egelhaaf
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