相关论文: Giant Rydberg Excitons in Cuprous Oxide
Rydberg states of excitons can reach microns in size and require extremely pure crystals. We introduce an experimental method for the rapid and spatially-resolved characterization of Rydberg excitons in copper oxide (Cu2O) with sub-micron…
We demonstrate that through localised Rydberg excitation in a three-dimensional cold atom cloud atomic motion can be rendered directed and nearly confined to a plane, without spatial constraints for the motion of individual atoms. This…
We analyze theoretically the Coulomb scattering processes of highly excited excitons in the direct bandgap semiconductor quantum wells. We find that contrary to the interaction of ground state excitons the electron and hole exchange…
Rydberg excitons in $\mathrm{Cu_2O}$ simultaneously give rise to two very different optical responses under resonant two-photon excitation: a coherent second-harmonic signal mediated by the excitonic second order susceptibility tensor…
We demonstrate that the optical linewidth of Rydberg excitons in Cu2O can be completely explained by scattering with acoustical and optical phonons, whereby the dominant contributions stems from the non-polar optical modes. The consequences…
Rydberg excitons, the solid-state counterparts of Rydberg atoms, have sparked considerable interest in harnessing their quantum application potentials, whereas a major challenge is realizing their spatial confinement and manipulation.…
Excitons, as bound states of electrons and holes, embody the solid state analogue of the hydrogen atom, whose quantum spectrum is explained within a classical framework by the Bohr-Sommerfeld atomic model. In a first hydrogenlike…
We use two-color pump-probe spectroscopy to study Rydberg excitons in Cu$_2$O in the presence of free carriers injected by above-band-gap excitation. Already at plasma densities $\rho_\text{eh}$ below one hundredth electron-hole pair per…
Experimental and theoretical investigations of excitons in cuprous oxide have revealed a significant fine-structure splitting of the excitonic Rydberg states caused by a strong impact of the valence band structure. We provide a…
Rydberg excitons are the solid-state analog of Rydberg atoms and can, e.g., for cuprous oxide, easily reach a large size in the region of $\mu$m for principal quantum numbers up to $n=25$. The fabrication of quantum well-like structures in…
Rydberg states of excitons in Cu$_2$O are known to interact strongly with other carriers in their surrounding such as other excitons, free charge carriers and static charged impurities. In cw-experiments, discriminating the individual…
The observation of giant Rydberg excitons in cuprous oxide $\left(\mathrm{Cu_{2}O}\right)$ up to a principal quantum number of $n=25$ by T.~Kazimierczuk \emph{et al.} [Nature \textbf{514}, 343, (2014)] inevitably raises the question whether…
Rydberg atoms have attracted considerable interest due to their huge interaction among each other and with external fields. They demonstrate characteristic scaling laws in dependence on the principal quantum number $n$ for features such as…
The realization of exciton-polaritons -- hybrid excitations of semiconductor quantum well excitons and cavity photons -- has been of great technological and scientific significance. In particular, the short-range collisional interaction…
The recent observation of high-lying Rydberg states of excitons in semiconductors with relatively high binding energy motivates exploring their applications in quantum nonlinear optics and quantum information processing. Here, we study…
Coherent optical control of individual particles has been demonstrated both for atoms and semiconductor quantum dots. Here we demonstrate the emergence of quantum coherent effects in semiconductor Rydberg excitons in bulk Cu$_2$O. Due to…
Excitons -- bound electron-hole pairs -- play a central role in light-matter interaction phenomena, and are crucial for wide-ranging applications from light harvesting and generation to quantum information processing. A long-standing…
Excitons play a key role in the linear optical response of 2D materials. However, their significance in the highly nonlinear optical response to intense mid-infrared light has often been overlooked. Using hBN as a prototypical example, we…
Recent experiments show that optically generated Rydberg excitons in cuprous oxide can neutralize charged impurities, strongly reducing stray electric fields and effectively purifying the crystal. Here, we develop a multichannel theory of…
Flexible Rydberg aggregates, assemblies of few Rydberg atoms coherently sharing electronic excitations while undergoing directed atomic motion, show great promise as quantum simulation platform for nuclear motional dynamics in molecules or…