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We analyze a polymerization-induced phase separation taking place in solutions of a polymer dissolved in a vinyl monomer undergoing an isothermal free-radical polymerization. The selected system was a solution of polyisobutylene (PIB) in…

材料科学 · 物理学 2013-11-22 Ezequiel R. Soule , Guillermo E. Elicabe , Julio Borrajo , Roberto J. J. Williams

The effect of a linear polymer dissolved in a reactive monomer on the kinetics of free-radical polymerization is studied. The selected system was a solution of polyisobutylene (PIB) in isobornyl methacrylate (IBoMA). Ternary phase diagrams…

材料科学 · 物理学 2013-11-22 Ezequiel R. Soule , Julio Borrajo , Roberto J. J. Williams

We perform a thermodynamic analysis of the polymerization-induced phase separation in nanoparticle-monomer-polymer blends using a simple model recently proposed by V. V. Ginzburg (Macromolecules 2005, 38, 2362.). The model was adapted for…

材料科学 · 物理学 2013-11-22 Ezequiel R. Soule , Julio Borrajo , Roberto J. J. Williams

The morphology and dynamics of polymerization-induced phase separation in the initially homogeneous solution of a non-reactive component in reactive monomers are investigated by incorporating the reaction kinetics into the time-dependent…

软凝聚态物质 · 物理学 2007-05-23 Kaifu Luo

Diblock copolymers by virtue of the chemical dissimilarity between the constituting blocks exhibit microphase separation in the melt state. The phase separated melt can successfully be exploited to control the morphology of the final semi…

软凝聚态物质 · 物理学 2018-02-19 Chitrita Kundu , Nikhil S. Joshi , Ashok Kumar Dasmahapatra

Poly(ethylene terephthalate) (PET) is a semi--crystalline polymer that can be crystallized to different degrees heating from the amorphous state. Even when primary crystallization has been completed, secondary crystallization can take place…

材料科学 · 物理学 2015-05-13 J. Sellares , J. A. Diego , J. Belana

Morphological transitions of phase separation associated with the asymmetry of lipid composition were investigated using micrometer-sized vesicles of lipid bilayers made from a lipid mixture. The complete macro-phase-separated morphology…

生物物理 · 物理学 2015-04-14 Shunsuke F. Shimobayashi , Masatoshi Ichikawa , Takashi Taniguchi

Polymer blends offer an exciting material for various potential applications due to their tunable properties by varying constituting components and their relative composition. Our simulation results unravel an intrinsic relationship between…

软凝聚态物质 · 物理学 2016-10-13 Ashok Kumar Dasmahapatra

We consider polymers made of magnetic monomers (Ising or Heisenberg-like) in a good solvent. These polymers are modeled as self-avoiding walks on a cubic lattice, and the ferromagnetic interaction between the spins carried by the monomers…

统计力学 · 物理学 2009-10-31 T. Garel , H. Orland , E. Orlandini

In this paper, we report dynamic Monte Carlo simulation results on the crystallization of crystalline/crystalline (A/B) symmetric binary polymer blend, wherein the melting temperature of A-polymer is higher than B-polymer. Crystallization…

软凝聚态物质 · 物理学 2015-06-18 Ashok Kumar Dasmahapatra

Experimental and modeling/simulation studies of phase equilibrium and growth morphologies of novel polymer-dispersed liquid crystal (PDLC) mixtures of PS (polystyrene) and liquid crystals that exhibit a direct isotropic/smectic-A (lamellar)…

软凝聚态物质 · 物理学 2015-05-13 Ezequiel R. Soule , Nasser Mohieddin Abukhdeir , Alejandro D. Rey

The kinetics of the free-radical polymerization of isobornyl methacrylate (IBoMA) at 80C, initiated by benzoyl peroxide (BPO), was determined by differential scanning calorimetry (DSC), using sample pans previously sealed in air or in…

材料科学 · 物理学 2013-11-27 Ezequiel R. Soule , Julio Borrajo , Roberto J. J. Williams

Crystallization within the discrete spheres of a block copolymer mesophase was studied by time-resolved x-ray scattering. The cubic packing of microdomains, established by self-assembly in the melt, is preserved throughout crystallization…

软凝聚态物质 · 物理学 2009-10-31 Yueh-Lin Loo , Richard A. Register , Anthony J. Ryan

The isothermal, isobaric spontaneous crystallization of a supercooled polymer melt is investigated by MD simulation of an ensemble of fully-flexible linear chains. Frustration is introduced via two incommensurate length scales set by the…

软凝聚态物质 · 物理学 2018-11-19 Andrea Giuntoli , Sebastiano Bernini , Dino Leporini

Isoporous membranes made from diblock copolymers have numerous applications, including water treatment and protein separation, and are successfully produced at a laboratory scale under controlled conditions. However, achieving optimal…

软凝聚态物质 · 物理学 2023-04-11 Nicolas Moreno , Suzana Nunes , Victor Calo

Block copolymer melts self-assemble in the bulk into a variety of nanostructures, making them perfect candidates to template the position of nanoparticles. The morphological changes of block copolymers are studied in the presence of a…

软凝聚态物质 · 物理学 2019-10-31 Javier Diaz , Marco Pinna , Andrei V. Zvelindovsky , Ignacio Pagonabarraga

We present fully atomistic Molecular Dynamics simulation results on a main-chain polymer, 1,4-Polybutadiene, in the merging region of the $\alpha$- and $beta$-relaxations. A real space analysis reveals the occurrence of localized motions…

软凝聚态物质 · 物理学 2015-06-25 Juan Colmenero , Arturo Narros , Fernando Alvarez , Arantxa Arbe , Angel J. Moreno

Traditional plastics demand a choice between durability (thermosets) and reprocessability (thermoplastics). Vitrimers are a recent class of polymer network combining both these qualities. Their increased cost of production can be offset by…

软凝聚态物质 · 物理学 2026-03-27 A. A. Rispo Constantinou , B. Magyari , G. Ianniruberto , E. van Ruymbeke , D. J. Read

Morphological transformations of amphiphilic AB diblock copolymers in mixtures of a common solvent (S1) and a selective solvent (S2) for the B block are studied using the simulated annealing method. We focus on the morphological…

软凝聚态物质 · 物理学 2017-03-28 Zheng Wang , Yuhua Yin , Run Jiang , Baohui Li

We investigate the phase behaviour of random copolymers melts via large scale Monte Carlo simulations. We observe macrophase separation into A and B--rich phases as predicted by mean field theory only for systems with a very large…

软凝聚态物质 · 物理学 2009-11-07 J. Houdayer , M. Mueller
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