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There is substantial interest in producing samples of ultracold molecules for possible applications in quantum computation, quantum simulation of condensed matter systems, precision measurements, controlled chemistry, and high precision…

原子物理 · 物理学 2013-05-30 J. F. Barry , E. S. Shuman , E. B. Norrgard , D. DeMille

It has been roughly three decades since laser cooling techniques produced ultracold atoms, leading to rapid advances in a vast array of fields. Unfortunately laser cooling has not yet been extended to molecules because of their complex…

原子物理 · 物理学 2015-05-27 E. S. Shuman , J. F. Barry , D. DeMille

Recently, laser cooling methods have been extended from atoms to molecules. The complex rotational and vibrational energy level structure of molecules makes laser cooling difficult, but these difficulties have been overcome and molecules…

原子物理 · 物理学 2019-02-18 M. R. Tarbutt

Chemical reactions can be surprisingly efficient at ultracold temperatures ( < 1mK) due to the wave nature of atoms and molecules. The study of reactions in the ultracold regime is a new research frontier enabled by cooling and trapping…

原子物理 · 物理学 2017-01-16 Lee R. Liu , Jessie T. Zhang , Yichao Yu , Nicholas R. Hutzler , Yu Liu , Till Rosenband , Kang-Kuen Ni

We propose a general method to cool the translational motion of molecules. Our method is an extension of single photon atomic cooling which was successfully implemented in our laboratory. Requiring a single event of absorption followed by a…

化学物理 · 物理学 2015-05-13 Edvardas Narevicius , S. Travis Bannerman , Mark G. Raizen

A recent progress on laser cooling of molecules is summarized. Since the development during 1980s for atomic species, laser cooling has been the very beginning step to cool and trap atoms for frontier research on quantum simulations,…

原子物理 · 物理学 2023-03-29 Eunmi Chae

A method for decelerating a continuous beam of neutral polar molecules is theoretically demonstrated. This method utilizes non-uniform, static electric fields and regions of adiabatic population transfer to generate a mechanical force that…

原子物理 · 物理学 2015-05-13 Eric R. Hudson

Laser cooling exploits the physics of light scattering to cool atomic and molecular gases to close to absolute zero. It is the crucial initial step for essentially all atomic gas experiments in which Bose-Einstein condensation and, more…

量子气体 · 物理学 2022-09-05 Florian Schreck , Klaasjan van Druten

An increasingly large variety of molecular species are being cooled down to low energies in recent years, and innovative ideas and powerful techniques continue to emerge to gain ever more precise control of molecular motion. In this brief…

量子气体 · 物理学 2024-05-24 Tim Langen , Giacomo Valtolina , Dajun Wang , Jun Ye

Optically trapped laser-cooled polar molecules hold promise for new science and technology in quantum information and quantum simulation. Large numerical aperture optical access and long trap lifetimes are needed for many studies, but these…

We introduce, analyze, and compare two novel methods of Single Photon Cooling that generically cool and compress molecular gases. The first method compresses the molecular gas density by three orders of magnitude and increases collision…

化学物理 · 物理学 2012-05-07 Yuval Shagam , Edvardas Narevicius

Cooling of molecules via free-space dissipative scattering of photons is thought not to be practicable due to the inherently large number of Raman loss channels available to molecules and the prohibitive expense of building multiple…

We demonstrate a scheme for direct absorption imaging of an ultracold ground-state polar molecular gas near quantum degeneracy. A challenge in imaging molecules is the lack of closed optical cycling transitions. Our technique relies on…

量子气体 · 物理学 2015-05-18 D. Wang , B. Neyenhuis , M. H. G. de Miranda , K. -K. Ni , S. Ospelkaus , D. S. Jin , J. Ye

We present the first experimental demonstration of radiation pressure force deflection and direct laser cooling for barium monohydride (BaH) molecules resulting from multiple photon scattering. Despite a small recoil velocity (2.7 mm/s) and…

The last few years have seen rapid progress in the application of laser cooling to molecules. In this review, we examine what kinds of molecules can be laser cooled, how to design a suitable cooling scheme, and how the cooling can be…

原子物理 · 物理学 2021-12-14 N. J. Fitch , M. R. Tarbutt

We have recently demonstrated that optical pumping methods combined with photoassociation of ultra-cold atoms can produce ultra-cold and dense samples of molecules in their absolute rovibronic ground state. More generally, both the external…

原子物理 · 物理学 2013-08-01 I. Manai , R. Horchani , M. Hamamda , A. Fioretti , M. Allegrini , H. Lignier , P. Pillet , D. Comparat

We present a study of Sisyphus cooling of molecules: the scattering of a single-photon remove a substantial amount of the molecular kinetic energy and an optical pumping step allow to repeat the process. A review of the produced cold…

化学物理 · 物理学 2014-04-11 Daniel Comparat

For experiments that require a quantum system to be in the ultra-cold regime, laser cooling is an essential tool. While techniques for laser cooling ions and neutral atoms have been refined and temperatures below the Doppler limit have been…

原子物理 · 物理学 2024-10-31 Caleb Heuvel-Horwitz , S. F. Yelin

We propose an alternative method to laser cooling. Our approach utilizes the extreme brightness of a supersonic atomic beam, and the adiabatic atomic coilgun to slow atoms in the beam or to bring them to rest. We show how internal-state…

Over the past decade, tremendous progress has been made to extend the tools of laser cooling and trapping to molecules. Those same tools have recently been applied to polyatomic molecules (molecules containing three or more atoms). In this…

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