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Perovskite manganites with small A-site ions, as the first and canonical branch of type-II multiferroics, are ideal systems to exhibit magnetism-induced ferroelectricity. Despite their established magnetoelectric phase diagrams under low…

材料科学 · 物理学 2026-01-15 Ming Yang , Jun Chen , Junfeng Wang , Chao Dong , Chengliang Lu , Gang Xu , Jinguang Cheng , Jianshi Zhou , Shuai Dong

The presence of superlattice reflections and detailed analyses of the powder neutron and x-ray diffraction data reveal that La rich (BF$_{0.50}$-LF$_{0.50}$)$_{0.50}$-(PT)$_{0.50}$ (BF-LF-PT) has ferroelectric rhombohedral crystal structure…

材料科学 · 物理学 2013-11-27 Anupinder Singh , Ratnamala Chatterjee , S. K. Mishra , P. S. R. Krishna , S. L. Chaplot

Antiferroelectrics are promising materials for high energy density capacitors and the search for environmentally-friendly and efficient systems is actively pursued. An elegant strategy to create and design new (anti)ferroic system relies on…

Magnetic properties of a series of (La0.7Sr0.3MnO3/SrRuO3) superlattices, where the SrRuO3 layer thickness is varying, are examined. A room-temperature magnetocaloric effect is obtained owing to the finite size effect which reduces the TC…

材料科学 · 物理学 2011-01-10 Q. Zhang , S. Thota , F. Guillou , P. Padhan , V. Hardy , A. Wahl , W. Prellier

In insulating materials with ordered magnetic spiral phases, ferroelectricity can emerge due to the breaking of inversion symmetry. This property is of both fundamental and practical interest, in particular with a view to exploiting it in…

The experimental observation that vanadate superlattices (LaVO$_3$)$_m$/SrVO$_3$ show ferromagnetism up to room temperature [U.\ L\"uders {\it et al.}, Phys.\ Rev.\ B {\bf 80}, 241102R (2009)] is investigated by means of density functional…

强关联电子 · 物理学 2016-12-13 Cosima Schuster , Ulrike Lueders , Udo Schwingenschloegl , Raymond Fresard

A new type of multiferroicity was experimentally discovered in 2003 in a perovskite manganite TbMnO$_3$ where its ferroelectricity is induced by cycloidally ordered Mn spins. Susequently, such spin-cycloid multiferroic phase was also…

强关联电子 · 物理学 2025-02-14 Masahito Mochizuki

We report the structural and magnetoelectrical properties of La$_{0.7}$Ca$_{0.3}$MnO$_3$/BaTiO$_3$ perovskite superlattices grown on (001)-oriented SrTiO$_3$ by the pulsed laser deposition technique. Magnetic hysteresis loops together with…

材料科学 · 物理学 2009-11-11 M. P. Singh , W. Prellier , Ch. Simon , B. Raveau

We present a unique example of giant magnetoelectric effect in a conventional multiferroic HoMnO3, where polarization is very large (~56 mC/m2) and the ferroelectric transition temperature is higher than the magnetic ordering temperature by…

强关联电子 · 物理学 2015-05-13 N. Hur , I. K. Jeong , M. F. Hundley , S. B. Kim , S. -W. Cheong

Despite the great technological and scientific importance, a well-controlled coupled behavior in magnetoelectric multiferroic materials at room temperature remains challenging. We demonstrate that the self-ordered A2BBO6 (e.g., A = La, B =…

材料科学 · 物理学 2015-05-14 M. P. Singh , K. D. Truong , S. Jandl , P. Fournier

LiNbO3 (LN) is renowned for its exceptional ferroelectric properties, particularly its notable linear electro-optical (EO) effect, which is highly advantageous for various applications such as high-speed communication, optical computation,…

材料科学 · 物理学 2024-08-20 Yalong Yu , Bo Xiong , Siqi Wu , Yekai Ren , Nuo Chen , Qingjiao Mi , Zhaojie Zheng , Kangping Lou , Rui Wang , Tao Chu

First-principles techniques are used to investigate the behavior of BiFeO$_{3}$/LaFeO$_{3}$ perovskite oxide superlattices epitaxially grown on a (001)-SrTiO$_3$ substrate. The calculations show that 1/1 superlattices exhibit a $Pmc2_1$…

材料科学 · 物理学 2015-06-16 Zeila Zanolli , Jacek C. Wojdel , Jorge Iniguez , Philippe Ghosez

In this contribution to the special issue on multiferroics we focus on multiferroicity driven by different forms of charge ordering. We will present the generic mechanisms by which charge ordering can induce ferroelectricity in magnetic…

材料科学 · 物理学 2011-07-22 Jeroen van den Brink , Daniel I. Khomskii

A series of superlattices and trilayers composed of ferromagnetic and ferroelectric or paraelectric layers were grown on (100) SrTiO3 by the pulsed laser deposition technique. Their structural and magneto-electric properties were examined.…

材料科学 · 物理学 2009-11-11 P. Murugavel , M. P. Singh , W. Prellier , B. Mercey , Ch. Simon , B. Raveau

The stability of a high-symmetry $P4mm$ polar phase in seventeen short-period ferroelectric perovskite superlattices with polar discontinuity is studied from first principles within the density-functional theory. It is shown that in most…

材料科学 · 物理学 2021-02-16 Alexander I. Lebedev

Oxide double perovskites wherein octahedra formed by both 3d elements and sp-based heavy elements give rise to unconventional magnetic ordering and correlated quantum phenomena crucial for futuristic applications. Here, by carrying out…

Superlattices composed of ferromagnetic La0.6Sr0.4MnO3 and ferroelectric 0.7Pb(Mg0,33Nb0.66)O3 0.3(PbTiO3) layers were fabricated on (100) LaAlO3 substrates by pulsed laser deposition technique. Ferromagnetic and frequency independent…

材料科学 · 物理学 2007-05-23 Ayan Roy Chaudhuri , R. Ranjith , S. B. Krupanidhi , R. V. K Mangalam , A. Sundaresan

Two-dimensional magnetic materials attract a lot of attention since they potentially exhibit new magnetic properties due to, e.g., strongly enhanced spin fluctuations. However, the suppression of the long-range magnetic order in two…

强关联电子 · 物理学 2024-06-25 Michal Kiaba , Andreas Suter , Zaher Salman , Thomas Prokscha , Binbin Chen , Gertjan Koster , Adam Dubroka

Perovskite oxide heterostructures offer an important path forward for stabilizing and controlling low-dimensional magnetism. One of the guiding design principles for these materials systems is octahedral connectivity. In superlattices…

材料科学 · 物理学 2017-11-08 Charles L. Flint , Arturas Vailionis , Hua Zhou , Hoyoung Jang , Jun-Sik Lee , Yuri Suzuki

Dielectric study on Ca3Mn2O7 features relaxor-like segmented dynamics below the antiferromagnetic ordering. Dipolar relaxations of different origin are spectrally resolved exhibiting distinct H-field alterations. This identifies their…

材料科学 · 物理学 2019-09-10 Pooja Sahlot , Gaurav Sharma , Vasant Sathe , Anand Mohan Awasthi