相关论文: The effect of pump depletion on reversible photode…
The influence of an applied electric field on reversible photodegradation of disperse orange 11 (DO11) doped into PMMA is measured using digital imaging and conductivity measurements. Correlations between optical imaging, which measures…
We use amplified spontaneous emission (ASE) and linear absorption spectroscopy to study the mechanisms of reversible photodegradation of 1-amino-2-methylanthraquinone (disperse orange 11-DO11) in solid poly(methyl methacrylate).…
In this work, we show that reversible photodegradation of Disperse Orange 11 doped in PMMA is not due to dye diffusion - a common phenomenon observed in many dye-doped polymers. The change in linear absorbance due to photodegradation of the…
Using a white light interferometric microscope (WLIM) we measure the photodamage induced change in the complex index of refraction of disperse orange 11 (DO11) dye-doped (poly)methyl-methacrylate. We find that the change in the imaginary…
We report on optical imaging studies of self-healing after laser-induced photodamage in disperse orange 11 dye doped into poly(methyl methacrylate) (PMMA) polymer. In particular, the high spatial-contrast image of the damage track made by a…
We report the observation of intensity feedback random lasing at 645 nm in Disperse Orange 11 dye-doped PMMA (DO11/PMMA) with dispersed ZrO$_2$ nanoparticles (NPs). The lasing threshold is found to increase with concentration, with the…
We report on the dynamics of photodegradation and subsequent recovery of two-photon fluorescence in a dye-doped polymer. The energy dependence suggests that photo-degradation is a linear process while recovery is entropic. Such recovery…
The mechanism of reversible photodegradation of 1-substituted aminoanthraquinones doped into poly(methyl methacrylate) and polystyrene is investigated. Time-dependent density functional theory is employed to predict the transition energies…
Using transmittance imaging microscopy we measure the wavelength dependence of reversible photodegradation in disperse orange 11 (DO11) dye-doped (poly)methyl-methacrylate (PMMA). The reversible and irreversible inverse quantum efficiencies…
One of the fundamental difficulties in implementing organic dyes in random lasers is irreversible photodegradation of the dye molecules, leading to loss of performance and the need to replace the dye. We report the observation of…
Resonant optical pumping in dense atomic media is discussed, where the absorption length is less than the smallest characteristic dimension of the sample. It is shown that reabsorption and multiple scattering of spontaneous photons…
Temperature dependent photodegradation and recovery studies of Dipserse Orange 11 (DO11) dye dissolved in poly(methyl methacrylate) and polystyrene polymer hosts are used as a test of the recently proposed correlated chromophore domain…
One of the primary difficulties in the implementation of organic-dye-based random lasers is the tendency of organic dyes to irreversibly photodecay. In this letter we report the observation of "reversible" photodegradation in a Rhodamine 6G…
Reversible photodegradation is a process that has been observed in several dye molecules, but the underlying mechanisms are not still well understood. In this contribution, we characterize a series of anthraquinone dyes to determine how…
Experimental and numerical investigation of single-beam and pump-probe interaction with a resonantly absorbing dense extended medium under strong and weak field-matter coupling is presented. Significant probe beam amplification and conical…
We examine how intense optical beams can penetrate deeply into highly absorbing media by a non-linear, photo-bleaching process. The role of stimulated recovery to the dye ground state can be important and is delineated. This analysis of…
All observations of photodegradation and self healing follow the predictions of the correlated chromophore domain model. [Ramini et.al. Polym. Chem., 2013, 4, 4948.] In the present work, we generalize the domain model to describe the…
We have developed a white light interferometric microscope (WLIM), which can spatially resolve the change in the complex index of refraction and apply it to study reversible photodegradation of 1,4-Diamino-9,10-anthraquinone doped into…
Integrated microring resonators have a broad range of applications in diverse fields with the potential to design compact, robust, energy-efficient devices crucial for quantum applications. Degenerate optical parametric oscillations (DOPOs)…
Photoreflectance is used for the characterisation of semiconductor samples, usually by sweeping the monochromatized probe beam within the energy range comprised between the highest value set by the pump beam and the lowest absorption…