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We propose a laser cooling concept for the translational motion of molecules which does not require repeated spontaneous emission by each molecule. The cooling works by repetition of three main steps: velocity selection of a narrow momentum…

量子物理 · 物理学 2007-05-23 C. H. Raymond Ooi , Kar Peter Marzlin , Juergen Audretsch

Recently a number of diatomic and polyatomics molecules has been identified as a prospective systems for Doppler/Sisyphus cooling. Doppler/Sisyphus cooling allows to decrease the kinetic energy of molecules down to microkelvin temperatures…

化学物理 · 物理学 2017-11-22 T. A. Isaev , A. V. Zaitsevskii , E. Eliav

We report on a general method for the rapid production of quantum degenerate gases. Using 174Yb, we achieve an experimental cycle time as low as (1.6-1.8) s for the production of Bose-Einstein condensates (BECs) of (0.5-1) x 10^5 atoms.…

原子物理 · 物理学 2016-04-22 Richard Roy , Alaina Green , Ryan Bowler , Subhadeep Gupta

We present a theoretical analysis of a novel scheme for optical cooling of particles that does not in principle require a closed optical transition. A tightly confined laser beam interacting with a trapped particle experiences a phase…

量子物理 · 物理学 2010-08-23 Peter Horak , André Xuereb , Tim Freegarde

Ultracold polar molecules are an ideal platform for studying many-body physics with long-range dipolar interactions. Experiments in this field have progressed enormously, and several groups are pursuing advanced apparatus for manipulation…

原子物理 · 物理学 2018-04-27 Jacob P. Covey , Luigi De Marco , Oscar L. Acevedo , Ana Maria Rey , Jun Ye

We report on Bose-Einstein condensation (BEC) in a gas of strontium atoms, using laser cooling as the only cooling mechanism. The condensate is formed within a sample that is continuously Doppler cooled to below 1\muK on a narrow-linewidth…

量子气体 · 物理学 2013-09-24 Simon Stellmer , Benjamin Pasquiou , Rudolf Grimm , Florian Schreck

We demonstrate rotational and vibrational cooling of cesium dimers by optical pumping techniques. We use two laser sources exciting all the populated rovibrational states, except a target state that thus behaves like a dark state where…

原子物理 · 物理学 2012-11-13 I. Manai , R. Horchani , H. Lignier , A. Fioretti , M. Allegrini , P. Pillet , D. Comparat

Quantum degenerate molecules represent a new paradigm for fundamental studies and practical applications. Association of already quantum degenerate atoms into molecules provides a crucial shortcut around the difficulty of cooling molecules…

量子气体 · 物理学 2010-08-11 Matt Mackie , Pierre Phou

Understanding collisions between ultracold molecules is crucial for making stable molecular quantum gases and harnessing their rich internal degrees of freedom for quantum engineering. Transient complexes can strongly influence collisional…

In this work we investigate the theory for three different uni-directional population transfer schemes in trapped multilevel systems which can be utilized to cool molecular ions. The approach we use exploits the laser-induced coupling…

量子物理 · 物理学 2010-01-27 C. Lazarou , M. Keller , B. M. Garraway

Beams of atoms and molecules are stalwart tools for spectroscopy and studies of collisional processes. The supersonic expansion technique can create cold beams of many species of atoms and molecules. However, the resulting beam is typically…

原子物理 · 物理学 2012-10-02 Nicholas R. Hutzler , Hsin-I Lu , John M. Doyle

All conventional methods to laser-cool atoms rely on repeated cycles of optical pumping and spontaneous emission of a photon by the atom. Spontaneous emission in a random direction is the dissipative mechanism required to remove entropy…

量子物理 · 物理学 2016-09-08 P. Maunz , T. Puppe , I. Schuster , N. Syassen , P. W. H. Pinkse , G. Rempe

We realize a continuous guided beam of cold deuterated ammonia with a flux of 3e11 ND3 molecules/s and a continuous free-space beam of cold potassium with a flux of 1e16 K atoms/s. A novel feature of the buffer gas source used to produce…

原子物理 · 物理学 2015-05-13 David Patterson , Julia Rasmussen , John M. Doyle

We consider the use of pulse-shaped broadband femtosecond lasers to optically cool rotational and vibrational degrees of freedom of molecules. Since this approach relies on cooling rotational and vibrational quanta by exciting an electronic…

原子物理 · 物理学 2017-09-13 Chien-Yu Lien , Scott R. Williams , Brian Odom

We present a practical roadmap to achieve optical cycling and laser cooling of asymmetric top molecules (ATMs). Our theoretical analysis describes how reduced molecular symmetry, as compared to diatomic and symmetric non-linear molecules,…

原子物理 · 物理学 2020-08-05 Benjamin L. Augenbraun , John M. Doyle , Tanya Zelevinsky , Ivan Kozyryev

One of the demanding frontiers in ultracold quantum science is identifying laser cooling schemes for complex atoms and molecules out of their vast spectra of internal states. Motivated by the prospect of expanding the set of available…

量子物理 · 物理学 2025-02-11 Anna Dawid , Niccolò Bigagli , Daniel W. Savin , Sebastian Will

We report optical trapping of laser-cooled molecules at sufficient density to observe molecule-molecule collisions for the first time in a bulk gas. SrF molecules from a red-detuned magneto-optical trap (MOT) are compressed and cooled in a…

原子物理 · 物理学 2024-05-09 Varun Jorapur , Thomas K. Langin , Qian Wang , Geoffrey Zheng , David DeMille

We explore a technique for decelerating molecules using a static magnetic field and optical pumping. Molecules travel through a spatially varying magnetic field and are repeatedly pumped into a weak-field seeking state as they move towards…

原子物理 · 物理学 2016-09-20 N. J. Fitch , M. R. Tarbutt

Only bosonic molecular species have been directly laser cooled to date, primarily due to an abundance of bosonic isotopes in nature and to their simpler hyperfine structure. Fermionic molecules provide new opportunities for ultracold…

原子物理 · 物理学 2024-08-07 Jinyu Dai , Qi Sun , Benjamin C. Riley , Debayan Mitra , Tanya Zelevinsky

We present a scheme to cool the motional state of neutral atoms confined in sites of an optical lattice by immersing the system in a superfluid. The motion of the atoms is damped by the generation of excitations in the superfluid, and under…

量子物理 · 物理学 2009-09-29 A. J. Daley , P. O. Fedichev , P. Zoller