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Coherent anti-Stokes Raman scattering (CARS) microscope system was built and applied to a non-intrusive gas concentration measurement of a mixing flow in a millimeter-scale channel. Carbon dioxide and nitrogen were chosen as test fluids and…

流体动力学 · 物理学 2015-08-07 Ken Yamamoto , Yuki Yamagata , Madoka Moriya , Reiko Kuriyama , Yohei Sato

We have developed an interferometric implementation of coherent anti-Stokes Raman scattering (CARS) which enables broadband coherent Raman spectroscopy free from non-resonant background (NRB), with a signal strength proportional to…

光学 · 物理学 2014-02-25 Brad Littleton , Thomas Kavanagh , Frederic Festy , David Richards

Coherent Anti Stokes Raman Scattering (CARS) offers many advantages for nonlinear bio-imaging, thanks to its sub-cellular spatial resolution and unique chemical specificity. Its working principle requires two incident pulsed laser beams…

光学 · 物理学 2020-08-19 Matthias Hofer , Siddarth Shivkumar , Bilal El Waly , Sophie Brasselet

Stimulated Raman scattering is a well-known nonlinear process that can be harnessed to produce optical gain in a wide variety of media. This effect has been used to produce the first silicon-based lasers and high-gain amplifiers.…

光学 · 物理学 2008-10-13 D. R. Solli , P. Koonath , B. Jalali

We theoretically investigate a scheme in which backward coherent anti-Stokes Raman scattering (CARS) is significantly enhanced by using slow light. Specifically, we reduce the group velocity of the Stokes excitation pulse by introducing a…

光学 · 物理学 2017-01-03 Li Gong , Haifeng Wang

Frequency modulation coherent anti-Stokes Raman scattering (FM CARS) is presented, using a compact as well as fast and widely tunable fiber-based light source. With this light source Raman resonances between 700 cm$^{-1}$ and 3200 cm$^{-1}$…

Since its first demonstration in the sixties, coherent anti-Stokes Raman scattering (CARS) has become a powerful spectroscopic sensing tool with broad applications in biology and chemistry. However, it is a complex nonlinear optical process…

光学 · 物理学 2020-07-15 Gombojav O. Ariunbold , Supriya Nagpal , Bryan Semon

Nonlinear optics in photonic integrated circuits is usually limited to utilizing the nonlinearity of a single material. In this work, we demonstrate the use of hybrid optical nonlinearities that occur in two different materials. This…

An integrated silicon nitride resonator is proposed as an ultra-compact source of bright single-mode quadrature squeezed light at 850 nm. Optical properties of the device are investigated and tailored through numerical simulations, with…

量子物理 · 物理学 2023-07-19 Ulrich B. Hoff , Bo M. Nielsen , Ulrik L. Andersen

We propose a new technique for comparing two Raman active samples. The method employs optical interference of the signals generated via coherent anti-Stokes Raman scattering (CARS) of broadband laser pulses with noisy spectra. It does not…

量子物理 · 物理学 2015-05-27 Evgeny A. Shapiro , Stanislav O. Konorov , Valery Milner

Single-shot time resolved Coherent Anti-Stokes Raman Scattering (CARS) is presented as a viable method for fast measurements of molecular spectra. The method is based on the short spatial extension of femtosecond pulses and maps time delays…

光学 · 物理学 2009-11-13 Yuri Paskover , I. Sh. Averbukh , Yehiam Prior

We present a scheme for an integrated four-wave mixing source of narrow-band path-entangled photon pairs with efficient spatial pump self-rejection. The scheme is based on correlated loss in a system of waveguides in Kerr nonlinear media.…

量子物理 · 物理学 2021-06-02 P. de la Hoz , A. Sakovich , A. Mikhalychev , M. Thornton , N. Korolkova , D. Mogilevtsev

Coherent anti-Stokes Raman scattering (CARS) spectroscopy with time-delayed ultrashort pulses and a single-pixel photodetector has shown great potential for spectroscopic imaging and transient studies in chemistry and biological research.…

光学 · 物理学 2023-12-05 Tianjian Lv , Bing Han , Ming Yan , Zhaoyang Wen , Kun Huang , Kangwen Yang , Heping Zeng

Silicon nitride (SiN) has emerged as a promising platform for integrated nonlinear photonics because of its low propagation loss, wide transparency window, and CMOS compatibility. Nonlinear processes arising from photon-electron…

State-preserving frequency conversion in the optical domain is a necessary component in many configurations of quantum information processing and communication. Thus far, nonlinear crystals are used for this purpose. Here, we report on a…

量子物理 · 物理学 2022-12-28 Alireza Aghababaei , Christoph Biesek , Frank Vewinger , Simon Stellmer

We experimentally demonstrate wide-band (>100 THz) frequency down-conversion of near-infrared (NIR) femtosecond-scale pulses from an Er:fiber laser to the mid-infrared (MIR) using four-wave-mixing (FWM) in photonic-chip silicon-nitride…

Silicon nitride (Si3N4), as a complementary metal-oxide-semiconductor (CMOS) material, finds wide use in modern integrated circuit (IC) technology. The past decade has witnessed tremendous development of Si3N4 in photonic areas, with…

We report stimulated Raman spectroscopy of the G phonon in both single and multi-layer graphene, through Coherent anti-Stokes Raman Scattering (CARS). The signal generated by the third order nonlinearity is dominated by a vibrationally…

介观与纳米尺度物理 · 物理学 2019-09-11 A. Virga , C. Ferrante , G. Batignani , D. De Fazio , A. D. G. Nunn , A. C. Ferrari , G. Cerullo , T. Scopigno

We present a tunable, hybrid waveguide-fiber optical parametric oscillator (OPO) synchronously pumped by an ultra-fast fiber laser exploiting four-wave mixing (FWM) generated in silicon nitride waveguides. Parametric oscillation results in…

We present multi-color imaging by stimulated Raman scattering (SRS) enabled by an ultrafast fiber-based light source with integrated amplitude modulation and frame-to-frame wavelength tuning. With a relative intensity noise level of -153.7…

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