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A wide variety of nuclear magnetic resonance experiments rely on the prediction and analysis of relaxation processes. Recently, innovative approaches have been introduced where the sample travels through a broad range of magnetic fields in…

We describe a method for precise estimation of the polarization of a mesoscopic spin ensemble by using its coupling to a single two-level system. Our approach requires a minimal number of measurements on the two-level system for a given…

量子物理 · 物理学 2009-11-11 G. Giedke , J. M. Taylor , D. D'Alessandro , M. D. Lukin , A. Imamoglu

Low thermal polarization of nuclear spins is a primary sensitivity limitation for nuclear magnetic resonance. Here we demonstrate optically pumped (microwave-free) nuclear spin polarization of $^{13}\mathrm{C}$ and $^{15}\mathrm{N}$ in…

介观与纳米尺度物理 · 物理学 2017-08-09 Ben L. Green , Ben G. Breeze , Gregory J. Rees , John V. Hanna , Jyh-Pin Chou , Viktor Ivády , Adam Gali , Mark E. Newton

Experimental investigation of nuclear spin effects on the electron spin polarization in singly negatively charged InP quantum dots is reported. Pump-probe photoluminescence measurements of electron spin relaxation in the microsecond…

介观与纳米尺度物理 · 物理学 2007-05-23 Bipul Pal , Sergey Yu. Verbin , Ivan V. Ignatiev , Michio Ikezawa , Yasuaki Masumoto

In nuclear magnetic resonance (NMR), the bulk magnetization of a sample is commonly assumed to be proportional to spin polarization, with each spin of the same type contributing equally to the measured signal. In this work, we prove the…

化学物理 · 物理学 2025-06-16 Danila A. Barskiy , Andrey Pravdivtsev

Dynamic nuclear polarization (DNP) has revolutionized the field of NMR spectroscopy, expanding its reach and capabilities to investigate diverse materials, biomolecules, and complex dynamic processes. Bringing high-efficiency DNP to the…

介观与纳米尺度物理 · 物理学 2024-02-27 Sahand Tabatabaei , Pritam Priyadarsi , Namanish Singh , Pardis Sahafi , Daniel Tay , Andrew Jordan , Raffi Budakian

Coupled electron-nuclear spins represent a promising quantum system, where the optically induced electron spin polarization can be dynamically transferred to nuclear spins via the hyperfine interaction. Most experiments on dynamic nuclear…

材料科学 · 物理学 2026-01-13 A. N. Anisimov , A. V. Poshakinskiy , G. V. Astakhov

A quasi-classical theoretical description of polarization and relaxation of nuclear spins in a quantum dot with one resident electron is developed for arbitrary mechanisms of electron spin polarization. The dependence of the…

强关联电子 · 物理学 2015-05-13 I. A. Merkulov , G. Alvarez , D. R. Yakovlev , T. C. Schulthess

We demonstrate ionization of a molecule with the bias voltage of a Scanning Tunnelling Microscope (STM) resulting in a coexistence of a neutral and ionic molecules, i.e. radical (paramagnetic) and non-radical (diamagnetic) states. This…

介观与纳米尺度物理 · 物理学 2024-04-02 Yishay Manassen , Michael Averbukh , Zion Hazan , Yahel Tzuriel , Pino Boscolo , Alexsander Shnirman , Baruch Horovitz

Hyperpolarized nanoparticles (NPs) offer high polarization levels with room temperature relaxation times exceeding half an hour. In this work, we demonstrate that the achievable hyperpolarization enhancement and relaxation (decay) time at…

We demonstrate a new method for electrical manipulation of nuclear spins utilizing dynamic nuclear polarization induced by quantum Hall effect breakdown. Nuclear spins are polarized and detected through the hyperfine interaction between a…

介观与纳米尺度物理 · 物理学 2009-04-17 Minoru Kawamura , Hiroyuki Takahashi , Yoshiaki Hashimoto , Shingo Katsumoto , Tomoki Machida

In III-V semiconductors it was shown theoretically that under optical cooling the nuclear spin polaron bound to neutral donors would form below some critical nuclear spin temperature TC [I. A. Merkulov, Phys. Solid State 40, 930 (1998)].…

介观与纳米尺度物理 · 物理学 2017-06-28 Denis Scalbert

Dynamic nuclear polarization (DNP) is a promising strategy for generating a significantly increased non-thermal spin polarization in nuclear magnetic resonance (NMR) applications thereby circumventing the need for strong magnetic fields.…

量子物理 · 物理学 2015-07-15 Alexander Karabanov , Daniel Wisniewski , Igor Lesanovsky , Walter Köckenberger

We study the nuclear spin population in a GaAs quantum well structure and demonstrate its initialization using an all-electrical nuclear magnetic resonance (NMR) device. In our device, nuclear spins are dynamically polarized in a sub-micron…

介观与纳米尺度物理 · 物理学 2007-05-23 T. Ota , G. Yusa , N. Kumada , S. Miyashita , Y. Hirayama

NV-diamonds have attracted keen interest for nanoscale sensing and spin manipulation. In particular, the non-equilibrium electron spin polarization after optical excitation of single NV centers has successfully been transferred to nuclear…

介观与纳米尺度物理 · 物理学 2021-11-24 R. Rizzato , F. Bruckmaier , K. S. Liu , S. J. Glaser , D. B. Bucher

We study the dynamics of optically-induced nuclear spin polarization in a fluorine-doped ZnSe epilayer via time-resolved Kerr rotation. The nuclear polarization in the vicinity of a fluorine donor is induced by interaction with coherently…

介观与纳米尺度物理 · 物理学 2016-02-24 F. Heisterkamp , E. Kirstein , A. Greilich , E. A. Zhukov , T. Kazimierczuk , D. R. Yakovlev , A. Pawlis , M. Bayer

We report achieving enhanced nuclear magnetization in a magnetic resonance force microscope experiment at 0.6 tesla and 4.2 kelvin using the dynamic nuclear polarization (DNP) effect. In our experiments a microwire coplanar waveguide…

The contribution of the polarization associated with the noncollinear parts of spins in the dielectric permeability tensor of multiferroic materials is considered. As the equilibrium state, we consider the systems of parallel spins, so we…

材料科学 · 物理学 2025-05-13 Pavel A. Andreev

Statistical mechanics underlies our understanding of macroscopic quantum systems. It is based on the assumption that out-of-equilibrium systems rapidly approach their equilibrium states, forgetting any information about their microscopic…

We have observed millisecond-long coherent evolution of nuclear spins in a quantum wire at 1.2 K. Local, all-electrical manipulation of nuclear spins is achieved by dynamic nuclear polarization in the breakdown regime of the Integer Quantum…

介观与纳米尺度物理 · 物理学 2009-10-01 A. Corcoles , C. J. B. Ford , M. Pepper , G. A. C. Jones , H. E. Beere , D. A. Ritchie