相关论文: Frequency Comb-Based Remote Sensing of Greenhouse …
Open-path dual-comb spectroscopy provides multi-species atmospheric gas concentration measurements with high precision. Here, we extend open-path dual comb spectroscopy to the mid-infrared 5 {\mu}m atmospheric window, enabling atmospheric…
Dual-frequency comb spectroscopy has emerged as a disruptive technique for measuring wide-spanning spectra with high resolution, yielding a particularly powerful technique for sensitive multi-component gas analysis. We present a…
Satellite-based greenhouse gases (GHG) sensing technologies play a critical role in the study of global carbon emissions and climate change. However, none of the existing satellite-based GHG sensing technologies can achieve the measurement…
We present gapless, high-resolution absorption and dispersion spectra obtained with quantum cascade laser frequency combs covering 55 cm$^{-1}$. Using phase-sensitive dual comb design, the comb lines are gradually swept over 10 GHz,…
A fieldable dual-comb spectrometer is described based on a "bootstrapped" frequency referencing scheme in which short-term optical phase coherence between combs is attained by referencing each to a free-running diode laser, whilst high…
Optical frequency-comb-based-high-resolution spectrometers offer enormous potential for spectroscopic applications. Although various implementations have been demonstrated, the lack of suitable mid-infrared comb sources has impeded…
In a recent study [1], we demonstrated a multi-heterodyne differential absorption lidar (DIAL) for greenhouse gas monitoring utilizing solid targets. The multi-frequency absorption measurement was achieved using electro-optic dual-comb…
Two frequency combs can be used to measure the full complex response of a sample in a configuration which can be alternatively viewed as the equivalent of a dispersive Fourier transform spectrometer, infrared time domain spectrometer, or a…
The broadband, coherent nature of narrow-linewidth fiber frequency combs is exploited to measure the full complex spectrum of a molecular gas through multi-heterodyne spectroscopy. We measure the absorption and phase shift experienced by…
A mid-Infrared frequency comb is produced via an optical parametric oscillator (OPO) pumped by an amplified 100 MHz Yb:fiber mode-locked laser. We use this source to make measurements of the concentration of the atmospherically-relevant…
Identification and quantification of trace gas sources is a major challenge for understanding and regulating air quality and greenhouse gas emissions. Current approaches either provide continuous but localized monitoring, or…
Frequency comb spectroscopy provides broadband access to molecular fingerprints with mode-defined spectral resolution. However, its deployment in non-cooperative gas sensing remains challenging because conventional implementations require…
Historically, there has been a trade-off in spectroscopic measurements between high spectral resolution, broadband coverage, and acquisition time. Optical frequency combs, initially envisioned for precision spectroscopy of the hydrogen atom…
We have demonstrated a new technique that provides massively parallel comb spectroscopy sensitive specifically to ions through the combination of cavity-enhanced direct frequency comb spectroscopy with velocity modulation spectroscopy.…
We present a versatile mid-infrared frequency comb spectroscopy system based on a doubly resonant optical parametric oscillator tunable in the 3-5.4 {\mu}m range and two detection methods, a Fourier transform spectrometer (FTS) and a…
In this paper, we introduce an all-fibered dual-comb spectrometer based on a new design of highly nonlinear fiber to efficiently convert frequency combs from 1.55 micron to 2 micron We show that our spectrometer can be used to measure…
Dual-comb spectroscopy allows for the rapid, multiplexed acquisition of high-resolution spectra without the need for moving parts or low-resolution dispersive optics. This method of broadband spectroscopy is most often accomplished via…
Mid-infrared high-resolution spectroscopy has proven an invaluable tool for the study of the structure and dynamics of molecules in the gas phase. The advent of frequency combs advances the frontiers of precise molecular spectroscopy. Here…
Frequency combs have revolutionized the field of optical spectroscopy, enabling researchers to probe molecular systems with a multitude of accurate and precise optical frequencies. While there have been tremendous strides in direct…
Dual-frequency comb spectroscopy permits broadband precision spectroscopic measurements with short acquisition time. A dramatic improvement of the maximal spectral bandwidth and the minimal measurement time can be expected when the lasers'…