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We measure nonlinear optical scattering from individual Au nanorods excited by ultrafast laser pulses on resonance with their longitudinal plasmon mode. Isolating single rods removes inhomogeneous broadening and allows the measurement of a…

Gold nanorod has generated great research interest due to its tunable longitudinal plasmon resonance. However, little progress has been made in the understanding of the effect. A major reason is that, except for metallic spheres and…

光学 · 物理学 2009-04-03 Cheng-ping Huang , Xiao-gang Yin , Huang Huang , Yong-yuan Zhu

Color centers in solids are the fundamental constituents of a plethora of applications such as lasers, light emitting diodes and sensors, as well as the foundation of advanced quantum information and communication technologies. Their…

Plasmonic dark modes are pure near-field resonances since their dipole moments are vanishing in far field. These modes are particularly interesting to enhance nonlinear light-matter interaction at the nanometer scale because radiative…

The two-photon luminescence (TPL) of gold nanoparticles (NP) was shown to result from the excitation of hot carriers, the plasmonic NP resonances playing an important role both for plasmon enhanced absorption and plasmon enhanced emission.…

介观与纳米尺度物理 · 物理学 2019-08-05 Céline Molinaro , Sylvie Marguet , Ludovic Douillard , Fabrice Charra , Céline Fiorini-Debuisschert

Confining light in extreme subwavelength scales is a tantalizing task. In this work, we report a study of individual plasmonic film-coupled nanostar resonators where plasmonic optical modes are trapped in ultrasmall volumes. Individual gold…

We demonstrate that the fluorescent emitters can increase light emission from the plasmonic nanostructures in turn. With the help of atomic force microscopy, a hybrid system consisting of a fluorescent nanodiamond and a gold nanoparticle…

Noble metal nanoparticles have been utilized for a vast amount of optical applications. For the applications that used metal nanoparticles as nanosensors and optical labeling, larger radiation damping is preferred (higher optical signal).…

光学 · 物理学 2022-03-02 Yanhe Yang , Weihai Ni , Hao Xie , Jian You , Weixiang Ye

Highly nonlinear optical processes, such as multiphoton photoemission, require high intensities, typically achieved with ultrashort laser pulses and, hence, were first observed with the advent of picosecond laser technology. An alternative…

Plasmonic nanoparticles influence the absorption and emission processes of nearby emitters due to local enhancements of the illuminating radiation and the photonic density of states. Here, we use the plasmon resonance of metal nanoparticles…

We demonstrate a bright and polarized fiber in-line single photon source based on plasmon-enhanced emission of colloidal single quantum dots into an optical nanofiber. We show that emission properties of single quantum dots can be strongly…

量子物理 · 物理学 2022-06-28 K. Muhammed Shafi , Ramachandrarao Yalla , Kali P. Nayak

The combination of single photon emitters (quantum dots) and tailored metal nanoparticles with defined size and shape allows a detailed study of the interaction between light and matter. The enhanced optical near-field of the nanoparticles…

介观与纳米尺度物理 · 物理学 2017-04-21 Gernot Schaffernak , Christian Gruber , Joachim R. Krenn , Markus Krug , Marija Gašparić , Martin Belitsch , Andreas Hohenau

Noble metal nanoparticles show specific optical properties due to the excitation of localized surface plasmons that make them attractive candidates for highly sensitive bionanosensors. The underlying physical principle is either an…

Anti-Stokes photoluminescence of metal nanoparticles, in which emitted photons have a higher energy than the incident photons, is an indicator of the temperature prevalent within a nanoparticle. Previous work has shown how to extract the…

光学 · 物理学 2020-08-21 Thomas Jollans , Martín Caldarola , Yonatan Sivan , Michel Orrit

Particle plasmons in metal nanoparticles have primarily been investigated through the use of local optical response approximations. However, as nanoparticle size approaches the average distance of electrons to the metal surface, mesoscopic…

光学 · 物理学 2023-06-28 Weixiang Ye

Understanding light-matter interaction at the nanoscale requires probing the optical properties of matter at the individual nano-absorber level. To this end, we have developed a nanomechanical photothermal sensing platform that can be used…

光学 · 物理学 2024-06-07 Kostas Kanellopulos , Robert G. West , Silvan Schmid

The two-photon luminescence (TPL) of small 10 nm x 40 nm colloidal gold nanorods (GNR) is investigated at the single object level, combining polarization resolved TPL and simultaneously acquired topography. A very high dependence of the TPL…

Optical antennas link objects to light. Here, we analyze metal nanorod antennas as cavities with variable reflection coefficients to derive the interaction of dipolar transitions with radiation through the antenna modes. The presented…

光学 · 物理学 2011-07-27 Tim H. Taminiau , Fernando D. Stefani , Niek F. van Hulst

We demonstrate the direct photothermal probing and mapping of single plasmonic nanostructures via the temperature induced detuning of nanomechanical string resonators. Single Au nanoslits are illuminated with a low-power polarized focused…

介观与纳米尺度物理 · 物理学 2014-04-25 Silvan Schmid , Kaiyu Wu , Peter Emil Larsen , Tomas Rindzevicius , Anja Boisen

We present the first experimental study of optical response of collective plasmon resonances in regular arrays of nanoresonators to local environment. Recently observed collective plasmon modes arise due to diffractive coupling of localised…

介观与纳米尺度物理 · 物理学 2015-05-18 V. G. Kravets , F. Schedin , A. V. Kabashin , A. N. Grigorenko
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