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相关论文: Multichannel quantum defect theory for ro-vibratio…

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Multichannel Quantum Defect Theory (MQDT) is shown to be capable of producing quantitatively accurate results for low-energy atom-molecule scattering calculations. With a suitable choice of reference potential and short-range matching…

原子物理 · 物理学 2015-03-19 James F. E. Croft , Alisdair O. G. Wallis , Jeremy M. Hutson , Paul S. Julienne

Multichannel quantum defect theory (MQDT) provides a powerful toolkit for describing and understanding collisions of cold alkali atoms. Various MQDT approximations differ primarily in how they characterize the so-called short-ranged…

原子物理 · 物理学 2023-08-01 Alyson Laskowski , Nirav Mehta

We show that multichannel quantum defect theory (MQDT) can be applied successfully as an efficient computational method for cold molecular collisions in Li+NH, which has a deep and strongly anisotropic interaction potential. In this…

化学物理 · 物理学 2013-05-10 James F. E. Croft , Jeremy M. Hutson

Multichannel quantum defect theory (MQDT) can provide an efficient alternative to full coupled-channel calculations for low-energy molecular collisions. However, the efficiency relies on interpolation of the Y matrix that encapsulates the…

化学物理 · 物理学 2013-05-10 James F. E. Croft , Jeremy M. Hutson , Paul S. Julienne

We present a formalism for cold and ultracold atom-diatom chemical reactions that combines a quantum close-coupling method at short-range with quantum defect theory at long-range. The method yields full state-to-state rovibrationally…

原子物理 · 物理学 2015-06-23 Jisha Hazra , Brandon P. Ruzic , John L. Bohn , N. Balakrishnan

We extend Multichannel Quantum Defect Theory (MQDT) to ultracold collisions involving high partial wave quantum numbers $L$. This requires a careful standardization of the MQDT reference wave functions at long range to ensure their linear…

原子物理 · 物理学 2015-06-12 Brandon P. Ruzic , Chris H. Greene , John L. Bohn

We present a general formulation of multichannel quantum-defect theory (MQDT) for anisotropic long-range potentials. The theory unifies the treatment of atomic and molecular interactions of all types, and greatly expands the set of…

原子物理 · 物理学 2020-08-19 Bo Gao

We present a multichannel quantum-defect theory for slow atomic collisions that takes advantages of the analytic solutions for the long-range potential, and both the energy and the angular-momentum insensitivities of the short-range…

原子物理 · 物理学 2009-11-11 Bo Gao , Eite Tiesinga , Carl J. Williams , Paul S. Julienne

We developed a general theoretical approach and a user-ready computer code that permit to study the dynamics of collisional energy transfer and ro-vibrational energy exchange in complex molecule-molecule collisions. The method is a mixture…

化学物理 · 物理学 2024-02-06 Carolin Joy , Bikramaditya Mandal , Dulat Bostan , Marie-Lise Dubernet , Dmitri Babikov

We extend the powerful formalism of multichannel quantum defect theory combined with a frame transformation to ultracold atom-molecule collisions in magnetic fields. By solving the coupled-channel equations with hyperfine and Zeeman…

化学物理 · 物理学 2024-09-10 Masato Morita , Paul Brumer , Timur V. Tscherbul

As a physically motivated and computationally simple model for cold atomic and molecular collisions, the multichannel quantum defect theory (MQDT) with frame transformation (FT) formalism provides an analytical treatment of scattering…

We develop an analytical model for ultracold atom-ion collisions using the multichannel quantum-defect formalism. The model is based on the analytical solutions of the r^-4 long-range potential and on the application of a frame…

原子物理 · 物理学 2015-05-28 Zbigniew Idziaszek , Andrea Simoni , Tommaso Calarco , Paul S. Julienne

Ultracold collisions of cold atoms or molecules make the bound states of the collision complex formed from the two colliding species accessible for control and manipulation of the cold species or the complex. Such resonances are best…

原子物理 · 物理学 2015-05-13 Paul S. Julienne

Mixed quantum/classical theory (MQCT) for the treatment of rotationally inelastic transitions during collisions of two identical molecules, described either as indistinguishable or distinguishable partners, is reviewed. The treatment of two…

化学物理 · 物理学 2025-11-21 Dulat Bostan , Bikramaditya Mandal , Dmitri Babikov

We present a quantum-defect theory (QDT) for the $-1/r^4$ type of long-range potential, as a foundation for a systematic understanding of charge-neutral quantum systems such as ion-atom, ion-molecule, electron-atom, and positron-atom…

原子物理 · 物理学 2014-02-18 Bo Gao

We present a quantum theory of ion-atom interaction that is applicable at energies comparable to or smaller than the atomic hyperfine splitting and takes proper account of the effects of identical nuclei. The theory reveals the subtlety and…

原子物理 · 物理学 2015-06-18 Ming Li , Li You , Bo Gao

The multichannel quantum defect theory (MQDT) can be reinterpreted as a quantum Poincare map in representation of angular momentum. This has two important implications: we have a paradigm of a true quantum Poincare map without…

chao-dyn · 物理学 2016-08-31 F. Leyvraz , R. A. Mendez-Sanchez , M. Lombardi , T. H. Seligman

We propose a hybrid quantum-classical algorithm for solving the time-independent Schr\"odinger equation for atomic and molecular collisions. The algorithm is based on the $S$-matrix version of the Kohn variational principle, which computes…

量子物理 · 物理学 2023-04-14 Xiaodong Xing , Alejandro Gomez Cadavid , Artur F. Izmaylov , Timur V. Tscherbul

We apply quantum defect theory to study low energy ground state atomic collisions including aligned dipole interactions such as those induced by an electric field. Our results show that coupled even ($l$) relative orbital angular momentum…

量子物理 · 物理学 2009-11-07 B. Deb , L. You

We show that quantum interference-based coherent control is a highly efficient tool for tuning ultracold molecular collision dynamics, and is free from the limitations of commonly used methods that rely on external electromagnetic fields.…

原子物理 · 物理学 2021-04-21 Adrien Devolder , Paul Brumer , Timur V. Tscherbul
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