相关论文: Model for Triplet State Engineering in Organic Lig…
Trion states of three correlated particles (e.g., two electrons and one hole) are essential to understand the optical spectra of doped or gated nanostructures, like carbon nanotubes or transition-metal dichalcogenides. We develop a…
Conventional photocells suffer a fundamental efficiency threshold imposed by the principle of detailed balance, reflecting the fact that good absorbers must necessarily also be fast emitters. This limitation can be overcome by `parking' the…
We discuss the transition strength between the disordered ground state and the basic low-lying triplet excitation for the Heisenberg chain with alternating exchange based on series expansions in the interdimer interaction up to tenth order.…
In this paper we consider the essential electronic excited states in parallel chains of semiconducting polymers that are currently being explored for photovoltaic and light-emitting diode applications. In particular, we focus upon various…
The hole doped Si(111)(2root3x2root3)R30(degrees)-Sn interface exhibits a symmetry-breaking insulator-insulator transition below 100 K that appears to be triggered by electron tunneling into the empty surface-state bands. No such transition…
A self-consistent, mean-field model of charge-carrier injection and unipolar transport in an organic semiconductor diode is developed utilizing the effective transport energy concept and taking into account a realistic density-of-states…
The research article studies the unconventional photon blockade effect in a hybrid optomechanical system with an embedded spin-triplet state. The interaction between the optomechanical system and the spin state generates new transition…
The spinel-structure CuIr$_{2}$S$_{4}$ compound displays a rather unusual orbitally-driven three-dimensional Peierls-like insulator-metal transition. The low-T symmetry-broken insulating state is especially interesting due to the existence…
The photoinduced excited-state dynamics of the keto and enol forms of cytosine is investigated using ab initio surface hopping in order to understand the outcome of molecular beam femtosecond pump-probe photoionization spectroscopy…
Electron beams enable highly localized near-field excitation of waveguided optical modes, yet their coupling is typically limited by short interaction times along straight-line trajectories with fixed impact parameters. Here, we…
In this paper we study the ground state phase diagram of a one-dimensional $t-U-J$ model, at half-filling. In the large-bandwidth limit and for ferromagnetic exchange with easy-plane anisotropy, a phase with gapless charge and massive spin…
Third order parametric down-conversion describes a class of nonlinear processes in which a pump photon can be down-converted into triplets of photons. It has been identified as a source of non-classical light, with capabilities beyond those…
Next-generation lithium-ion batteries with silicon anodes have positive characteristics due to higher energy densities compared to state-of-the-art graphite anodes. However, the large volume expansion of silicon anodes can cause high…
We consider a 2D electron system on a square lattice with hopping beyond nearest neighbors. The existence of the quantum critical point associated with an electronic topological transition in the noninteracting system results in density…
We have investigated energies, magnetic dipole hyperfine structure constants ($A_{hyf}$) and electric dipole (E1) matrix elements of a number of low-lying states of the triply ionized tin (Sn$^{3+}$) by employing relativistic…
Radiationless deactivation channels of 2-thiocytosine in aqueous environment are revisited by means of quantum-chemical simulations of excited-state absorption spectra, and investigations of potential energy surfaces of the chromophore…
The low-energy electronic structure of the trilayer cuprate superconductor Bi$_2$Sr$_2$Ca$_2$Cu$_3$O$_{10+\delta}$ near optimal doping is investigated by angle-resolved photoemission spectroscopy. The normal state quasiparticle dispersion…
The performance of nano-scale energy conversion devices is studied in the framework of state-space models where a device is described by a graph comprising states and transitions between them represented by nodes and links, respectively.…
The computational design of heteroatom-doped organic dyes for dye-sensitized solar cells (DSSCs) remains challenging, as predictive methods must accurately describe long-range charge-transfer (CT) excitations while remaining computationally…
Structurally well-defined TIPS-acetylene substituted tetracene (TIPS BT1') and pentacene (TIPS BP1') dimers utilizing a [2.2.1] bicyclic norbornyl bridge have been studied -primarily using time-resolved spectroscopic methods - to uncover…