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We report on the magnetoelectric dynamics in the linear magnetoelectric antiferromagnet TbPO$_4$ studied by broadband dielectric spectroscopy. For the phase transition into the magnetoelectric antiferromagnetic phase at $T_{N} \approx 2.3$…

强关联电子 · 物理学 2024-11-05 Christoph P. Grams , Markus Grüninger , Joachim Hemberger

By using broadband linear and nonlinear dielectric spectroscopy we studied the magnetoelectric dynamics in the chiral antiferromagnet MnWO4. In the multiferroic phase the dielectric response is dominated by the dynamics of domains and…

强关联电子 · 物理学 2014-04-25 D. Niermann , C. P. Grams , M. Schalenbach , P. Becker , L. Bohaty , J. Stein , M. Braden , J. Hemberger

The behavior of the low-frequency electromagnon in multiferroic DyMnO3 has been investigated in external magnetic fields and in a magnetically ordered state. Significant softening of the electromagnon frequency is observed for external…

We report the discovery of a complete suppression of ferroelectricity in $MnWO_4$ by 10 % iron substitution and its restoration in external magnetic fields. The spontaneous polarization in $Mn_{0.9}Fe_{0.1}WO_4$ arises below 12 K in…

强关联电子 · 物理学 2008-03-08 R. P. Chaudhury , B. Lorenz , Y. Q. Wang , Y. Y. Sun , C. W. Chu

The time dependence of switching multiferroic domains in MnWO$_4$ has been studied by time-resolved polarized neutron diffraction. Inverting an external electric field inverts the chiral magnetic component within rise times ranging between…

强关联电子 · 物理学 2015-06-18 M. Baum , J. Leist , Th. Finger , K. Schmalzl , A. Hiess , L. P. Regnault , P. Becker , L. Bohaty , G. Eckold , M. Braden

We report on the microwave, terahertz (THz), infrared and Raman spectroscopic studies of $BiMn_{7}O_{12}$ ceramics, shedding more light into the nature of two structural phase transitions and their possible relation with ferroelectricity in…

Type-II multiferroics, where spin interactions induce a ferroelectric polarization, are interesting for new device functionalities due to large magnetoelectric coupling. We report on a new type of multiferroicity in the quadruple-perovskite…

We have studied the magnetic field dependence of far-infrared active magnetic modes in a single ferroelectric domain \BFO/ crystal at low temperature. The modes soften close to the critical field of 18.8\,T along the [001] (pseudocubic)…

强关联电子 · 物理学 2013-06-26 U. Nagel , Randy S. Fishman , T. Katuwal , H. Engelkamp , D. Talbayev , Hee Taek Yi , S. -W. Cheong , T. Rõõm

We examine the low-energy excitations in the vicinity of the quantum critical point in LiHoF$_4$, a physical realization of the Transverse Field Ising Model, focusing on the long-range fluctuations which soften to zero energy at the…

强关联电子 · 物理学 2024-10-25 P. C. E. Stamp , D. M. Silevitch , M. Libersky , Ryan McKenzie , A. A. Geim , T. F. Rosenbaum

We investigate the magnetization dynamics of $TmFeO_3$ single crystals across the spin-reorientation phase transition using broadband microwave absorption spectroscopy up to 87.5 GHz. Temperature- and magnetic-field-dependent…

The chiral components in the magnetic order in multiferroic MnWO4 have been studied by neutron diffraction using spherical polarization analysis as a function of temperature and of external electric field. We show that sufficiently close to…

强关联电子 · 物理学 2009-07-31 T. Finger , D. Senff , K. Schmalzl , W. Schmidt , L. P. Regnault , P. Becker , L. Bohaty , M. Braden

We report the remarkably robust ferroelectric state in the multiferroic compound Mn$_{1-x}$Zn$_x$WO$_4$. The substitution of the magnetic Mn$^{2+}$ with nonmagnetic Zn$^{2+}$ reduces the magnetic exchange and provides control of the various…

强关联电子 · 物理学 2011-01-12 R. P. Chaudhury , F. Ye , J. A. Fernandez-Baca , B. Lorenz , Y. Q. Wang , Y. Y. Sun , H. A. Mook , C. W. Chu

The spin-wave excitations of the multiferroic $\rm MnWO_4$ have been measured in its low-temperature collinear commensurate phase using high-resolution inelastic neutron scattering. These excitations can be well described by a Heisenberg…

We have studied the impact of the magnetic field on the electromagnon excitations in TbMnO3 crystal. Applying magnetic field along the c axis, we show that the electromagnons transform into pure antiferromagnetic modes, losing their polar…

材料科学 · 物理学 2011-07-06 P. Rovillain , M. Cazayous , Y. Gallais , M-A. Measson , A. Sacuto , H. Sakata , M. Mochizuki

The magnetoelectric coupling, i.e., cross-correlation between electric and magnetic orders, is a very desirable property to combine functionalities of materials for next-generation switchable devices. Multiferroics with spin-driven…

The structural phase transition in hexagonal BaMnO$_3$ occurring at $T_c$=130 K was studied in ceramic samples using electron and X-ray diffraction, second harmonic generation as well as by dielectric and lattice dynamic spectroscopies. The…

Our measured dielectric constant and mechanical response of multiferroic BiFeO3 indicate four phase transitions below room temperature. Features correlate with those reported at 50K (from a peak in the zero-field-cooled magnetic…

材料科学 · 物理学 2008-06-23 S. A. T. Redfern , C. Wang , J. W. Hong , G. Catalan , J. F. Scott

The multiferroic compound CuO exhibits low temperature magnetic properties similar to antiferromagnetic iron oxides, while the electronic properties have much more in common with the high $T_c$ cuprate superconductors. This suggests novel…

强关联电子 · 物理学 2016-11-02 Johan Hellsvik , Johan H. Mentink , José Lorenzana

By an electrical-pump--optical-probe technique we show that the electric-field-induced reversal of the magnetic order parameter in multiferroic MnWO$_4$ occurs on the time scale of milliseconds and maintains a rigid coupling of the…

强关联电子 · 物理学 2012-04-16 T. Hoffmann , P. Thielen , P. Becker , L. Bohaty , M. Fiebig

We have carried out a detailed experimental investigation on CuO using dielectric constant, ac resistance, Raman spectroscopy and X-ray diffraction measurements at high pressures and room temperature. Both dielectric constant and dielectric…

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