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In the present paper, we develop a semiclassical quasi-static model accounting for molecular double ionization in an intense laser pulse. With this model, we achieve insight into the dynamics of two highly-correlated valence electrons under…

原子与分子团簇 · 物理学 2009-11-13 Di-Fa Ye , Jing Chen , Jie Liu

Almost ten years ago, energetic neutral hydrogen atoms were detected after a strong-field double ionization of H$_2$. This process, called 'frustrated tunneling ionization', occurs when an ionized electron is recaptured after being driven…

In strong laser-atom interactions, the Coulomb potential can affect the trajectories of rescattering electron in high-order harmonic generation (HHG). Here, by constructing a semi-analytical Coulomb-included model and comparing it with…

原子物理 · 物理学 2025-12-16 Yigen Peng , Jiayin Che , Ruihua Xu , Shang Wang , Xuejiao Xie , Yanjun Chen

Coulomb dissociation is an especially simple and important reaction mechanism. Since the perturbation due to the electric field of the (target) nucleus is exactly known, firm conclusions can be drawn from such measurements. Electromagnetic…

核理论 · 物理学 2007-05-23 G. Baur , K. Hencken , D. Trautmann , S. Typel

We study ionization dynamics of aligned diatomic molecules N$_2$ in strong elliptical laser fields experimentally and theoretically. The alignment dependence of photoelectron momentum distributions (PMDs) of N$_2$ measured in experiments is…

We investigate the photoelectron angular emission distributions obtained by strong field dissociative ionization of H$_2$ using cold target recoil ion momentum spectroscopy. In case of employing laser light with an ellipticity close to 0.9…

We consider the dynamics of electrons in combined strong laser and Coulomb fields. Under a timescale separation condition, we reduce this dynamics to a guiding-center framework. More precisely, we derive a hierarchy of models for the…

混沌动力学 · 物理学 2018-11-28 Jonathan Dubois , S. Berman , C. Chandre , T. Uzer

Coulomb dissociation is an especially simple and important reaction mechanism. Since the perturbation due to the electric field of the (target) nucleus is exactly known, firm conclusions can be drawn from such measurements. Electromagnetic…

核理论 · 物理学 2011-07-19 Gerhard Baur , Kai Hencken , Dirk Trautmann

The full three-dimensional photoelectron momentum distributions of argon are measured in intense near-circularly polarized laser fields. We observed that the transverse momentum distribution of ejected electrons by 410-nm near-circularly…

原子物理 · 物理学 2020-02-19 Xiang Huang , Qingbin Zhang , Shengliang Xu , Xianglong Fu , Xu Han , Wei Cao , Peixiang Lu

The role of Coulomb focusing in above-threshold ionization in an elliptically polarized mid-infrared strong laser field is investigated within a semiclassical model incorporating tunneling and Coulomb field effects. It is shown that Coulomb…

原子物理 · 物理学 2015-05-30 Chengpu Liu , Karen Z. Hatsagortsyan

We study ionization of atoms in strong elliptically-polarized laser fields. We focus on the physical origin of the offset angle in the photoelectron momentum distribution and its possible relation to a specific time. By developing a model…

原子物理 · 物理学 2022-12-12 Y. G. Peng , J. Y. Che , C. Chen , G. G. Xin , Y. J. Chen

A recent paper reported elliptically polarized high-order harmonics from aligned N$_2$ using a linearly polarized driving field [X. Zhou \emph{et al.}, Phys. Rev. Lett. \textbf{102}, 073902 (2009)]. This observation cannot be explained in…

原子物理 · 物理学 2010-03-29 Adam Etches , Christian Bruun Madsen , Lars Bojer Madsen

The disassembly of molecular clusters $(N_2)_n$ ($n$=50-3000) in strong optical fields is investigated using two-dimensional time-of-flight spectrometry. Very highly charged ions are formed with a two-component energy distribution. A…

原子与分子团簇 · 物理学 2009-11-10 M. Krishnamurthy , D. Mathur , V. Kumarappan

Energetic H$_2^+$ ions are formed as a result of intra-molecular rearrangement during fragmentation of linear alcohols (methanol, ethanol, propanol, hexanol, and dodecanol) induced by intense optical fields produced by 100 fs long,…

原子物理 · 物理学 2009-11-10 M. Krishnamurthy , F. A. Rajgara , D. Mathur

Ultraperipheral heavy-ion collisions (UPCs) offer unique opportunities to study processes under strong electromagnetic fields. In these collisions, highly charged fast-moving ions carry strong electromagnetic fields that can be effectively…

核理论 · 物理学 2024-06-21 Jie Zhao , Jinhui Chen , Xu-Guang Huang , Yu-Gang Ma

The role of the Coulomb potential of the atomic core for creation of caustics in the photoelectron momentum distribution for tunneling ionization in a linearly polarized strong laser field, usually termed as Coulomb focusing, is…

原子物理 · 物理学 2018-06-20 Jiří Daněk , Karen Z. Hatsagortsyan , Christoph H. Keitel

We develop a time-dependent theory to investigate electron dynamics and photoionization processes of diatomic molecules interacting with strong laser fields including electron-electron correlation effects. We combine the recently formulated…

化学物理 · 物理学 2016-02-02 Henrik R. Larsson , Sebastian Bauch , Lasse Kragh Sørensen , Michael Bonitz

Fragmentation dynamics in the Coulomb explosion of hydrocarbons, specifically methane, ethane, propane, and butane, are investigated using time dependent density functional theory (TDDFT) simulations. The goal of this work is to elucidate…

化学物理 · 物理学 2024-10-11 Samuel S. Taylor , Kálmán Varga , Károly Mogyorósi , Viktor Chikán , Cody Covington

A phenomenological optical potential is generalized to include the Coulomb and nuclear interactions caused by the dynamical deformation of its surface. In the high-energy approach analytical expressions for elastic and inelastic scattering…

核理论 · 物理学 2009-11-11 V. K. Lukyanov , Z. Metawei , E. V. Zemlyanaya

Strong electric fields can be used to align molecules. However, a non-polar molecule such as H$_2$ has no preference for its orientation. There are thus two equivalent configurations with equal energy separated by a potential-energy…

化学物理 · 物理学 2025-12-02 J. Amira Geuther , Marit R. Fiechter , Jeremy O. Richardson