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We explore chiroptical phenomena in 3D chiral nano-gap antennas using topology optimization. The characteristic helical geometries of the topology-designed antennas exhibit giant chiral dissymmetry (g=-1.70) considering the gap intensity,…

光学 · 物理学 2024-02-20 Atsushi Taguchi , Yamato Fukui , Keiji Sasaki

Sensitivity to molecular chirality is crucial for many fields, from biology and chemistry to the pharmaceutical industry. By generating superchiral light, nanophotonics has brought innovative solutions to reduce the detection volume and…

Nanoantennas for visible and infrared radiation can strongly enhance the interaction of light with nanoscale matter by their ability to efficiently link propagating and spatially localized optical fields. This ability unlocks an enormous…

光学 · 物理学 2012-07-09 Paolo Biagioni , Jer-Shing Huang , Bert Hecht

We theoretically investigate light matter interactions for chiral molecules in the presence of non-chiral nanoantennas. Isotropic nanostructures supporting optical-frequency electric or magnetic dipoles are sufficient to locally enhance the…

介观与纳米尺度物理 · 物理学 2013-06-14 Aitzol Garcia-Etxarri , Jennifer A. Dionne

Chiral fields with large optical chirality are very important in chiral molecules analysis, sensing and other measurements. Plasmonic nanostructures have been proposed to realize such super chiral fields for enhancing weak chiral signals.…

光学 · 物理学 2015-09-14 Xiaorui Tian , Yurui Fang , Mengtao Sun

Plasmon nanoantennas are extensively used with molecular systems for the chemical and biological ultra-sensing, for boosting the molecular emissive and energy transfer properties, for the nanoscale catalysis, and for building advanced…

A chiral near field with a highly contorted electromagnetic field builds a bridge to match the chiral molecules and light wavelengths with large size differences. It significantly enhances the circular dichroism of chiral molecules and has…

光学 · 物理学 2022-03-23 Li Hu , Zhiguang Sun , Yingdong Nie , Yingzhou Huang , Yurui Fang

Manipulating external stimuli is crucial for enhancing and controlling the optical response in chiral structures. This study introduces chiral structures composed of single, dimer, or trimer arrays of plasmonic and magneto-plasmonic…

Plasmonic nanoantennas containing nano-gaps support "hotspots" for greatly enhanced light-matter interactions, but suffer from inherent high losses, a long-standing issue that hinders practical applications. Here we report a strategy to…

光学 · 物理学 2024-11-25 Xiaoqing Luo , Rixing Huang , Dangyuan Lei , Guangyuan Li

Plasmonic nanoantenna is of promising applications in optical sensing, single-molecular detection, and enhancement of optical nonlinear effect, surface optical spectroscopy, photochemistry, photoemission, photovoltaics, etc. Here we show…

光学 · 物理学 2015-08-14 Qiang Zhang , Jun-Jun Xiao , Meili Li , Dezhuan Han , Lei Gao

Nanophotonic chiral antennas exhibit orders of magnitude higher circular dichroism (CD) compared to molecular systems. Merging magnetism and structural chirality at the nanometric level allows for the efficient magnetic control of the…

The research area of plasmonics promises devices with ultrasmall footprint operating at ultrafast speeds and with lower energy consumption compared to conventional electronics. These devices will operate with light and bridge the gap…

光学 · 物理学 2015-12-22 Shobhit K. Patel , Christos Argyropoulos

We report on a chiral nanostructure, which we term a "butterfly nanoantenna," that, when used in a metasurface, allows the direct conversion of a linearly polarized beam into a nonlinear optical far-field of arbitrary complexity. The…

光学 · 物理学 2017-02-03 A. Calà Lesina , P. Berini , L. Ramunno

The possibility to enhance chiral light-matter interactions through plasmonic nanostructures provides entirely new opportunities for greatly improving the detection limits of chiroptical spectroscopies down to the single molecule level. The…

光学 · 物理学 2016-04-19 M. H. Alizadeh , B. M. Reinhard

A planar chiral plasmonic nanoantenna exhibiting an excitation-chirality-dependent hot spot in a nanogap is numerically investigated. Additionally, the underlying design principles are examined, providing a broadly applicable framework for…

The interaction between circularly polarized (CP) light and matter is governed by two fundamental quantities: spin angular momentum (SAM) and optical chirality (OC). While these quantities are inseparable in free space, they can be…

We present the design and optical characterization of a plasmonic metasurface engineered to exhibit strong polarization anisotropy under both linearly and circularly polarized light. The metasurface consists of geometrically asymmetric gold…

Over the last few years, optical nanoantennas are continuously attracting interest owing to their ability to efficiently confine, localize resonance, and significantly enhanced electromagnetic fields at subwavelength scale. However, such…

光学 · 物理学 2020-10-28 Liyi Hsu , Fadi I. Baida , Abdoulaye Ndao

Chirality is at the origin of life and is ubiquitous in nature. An object is deemed chiral if it is non-superimposable with its own mirror image. This relates to how circularly polarized light interacts with such object, a circular…

In the close vicinity of a chiral nanostructure, the circular dichroism of a biomolecule could be greatly enhanced, due to the interaction with the local superchiral fields. Modest enhancement of optical activity using a planar…

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