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Chemically active Janus particles generate tangential concentration gradients along their surface for self-propulsion. Although this is well studied in unbounded domains, the analysis in biologically relevant environments such as…

软凝聚态物质 · 物理学 2021-11-29 Akash Choudhary , K. V. S. Chaithanya , Sébastien Michelin , S. Pushpavanam

Surface bound catalytic chemical reactions self-propel chemically active Janus particles. In the vicinity of boundaries, these particles exhibit rich behavior, such as the occurrence of wall-bound steady states of "sliding". Most active…

Catalytically active Janus particles suspended in solution create gradients in the chemical composition of the solution along their surfaces, as well as along any nearby container walls. The former leads to self-phoresis, while the latter…

软凝聚态物质 · 物理学 2016-09-22 W. E. Uspal , M. N. Popescu , S. Dietrich , M. Tasinkevych

Janus particles self-propel by generating local tangential concentration gradients along their surface. These gradients are present in a thin layer whose thickness is small compared to the particle size. Chemical asymmetry along the surface…

软凝聚态物质 · 物理学 2021-03-31 Prathmesh M. Vinze , Akash Choudhary , S. Pushpavanam

Many biological microswimmers are capable of chemotaxis, i.e., they can sense an ambient chemical gradient and adjust their mechanism of motility to move towards or away from the source of the gradient. Synthetic active colloids endowed…

软凝聚态物质 · 物理学 2024-06-18 Viviana Mancuso , Mihail N. Popescu , William E. Uspal

Self-phoretic Janus particles move by inducing -- via non-equilibrium chemical reactions occurring on their surfaces -- changes in the chemical composition of the solution in which they are immersed. This process leads to gradients in…

软凝聚态物质 · 物理学 2018-01-30 W. E. Uspal , M. N. Popescu , M. Tasinkevych , S. Dietrich

We study the effect of a nearby planar wall on the propulsion of a phoretic Janus micro-swimmer driven by asymmetric reactions on its surface which absorb reactants and generate products. We show that the behaviour of these swimmers near a…

软凝聚态物质 · 物理学 2017-06-01 Yahaya Ibrahim , Tanniemola B. Liverpool

The dynamics of self-propelled colloidal particles are strongly influenced by their environment through hydrodynamic and, in many cases, chemical interactions. We develop a theoretical framework to describe the motion of confined active…

流体动力学 · 物理学 2025-08-29 Günther Turk , Rajesh Singh , Howard A. Stone

Active particles affect their environment as much as the environment affects their active motion. Here, we present an experimental system where both can be simultaneously adjusted in situ using an external AC electric field. The environment…

We study the self-diffusiophoresis of a spherical chemically active particle near a planar, impermeable wall, with a focus on the influence of particle orientation on propulsion. We analyze a Janus particle with asymmetric surface chemical…

软凝聚态物质 · 物理学 2026-03-03 Tachin Ruangkriengsin , Günther Turk , Howard A. Stone

An important challenge in active matter lies in harnessing useful global work from entities that produce work locally, e.g., via self-propulsion. We investigate here the active matter version of a classical capillary rise effect, by…

We study the dynamics of active Janus particles that self-propel in solution by light-activated catalytic decomposition of chemical "fuel." We develop an analytical model of a photo-active self-phoretic particle that accounts for…

软凝聚态物质 · 物理学 2019-05-23 W. E. Uspal

A longstanding goal in colloidal active matter is to understand how gradients in fuel concentration influence the motion of phoretic Janus particles. Here, we present a theoretical description of the motion of a spherical phoretic Janus…

软凝聚态物质 · 物理学 2025-05-28 Parvin Bayati , Stewart A. Mallory

We investigate the structure formation of amphiphilic molecules at planar walls using density functional theory. The molecules are modeled as (hard) spheres composed of a hydrophilic and hydrophobic part. The orientation of the resulting…

软凝聚态物质 · 物理学 2015-05-20 Gerald Rosenthal , Sabine H. L. Klapp

Chemically active colloids move by creating gradients in the composition of the surrounding solution and by exploiting the differences in their interactions with the various molecular species in solution. If such particles move near…

软凝聚态物质 · 物理学 2017-02-24 M. N. Popescu , W. E. Uspal , S. Dietrich

Active matter classifies systems consisting of self-propelled units which convert the energy stored locally or extracted from their environment into directed motion. It has recently attracted considerable attention due to rich new physics…

等离子体物理 · 物理学 2026-04-09 Volodymyr Nosenko

We study a simple model for a particle that is active due to self-phoresis and that has been proposed to model symmetric camphor grains. The particle generates a concentration field through the continuous emission of a chemical substance,…

统计力学 · 物理学 2026-02-18 Leah Anderson , David S. Dean

For natural microswimmers, the interplay of swimming activity and external flow can promote robust motion, e.g. propulsion against ("upstream rheotaxis") or perpendicular to the direction of flow. These effects are generally attributed to…

软凝聚态物质 · 物理学 2018-01-30 Jaideep Katuri , William E. Uspal , Juliane Simmchen , Albert Miguel-López , Samuel Sánchez

Catalytic microswimmers typically swim close to walls due to hydrodynamic and/or phoretic effects. The walls in turn are known to affect their propulsion, making it difficult to single out the contributions that stem from particle-based…

We experimentally investigate active motion of spherical Janus colloidal particles in a viscoelastic fluid. Self-propulsion is achieved by a local concentration gradient of a critical polymer mixture which is imposed by laser illumination.…

软凝聚态物质 · 物理学 2016-03-31 Juan Ruben Gomez-Solano , Alex Blokhuis , Clemens Bechinger
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