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We study a three-orbital Hubbard model with negative Hund coupling in infinite dimensions, combining dynamical mean-field theory with continuous time quantum Monte Carlo simulations. This model, which is relevant for the description of…

超导电性 · 物理学 2018-12-13 Kosuke Ishigaki , Joji Nasu , Akihisa Koga , Shintaro Hoshino , Philipp Werner

Strong spin-orbit coupling (SOC) effects of heavy $d$-orbital elements have long been neglected in describing the ground states of their compounds thereby overlooking a variety of fascinating and yet unexplored magnetic and electronic…

The electronic states of isostructural single-component molecular conductors [M(tmdt)2] (M= Ni, Au, and Cu) are theoretically studied. By considering fragments of molecular orbitals as basis functions, we construct a multiorbital model…

强关联电子 · 物理学 2013-04-17 Hitoshi Seo , Shoji Ishibashi , Yuichi Otsuka , Hidetoshi Fukuyama , Kiyoyuki Terakura

We present the influence of spin correlation on the metal-insulator transitions (MIT) in two-orbital Hubbard models by the Kotliar-Ruckenstein slave-boson approach. In the asymmetric half-filling situation, the two orbits simultaneously…

强关联电子 · 物理学 2015-03-19 Ya-Min Quan , Liang-Jian Zou , Hai-Qing Lin

Transition-metal heterostructures offer the fascinating possibility of controlling orbital degrees of freedom via strain. Here, we investigate theoretically the degree of orbital polarization that can be induced by epitaxial strain in…

强关联电子 · 物理学 2014-08-14 Oleg E. Peil , Michel Ferrero , Antoine Georges

We investigate the ground-state property and the excitation gap of a one-dimensional spin-orbital model with isotropic spin and anisotropic orbital exchange interactions, which represents the strong-coupling limit of a two-orbital Hubbard…

强关联电子 · 物理学 2009-11-13 Hiroaki Onishi

Correlated oxides, such as BiMnO$_3$ and LaMnO$_3$, show complex interplay of electronic correlations and crystal structure exhibiting multiple first order phase transitions, some without a clear order parameter. The quantitative…

强关联电子 · 物理学 2022-12-12 Gheorghe Lucian Pascut , Kristjan Haule

We solve the Periodic Anderson model in the Mott-Hubbard regime, using Dynamical Mean Field Theory. Upon electron doping of the Mott insulator, a metal-insulator transition occurs which is qualitatively similar to that of the single band…

强关联电子 · 物理学 2009-11-13 G. Sordi , A. Amaricci , M. J. Rozenberg

The combination of strong spin-orbit coupling and Coulomb interactions makes the $5d$ iridates a unique platform for realizing novel correlated electronic states. Here, utilizing infrared spectroscopy, we demonstrate that a robust Mott…

强关联电子 · 物理学 2026-03-06 Kai Wang , Jun Yang , Chaoyang Kang , Weikang Wu , Wenka Zhu , Jianzhou Zhao , Yaomin Dai , Bing Xu

Based on first-principles calculations and symmetry analysis, we propose that a transition metal rutile oxide, in particular $\beta'$-PtO$_2$, can host a three-dimensional topological Dirac semimetal phase. We find that $\beta'$-PtO$_2$…

强关联电子 · 物理学 2019-01-23 Rokyeon Kim , Bohm-Jung Yang , Choong H. Kim

The layered metal phosphorous trisulfide FePS$_3$ is reported to be a Mott insulator at ambient conditions and to undergo structural and insulator-metal phase transitions under pressure. However, the character of the resulting metallic…

强关联电子 · 物理学 2022-02-28 Minsung Kim , Heung-Sik Kim , Kristjan Haule , David Vanderbilt

We consider a lattice model of itinerant electrons coupled to an array of localized classical Heisenberg spins. The nature of the ground state ordered magnetic phases that result from the indirect spin-spin coupling mediated by the…

强关联电子 · 物理学 2017-05-25 Wenjian Hu , Richard T. Scalettar , Rajiv R. P. Singh

Phase transition and critical properties of Ising-like spin-orbital interacting systems in 2-dimensional triangular lattice are investigated. We first show that the ground state of the system is a composite spin-orbital ferro-ordered phase.…

统计力学 · 物理学 2009-11-13 Huai-Bao Tang , Dong-Meng Chen , Xiang-Fei Wei , Liang-Jian Zou

A recently synthesised series of isostructural compounds Ba$_4$NbTM$_3$O$_{12}$ (TM = Mn, Rh and Ir) with transition-metal trimers in a face-sharing geometry makes it possible to examine a tendency to the molecular orbitals (MO) formation…

强关联电子 · 物理学 2021-04-02 Evgenia V. Komleva , Daniel I. Khomskii , Sergey V. Streltsov

Motivated by the unexplored complexity of phases present in the multiorbital Hubbard model, we analyze in this work the behavior of a degenerate two-orbital anisotropic Hubbard model at half filling where both orbitals have equal bandwidths…

强关联电子 · 物理学 2015-05-20 Hunpyo Lee , Yu-Zhong Zhang , Harald O. Jeschke , Roser Valenti

The interplay between spin and orbital degrees of freedom gives rise to a variety of emergent phases in correlated 4d and 5d transition-metal systems. Strong spin-orbit coupling (SOC) significantly alters Jahn-Teller (JT) physics, often…

强关联电子 · 物理学 2025-05-28 A. S. Miñarro , G. Herranz

The effect of disorder on a class of transition metal oxides described by a single orbital Hubbard model at half filling is investigated. The phases are characterized by the nature of the electronic and spin excitations. The frequency and…

强关联电子 · 物理学 2008-07-23 Kohjiro Kobayashi , Byounghak Lee , Nandini Trivedi

The quasi-particle spectra in the metallic rutile and insulating monoclinic phases of VO$_2$ are shown to be dominated by local Coulomb interactions. In the rutile phase the small orbital polarization among V 3d t_2g states leads to weak…

强关联电子 · 物理学 2007-05-23 A. Liebsch , H. Ishida , G. Bihlmayer

Motivated by the experiments on the organic compound $(Per)_{2}[Pt(mnt)_{2}]$, we study the ground state of the one-dimensional Kondo lattice model at quarter filling with the density matrix renormalization group method. We show a coupled…

强关联电子 · 物理学 2020-12-29 Yixuan Huang , D. N. Sheng , C. S. Ting

We show how in multi-band materials, the Hund's coupling plays a crucial role in tuning the degree of electronic correlation. While in half-filled systems it enhances the correlations, in all other cases it pushes the boundary for the Mott…

强关联电子 · 物理学 2011-06-02 Luca de' Medici