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The structure of ionic adsorption layers is studied via a proper thermodynamic treatment of the electrostatic and non-electrostatic interactions between the surfactant ions as well as of the effect of thermodynamic non-locality. The…

软凝聚态物质 · 物理学 2014-10-28 R. Tsekov

A novel wireless microstrip-based RF sensor designed for detecting changes in ionic content of water and the addition of solid contaminant objects is proposed and demonstrated. The sensor can be installed on the exterior wall of dielectric…

信号处理 · 电气工程与系统科学 2024-01-26 Sobhan Gholami , EMre Unal , Hilmi Volkan Demir

We investigate the dynamics of water confined in soft ionic nano-assemblies, an issue critical for a general understanding of the multi-scale structure-function interplay in advanced materials. We focus in particular on hydrated…

材料科学 · 物理学 2017-08-23 Quentin Berrod , Samuel Hanot , Armel Guillermo , Stefano Mossa , Sandrine Lyonnard

Nanopores in solid state membranes are a tool able to probe nanofluidic phenomena or can act as a single molecular sensor. They also have diverse applications in filtration, desalination or osmotic power generation. Many of these…

Some aspects of direct ion transfer across the water/1,2-dichloroethane are analyzed using a very simple model based on thermodynamic considerations. It was concluded that ion solvation by water molecules may occur in some particular cases…

化学物理 · 物理学 2008-02-03 C. Sanchez , S. A. Dassie , A. M. Baruzzi , E. P. M. Leiva

Dynamic fluctuations in hydrogen-bond network of water occur from femto- to nano-second timescale and provides insights into structural/dynamical aspects of water at ion-water interfaces. Employing terahertz spectroscopy assisted with…

软凝聚态物质 · 物理学 2023-06-02 Abhishek K. Singh , Luan C. Doan , Djamila Lou , Chengyuan Wen , Nguyen Q. Vinh

A program is underway to develop liquid-hydrogen energy absorbers for ionization cooling of muon-beam transverse emittance. Minimization of multiple-scattering-induced beam heating requires thin windows. The first window prototype has been…

Porous graphene has high mechanical strength and atomic layer thickness, which make it a promising material for material separation and biomolecule sensing. Electrostatic interactions between charges in aqueous solution are a kind of strong…

化学物理 · 物理学 2016-08-02 Yinghua Qiu , Kun Li , Weiyu Chen , Wei Si , Qiyan Tan , Yunfei Chen

Selective ion transport is a hallmark of biological ion channel behavior but is a major challenge to engineer into artificial membranes. Here, we demonstrate, with all-atom molecular dynamics simulations, that bare graphene nanopores yield…

介观与纳米尺度物理 · 物理学 2017-08-22 Subin Sahu , Michael Zwolak

A field theoretic variational approach is introduced to study ion penetration into water-filled cylindrical nanopores in equilibrium with a bulk reservoir. It is shown that (i) an ion located in a neutral pore undergoes two opposing…

软凝聚态物质 · 物理学 2015-05-19 Sahin Buyukdagli , Manoel Manghi , John Palmeri

We present a coarse-grained model for ionic surfactants in explicit aqueous solutions, and study by computer simulation both the impact of water content on the morphology of the system, and the consequent effect of the formed interfaces on…

软凝聚态物质 · 物理学 2015-03-16 Samuel Hanot , Sandrine Lyonnard , Stefano Mossa

Ion channels form pores across the lipid bilayer, selectively allowing inorganic ions to cross the membrane down their electrochemical gradient. While the study of ion desolvation free-energies have attracted much attention, the role of…

化学物理 · 物理学 2012-07-31 Diego Prada-Gracia , Francesco Rao

We use molecular dynamics simulations in two dimensions to investigate the possibility that a core-softened potential can reproduce static and dynamic anomalies found experimentally in liquid water: (i) the increase in specific volume upon…

软凝聚态物质 · 物理学 2009-10-31 A. Scala , M. Reza Sadr-Lahijany , N. Giovambattista , S. V. Buldyrev , H. E. Stanley

We propose an experiment to observe interference of a single electron as it is transported along two parallel quasi-one-dimensional channels trapped in a single minimum of a travelling periodic electric field. The experimental device is a…

Solvation of ions is ubiquitous on our planet. Solvated ions have a profound effect on the behavior of ionic solutions, which is crucial in nature and technology. Experimentally, ions have been classified into "structure makers" or…

软凝聚态物质 · 物理学 2021-07-27 Rui Shi , Anthony J. Cooper , Hajime Tanaka

Using X-ray free electron laser (XFEL) radiation to conduct an X-ray pump X-ray probe experiment, we studied strongly ionized water as part of our ongoing work on radiation damage. After irradiance with a pump pulse with a nominal fluence…

Water autoionization plays a critical role in determining pH and properties of various chemical and biological processes occurring in the water mediated environment. The strikingly unsymmetrical potential energy surface of the dissociation…

化学物理 · 物理学 2023-12-29 Ling Liu , Yingqi Tian , Chungen Liu

Ion transport through narrow water--filled channels is impeded by a high electrostatic barrier. The latter originates from the large ratio of the dielectric constants of the water and a surrounding media. We show that ``doping'', i.e.…

软凝聚态物质 · 物理学 2009-11-11 J. Zhang , A. Kamenev , B. I. Shklovskii

The extraction of information carried by light plays an increasingly important role in optical communication, imaging, and detection. However, the information can only be successfully extracted when the light pulse is comparably strong,…

光学 · 物理学 2026-05-25 Zhen Yang , Zeng-Quan Yan , Li Wang , Xiao-Wei Wang , Ka-Di Zhu , Xian-Min Jin

A first-principles approach for calculating ion separation in solution through two-dimensional (2D) membranes is proposed and applied. Ionic energy profiles across the membrane are obtained first, where solvation effects are simulated…

软凝聚态物质 · 物理学 2024-12-19 Nicéphore Bonnet , Nicola Marzari
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