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Particle plasmons in metal nanoparticles have primarily been investigated through the use of local optical response approximations. However, as nanoparticle size approaches the average distance of electrons to the metal surface, mesoscopic…

光学 · 物理学 2023-06-28 Weixiang Ye

This review provides a broad overview of the studies and effects of nonlocal response in metallic nanostructures. In particular, we thoroughly present the nonlocal hydrodynamic model and the recently introduced generalized nonlocal optical…

光学 · 物理学 2015-04-21 Søren Raza , Sergey I. Bozhevolnyi , Martijn Wubs , N. Asger Mortensen

Non-local effects in the optical response of noble metals are shown to produce significant blueshift and near-field quenching of plasmons in nanoparticle dimers, nanoshells, and thin metal waveguides. Compared with a local description…

其他凝聚态物理 · 物理学 2012-11-13 F. Javier Garcia de Abajo

According to the hydrodynamic Drude model, surface-plasmon resonances of metallic nanostructures blueshift owing to the nonlocal response of the metal's electron gas. The screening length characterising the nonlocal effect is often small…

光学 · 物理学 2016-07-07 Ory Schnitzer , Vincenzo Giannini , Stefan A. Maier , Richard V. Craster

Nonlocal effects have been shown to be responsible for a variety of non-trivial optical effects in small-size plasmonic nanoparticles, beyond classical electrodynamics. However, it is not clear whether optical mode descriptions can be…

A rigorous account of quantum nonlocal effects is paramount for understanding the optical response of metal nanostructures and for designing plasmonic devices at the nanoscale. Here, we present a scheme for retrieving the quantum surface…

介观与纳米尺度物理 · 物理学 2023-09-06 P. A. D. Gonçalves , F. Javier García de Abajo

We provide theoretical and numerical tools to quantitatively study the impact of nonlocality arising from free electrons in metals on the optical properties of metallo-dielectric multilayers. Though effects due to nonlocality are in general…

Theoretical description of oscillations of electron liquid in large metallic nanospheres (with radius of few tens nm) is formulated within random-phase-approximation semiclassical scheme. Spectrum of plasmons is determined including both…

介观与纳米尺度物理 · 物理学 2015-05-14 W. Jacak , J. Krasnyj , J. Jacak , R. Gonczarek , A. Chepok , L. Jacak , D. Z. Hu , D. Schaadt

For the metallic nanoparticles, smaller than the free electron path, an impact of the particle's surface on the nonlocal effects emerging is shown. Light-induced current inside the particle begins to depend on the spatial derivatives of the…

介观与纳米尺度物理 · 物理学 2017-03-08 P. M. Tomchuk , D. V. Butenko

The plasmon response of metallic nanostructures is anticipated to exhibit nonlocal dynamics of the electron gas when exploring the true nanoscale. We extend the local-response approximation (based on Ohm's law) to account for a general…

介观与纳米尺度物理 · 物理学 2014-03-04 N. Asger Mortensen

Surface plasmons on metals can concentrate light into sub-nanometric volumes and on these near atomic length scales the electronic response at the metal interface is smeared out over a Thomas-Fermi screening length. This nonlocality is a…

介观与纳米尺度物理 · 物理学 2015-06-16 Yu Luo , A. I. Fernandez-Dominguez , Aeneas Wiener , S. A. Maier , J. B. Pendry

Optical response of free-electron gas leads to inherent nonlinear optical behaviour of nanostructured plasmonic materials enabled via both strong local field enhancements and inherent complex electron dynamics. We present a comprehensive…

Historically, the field of plasmonics has been relying on the framework of classical electrodynamics, with the local-response approximation of material response being applied even when dealing with nanoscale metallic structures. However,…

The spontaneous emission rate of dipole emitters close to plasmonic dimers are theoretically studied within a nonlocal hydrodynamic model. A nonlocal model has to be used since quantum emitters in the immediate environment of a metallic…

The effect of nonlocality on the optical response of metals lies at the forefront of research in nanoscale physics and, in particular, quantum plasmonics. In alkali metals, nonlocality manifests predominantly as electron density spill-out…

介观与纳米尺度物理 · 物理学 2025-03-06 Ida Juliane Bundgaard , Christian Nicolaisen Hansen , P. Elli Stamatopoulou , Christos Tserkezis

We analyze electromagnetic modes in multi-layered nano-composites and demonstrate that the response of a majority of realistic layered structures is strongly affected by the non-local effects originating from strong field oscillations…

光学 · 物理学 2007-05-25 Justin Elser , Viktor A. Podolskiy , Ildar Salakhutdinov , Ivan Avrutsky

Localized surface plasmons (LSP) in semiconductor particles are expected to exhibit spatial nonlocal response effects as the geometry enters the nanometer scale. To investigate these nonlocal effects, we apply the hydrodynamic model to…

介观与纳米尺度物理 · 物理学 2017-09-13 J. R. Maack , N. A. Mortensen , M. Wubs

We investigate the effects of hydrodynamic nonlocal response in hyperbolic metamaterials (HMMs), focusing on the experimentally realizable parameter regime where unit cells are much smaller than an optical wavelength but much larger than…

光学 · 物理学 2013-06-19 Wei Yan , N. Asger Mortensen , Martijn Wubs

In plasmonics, nonlocal effects arise when the material response to optical excitations is strongly dependent on the spatial correlations of the excitation. It is well known that a classical free electron gas system supports local Drude…

Plasmons in atomically thin materials offer a compelling route to trigger nonlinear light-matter interactions through extreme optical confinement in the two-dimensional (2D) limit. However, optical nonlocality in plasmons is typically…

介观与纳米尺度物理 · 物理学 2025-12-23 Line Jelver , Joel D. Cox
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