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An important goal in molecular physics and chemistry today is to obtain structure-dependent information about molecular function to obtain a deeper understanding into chemical reactions. However, until now, asymmetric tops, which comprise…

We theoretically investigate correlated electron dynamics in high-harmonic generation (HHG), using all-electron \emph{ab initio} simulations for three-dimensional real alkali-metal atoms. The resulting harmonic spectra exhibit a plateau…

原子物理 · 物理学 2019-04-10 Yang Li , Takeshi Sato , Kenichi L. Ishikawa

Electromagnetic (EM) waves with helical wavefront carry orbital angular momentum (OAM), which is associated with the azimuthal phase of the complex electric field. OAM is a new degree of freedom in EM waves and is promising for channel…

经典物理 · 物理学 2016-11-10 Menglin L. N. Chen , Li Jun Jiang , Wei E. I. Sha

We explore the possibility of forming a oriented polar molecule directly from a pair of colliding atoms. The process comprises the photoassociation and vibrational stabilization along with the molecular orientation. These processes are…

量子物理 · 物理学 2026-01-14 Murilo D. Forlevesi , Edson Denis Leonel , Emanuel F. de Lima

We present a new magnetic field generation mechanism in underdense plasmas driven by the beating of two, co-propagating, Laguerre-Gaussian (LG) orbital angular momentum (OAM) laser pulses with different frequencies and also different twist…

等离子体物理 · 物理学 2018-10-10 Y. Shi , J. Vieira , R. M. G. M. Trines , R. Bingham , B. F. Shen , R. J. Kingham

X-ray beams carrying orbital angular momentum (OAM), are emerging as a powerful tool to probe matter. Recently, a method called self-seeded FEL with OAM (SSOAM) has been proposed to generate high-power x-ray OAM pulses, which places the…

加速器物理 · 物理学 2025-06-10 Chenzhi Xu , Jiawei Yan , Gianluca Geloni , Christoph Lechner , Haixiao Deng

The ability to perform attosecond-pump attosecond-probe spectroscopy (APAPS) is a longstanding goal in ultrafast science. While first pioneering experiments demonstrated the feasibility of APAPS, the low repetition rates (10-120 Hz) and the…

On the basis of real-time ab initio calculations, we study the non-perturbative interaction of two-color laser pulses with MgO crystal in the strong field regime to generate isolated attosecond pulse from high-harmonic emissions from MgO…

光学 · 物理学 2021-01-13 Zahra Nourbakhsh , Nicolas Tancogne-Dejean , Hamed Merdji , Angel Rubio

High harmonic generation (HHG) with longitudinal optical orbital angular momentum has attracted much attention over the past decade. Here, we present the first study on the HHG with transverse orbital angular momentum driven by the…

光学 · 物理学 2023-08-11 Yiqi Fang , Shengyue Lu , Yunquan Liu

Harmonic generation in atoms and molecules has reshaped our understanding of ultrafast phenomena beyond the traditional nonlinear optics and has launched attosecond physics. Harmonics from solids represent a new frontier, where both…

材料科学 · 物理学 2021-09-01 G. P. Zhang , Y. H. Bai

Recent measurements on high-order harmonic generation (HHG) from N$_2$ aligned perpendicular to the driving laser polarization [B. K. McFarland {\it el al}, Science {\bf 322}, 1232 (2008)] have shown a maximum at the rotational…

原子物理 · 物理学 2009-10-30 Anh-Thu Le , R. R. Lucchese , C. D. Lin

The generation of attosecond X-ray pulses has garnered significant attention within the X-ray free-electron laser (FEL) community due to their potential for ultrafast time-resolved studies. Such pulses enable the investigation of electron…

加速器物理 · 物理学 2025-12-01 Tu Lingjun , Sun Hao , Yi Huaiqian , Zeng Li , Liang Yifan , Yu Yong , Wang Xiaofan , Zhang Weiqing

Sub-10-attosecond pulses with half-cycle electric fields provide exceptional options to detect and manipulate electrons in the atomic timescale. However, the availability of such pulses is still challenging. Here, we propose a method to…

等离子体物理 · 物理学 2021-05-26 Yinren Shou , Ronghao Hu , Zheng Gong , Jinqing Yu , Jia erh Chen , Gerard Mourou , Xueqing Yan , Wenjun Ma

The interaction between relativistic electron beams and intense laser fields has been extensively studied for generating high-energy radiation. However, achieving coherent radiation from such interactions needs to precisely control the…

等离子体物理 · 物理学 2025-09-01 H. Peng , T. W. Huang , C. N. Wu , K. Jiang , R. Li , C. Riconda , S. Weber , C. T. Zhou

High-order harmonic generation (HHG) in aligned linear molecules can offer valuable information about strong-field interactions in lower-lying molecular orbitals, but extracting this information is difficult for three-dimensional molecular…

We examine how the generation and propagation of high-order harmonics in a partly ionized gas medium affect their strength and synchronization. The temporal properties of the resulting attosecond pulses generated in long gas targets can be…

光学 · 物理学 2009-11-13 T. Ruchon , C. P. Hauri , K. Varju , E. Gustafsson , R. Lopez-Martens , A. L'Huillier

Doppler harmonic generation of a high-power laser on a relativistic plasma mirror is a promising path to produce bright attosecond light bursts. Yet, a major challenge has been to find a way to generate isolated attosecond pulses, better…

等离子体物理 · 物理学 2020-10-07 H. Kallala , F. Quéré , H. Vincenti

Optical chirality (OC) - one of the fundamental quantities of electromagnetic fields - corresponds to the instantaneous chirality of light. It has been utilized for exploring chiral light-matter interactions in linear optics, but has not…

光学 · 物理学 2018-04-04 Ofer Neufeld , Oren Cohen

We study numerically the interaction between an intense circularly polarized laser field and an electron moving in a potential which has a discrete cylindrical symmetry with respect to the laser pulse propagation direction. This setup…

原子物理 · 物理学 2009-11-07 F. Ceccherini , D. Bauer