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Magneto-transport properties in hybrid magnetic tunnel junctions (MTJs) integrating self-assembled monolayers (SAMs) as tunnel barriers are critically influenced by spinterface effects, which arise from the electronic properties at…

We have investigated the conductance properties of C60-containing self-assembled monolayers (SAMs), which are used in organic field-effect transistors, employing a combination of molecular-dynamics simulations, semiempirical electronic…

介观与纳米尺度物理 · 物理学 2015-06-19 Susanne Leitherer , Christof Jäger , Marcus Halik , Timothy Clark , Michael Thoss

We present a theoretical analysis aimed at understanding electrical conduction in molecular tunnel junctions. We focus on discussing the validity of coherent versus incoherent theoretical formulations for single-level tunneling to explain…

介观与纳米尺度物理 · 物理学 2016-06-06 Alvar R. Garrigues , Li Yuan , Lejia Wang , Eduardo R. Mucciolo , Damien Thompson , Enrique del Barco , Christian A. Nijhuis

We have fabricated a variety of novel molecular tunnel junctions based on self-assembled-monolayers (SAM) of two-component solid-state mixtures of molecular wires (1,4 methane benzene-dithiol; Me-BDT with two thiol anchoring groups), and…

材料科学 · 物理学 2009-11-11 Vladimir Burtman , Alexander S. Ndobe , Valy Z. Vardeny

Understanding electron transport processes in molecular wires connected between contacts is a central focus in the field of molecular electronics. Especially, the dephasing effect causing tunneling-to-hopping transition has great importance…

介观与纳米尺度物理 · 物理学 2012-06-26 Daijiro Nozaki , Claudia Gomes da Rocha , Horacio M. Pastawski , Gianaurelio Cuniberti

In weakly interacting organic semiconductors, static and dynamic disorder often have an important impact on transport properties. Describing charge transport in these systems requires an approach that correctly takes structural and…

The conductance of single molecule junctions is calculated using a Landauer approach combined to many-body perturbation theory MBPT) to account for electron correlation. The mere correction of the density-functional theory eigenvalues,…

介观与纳米尺度物理 · 物理学 2015-05-27 T. Rangel , A. Ferretti , P. E. Trevisanutto , V. Olevano , G. -M. Rignanese

The transport through a quantum-scale device may be characterized by the transmission eigenvalues. These values constitute a junction PIN code where, for example, in single-atom metallic contacts the number of transmission channels is also…

介观与纳米尺度物理 · 物理学 2011-08-01 Justin P. Bergfield , Joshua D. Barr , Charles A. Stafford

The study of the effects of scaling on magnetic tunnel junction (MTJ) devices has become an important topic in the field of spin-based memory devices. Here, we investigate the effect of elastic dephasing on trilayer and pentalayer MTJ…

介观与纳米尺度物理 · 物理学 2018-09-18 Debasis Das , Ashwin Tulapurkar , Bhaskaran Muralidharan

The characteristics of molecular electronic devices are critically determined by metal-organic interfaces, which influence the arrangement of the orbital levels that participate in charge transport. Studies on self-assembled monolayers…

In transport calculations for molecular junctions based on density functional theory the choice of exchange and correlation functional may dramatically affect the results. In particular local and semi-local functionals tend to…

介观与纳米尺度物理 · 物理学 2009-11-13 C. Toher , S. Sanvito

The effect of dephasing on electron transport through a benzene molecule is carefully examined using a phenomenological model introduced by B\"{u}ttiker. Within a tight-binding framework all the calculations are performed based on the…

介观与纳米尺度物理 · 物理学 2011-04-14 Moumita Dey , Santanu K. Maiti , S. N. karmakar

This thesis investigates the mechanically controlled break junctions, with a particular emphasis on elucidating the behaviour of molecular currents at room temperature. The core of this experimental investigation involves a detailed…

介观与纳米尺度物理 · 物理学 2024-09-17 Giovanna Angelis Schmidt

Molecular self-assembly has been extensively used for surface modification of metals and oxides for a variety of applications, including molecular and organic electronics. One of the goals of this research is to learn how the electronic…

材料科学 · 物理学 2009-11-13 M. F. Calhoun , J. Sanchez , D. Olaya , M. E. Gershenson , V. Podzorov*

We consider electronic transport through a single-molecule junction where the molecule has a degenerate spectrum. Unlike previous transport models, and theories a rate-equations description is no longer possible, and the quantum coherences…

介观与纳米尺度物理 · 物理学 2013-05-29 Maximilian G. Schultz

In a current-carrying single-molecular junction (SMJ), a hierarchy of hybrid energy transport processes takes place under a highly nonequilibrium situation, including energy transfer from electrons to molecular vibrations via…

介观与纳米尺度物理 · 物理学 2022-11-02 Gen Li , Bing-Zhong Hu , Wen-Hao Mao , Nuo Yang , Jing-Tao Lü

Electronic transport properties for single-molecule junctions have been widely measured by several techniques, including mechanically controllable break junctions, electromigration break junctions or by means of scanning tunneling…

介观与纳米尺度物理 · 物理学 2020-07-22 Ferdinand Evers , Richard Korytár , Sumit Tewari , Jan M. van Ruitenbeek

Novel organic materials formed from functional molecules are attractive for various nanoelectronic applications because they are environmentally friendly, widely available and inexpensive. Recent advancement in bottom-up fabrication methods…

介观与纳米尺度物理 · 物理学 2022-12-14 Abdalghani Daaoub , Renhang Wang , Ross Davidson , Sara Sangtarash , Hatef Sadeghi

We investigate the interplay of quantum interference effects and electronic-vibrational coupling in electron transport through single-molecule junctions, employing a nonequilibrium Green's function approach. Our findings show that inelastic…

介观与纳米尺度物理 · 物理学 2013-02-18 R. Härtle , M. Butzin , M. Thoss

Non-equilibrium Green's functions (NEGF) formalism combined with extended Huckel (EHT) and charging model are used to study electrical conduction through single-molecule junctions. Analyzed molecular complex is composed of asymmetric…

介观与纳米尺度物理 · 物理学 2009-11-11 Kamil Walczak , Sergey Edward Lyshevski
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