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Using muon spin resonance we examine the organometallic hybrid compound Cu(1,3-benzenedicarboxylate) [Cu(1,3-bdc)], which has structurally perfect spin 1/2 copper kagome planes separated by pure organic linkers. This compound has…

The electron spin resonance (ESR) spectroscopy was employed to investigate the spin dynamics in triangular lattice antiferromagnets CuCr$_{1-x}$Mg$_{x}$O$_2$ with $x =$ 0 and 0.02. All spectra can be well fitted by a single Lorentzian…

强关联电子 · 物理学 2012-07-16 Renwen Li , Zhe Qu , Wei Tong , Yuheng Zhang

We report $^{35}$Cl NMR, ESR, $\mu$SR and specific heat measurements on the $S=1/2$ frustrated kagom\'e magnet kapellasite, $\alpha-$Cu$_3$Zn(OH)$_6$Cl$_2$, where a gapless spin liquid phase is stabilized by a set of competing exchange…

We have performed thermodynamic and neutron scattering measurements on the S=1/2 kagome lattice antiferromagnet Zn Cu_3 (OH)_6 Cl_2. The susceptibility indicates a Curie-Weiss temperature of ~ -300 K; however, no magnetic order is observed…

Muon spin relaxation ($\mu$SR) and magnetic susceptibility measurements have been performed on the pure and diluted spin 1/2 kagom\'{e} system (Cu$_x$Zn$_{1-x}$)$_{3}$V$_{2}$O$_7$(OH)$_{2}$ 2H$_2$O. In the pure $x=1$ system we found a…

High-field electron spin resonance (ESR) measurements have been performed on vesignieite BaCu$_3$V$_2$O$_8$(OH)$_2$, which is considered as a nearly ideal model substance of $S$=1/2 kagome antiferromagnet, in the temperature region from 1.9…

We present thermodynamic studies of a new spin-1/2 antiferromagnet containing undistorted kagome lattices---barlowite Cu$_{4}$(OH)$_{6}$FBr. Magnetic susceptibility gives $\theta_{CW}$ = $-$136 K, while long-range order does not happen…

强关联电子 · 物理学 2014-12-05 Tian-Heng Han , John Singleton , John A. Schlueter

We report the study of high quality samples of the frustrated S = 1/2 kagome antiferromagnet vesignieite, Cu3Ba(VO5H)2. Neutron powder diffraction measurements evidence the high quality of the kagome lattice and show no sign of a transition…

We report thermodynamic measurements of the S=1/2 kagome lattice antiferromagnet ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$, a promising candidate system with a spin-liquid ground state. Using single crystal samples, the magnetic susceptibility both…

强关联电子 · 物理学 2012-04-16 Tianheng Han , Shaoyan Chu , Young S. Lee

We report results of magnetic susceptibility, specific heat, and muon spin relaxation ($\mu$SR) measurements on the polycrystalline Ba$_6$Nd$_2$Ti$_4$O$_{17}$, a disorder-free triangular-lattice antiferromagnet. The absence of long-range…

强关联电子 · 物理学 2024-11-21 C. Y. Jiang , B. L. Chen , K. W. Chen , J. C. Jiao , Y. Wang , Q. Wu , N. Y. Zhang , M. Y. Zou , P. -C. Ho , O. O. Bernal , L. Shu

The spin dynamics of the ferromagnetic Kondo lattice CeRuPO is investigated by Electron Spin Resonance (ESR) at microwave frequencies of 1, 9.4, and 34~GHz. The measured resonance can be ascribed to a rarely observed bulk Ce3+ resonance in…

强关联电子 · 物理学 2010-10-13 T. Förster , J. Sichelschmidt , C. Krellner , C. Geibel , F. Steglich

We report the thermodynamic and muon spin relaxation ($\mu$SR) evidences for a possible gapless spin liquid in Tm$_{3}$Sb$_{3}$Zn$_{2}$O$_{14}$, with the rare-earth ions Tm$^{3+}$ forming a two-dimensional kagom\'{e} lattice. We extract the…

强关联电子 · 物理学 2018-11-09 Zhaofeng Ding , Yanxing Yang , Jian Zhang , Cheng Tan , Zihao Zhu , Gang Chen , Lei Shu

New physics can emerge in magnetic materials where quantum fluctuations are enhanced due to reduced dimensionality and strong frustration. One long sought example is the resonating-valence-bond (RVB) state, where atomic magnetic moments are…

We investigate the lattice dynamics in the spin-1/2 frustrated kagome compound herbertsmithite ZnCu$_3$(OH)$_6$Cl$_2$ by a combination of infrared spectroscopy measurements and ab initio density functional theory calculations, and provide…

强关联电子 · 物理学 2020-04-29 Ying Li , A. Pustogow , M. Bories , P. Puphal , C. Krellner , M. Dressel , Roser Valenti

We study the magnetic properties of the metallic kagome system $\left(\mathrm{Fe}_{1-x} \mathrm{Co}_{x}\right) \mathrm{Sn}$ by a combination of Muon Spin Relaxation ($\mu \mathrm{SR}$), magnetic susceptibility and Scanning Tunneling…

Temperature-dependent dynamical spin correlations, which can be readily accessed via a variety of experimental techniques, hold the potential of offering a unique fingerprint of quantum spin liquids and other intriguing dynamical states. In…

强关联电子 · 物理学 2021-01-21 P. Prelovšek , M. Gomilšek , T. Arh , A. Zorko

Spin-1/2 kagome-lattice Heisenberg antiferromagnet is theoretically known to have a quantum spin liquid ground state, one of the frontiers of condensed matter physics. The search for the model substances has been continued for a long time,…

强关联电子 · 物理学 2024-08-21 Hidekazu Tanaka

Magnetic susceptibility and muon spin relaxation (muSR) experiments have been carried out on the quasi-2D triangular-lattice spin S = 2 antiferromagnet FeGa2S4. The muSR data indicate a sharp onset of a frozen or nearly-frozen spin state at…

We present a Raman spectroscopic investigation of the Herbertsmithite ZnCu3(OH)6Cl2, the first realization of a Heisenberg s=1/2 antiferromagnet on a perfect kagome lattice. The magnetic excitation spectrum of this compound is dominated by…

We consider the polarization function P^{exp}_Z(t) measured by the muon-spin relaxation (muSR) technique for the SrCr8Ga4O19 and ZnCu3(OH)6Cl2 spin-liquid systems. We show the functional form of P^{exp}_Z(t) to imply that, in the…

强关联电子 · 物理学 2022-06-14 P. Dalmas de Reotier , A. Yaouanc
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