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The thermoelectric properties of n type nanoscale three dimensional (3D) Si phononic crystals (PnCs) with spherical pores are studied. Density functional theory and Boltzmann transport equation under the relaxation time approximation are…

材料科学 · 物理学 2014-10-31 Lina Yang , Nuo Yang , Baowen Li

The thermal conductivity of nanostructures needs to be as small as possible so that it will have a greater efficiency for solid-state electricity generation/refrigeration by thermoelectrics. We studied how the period length and the mass…

介观与纳米尺度物理 · 物理学 2013-01-14 Lina Yang , Nuo Yang , Baowen Li

Thermal phonon transport in square- and triangular-lattice Si phononic crystal (PnC) nanostructures with a period of 300 nm was investigated by measuring the thermal conductivity using micrometer-scale time-domain thermoreflectance. The…

介观与纳米尺度物理 · 物理学 2015-05-22 Junki Nakagawa , Yuta Kage , Takuma Hori , Junichiro Shiomi , Masahiro Nomura

Porous materials provide a large surface to volume ratio, thereby providing a knob to alter fundamental properties in unprecedented ways. In thermal transport, porous nanomaterials can reduce thermal conductivity by not only enhancing…

Thermoelectric device is a promising next-generation energy solution owing to its capability to transform waste heat into useful electric energy, which can be realized in materials with high elec- tric conductivities and low thermal…

材料科学 · 物理学 2018-07-10 Kisung Chae , Seoung-Hun Kang , Seon-Myeong Choi , Duck Young Kim , Young-Woo Son

Introducing hierarchical disorder from multiple defects into materials through nanostructuring is one of the most promising directions to achieve extremely low thermal conductivities and thus improve thermoelectric performance. The success…

材料科学 · 物理学 2019-09-16 Laura de Sousa Oliveira , Vassilios Vargiamidis , Neophytos Neophytou

Controlling thermal transport at the nanoscale is vital for many applications. Previously, it has been shown that this control can be achieved with periodically nanostructured two-dimensional phononic crystals, for the case of suspended…

介观与纳米尺度物理 · 物理学 2024-06-12 Samuli Heiskanen , Tuomas Puurtinen , Ilari J. Maasilta

Engineering materials to include nanoscale porosity or other nanoscale structures has become a well-established strategy for enhancing the thermoelectric performance of dielectrics. However, the approach is only considered beneficial for…

材料科学 · 物理学 2021-10-14 Hosseini , S. Aria , Romano , Giuseppe , Greaney , P. Alex

Boundary scattering in hierarchically disordered nanomaterials is an effective way to reduce the thermal conductivity of thermoelectric materials and increase their performance. In this work we investigate thermal transport in silicon based…

材料科学 · 物理学 2019-02-27 Dhritiman Chakraborty , Laura de Sousa Oliveira , Neophytos Neophytou

Low dimensional materials provide the possibility of improved thermoelectric performance due to the additional length scale degree of freedom for engineering their electronic and thermal properties. As a result of suppressed phonon…

介观与纳米尺度物理 · 物理学 2010-06-23 Neophytos Neophytou , Martin Wagner , Hans Kosina , Siegfried Selberherr

The addition of porosity to thermoelectric materials can significantly increase the figure of merit, ZT, by reducing the thermal conductivity. Unfortunately, porosity is also detrimental to the thermoelectric power factor in the numerator…

介观与纳米尺度物理 · 物理学 2021-03-29 S. Aria Hosseini , Giuseppe Romano , P. Alex Greaney

As a result of suppressed phonon conduction, large improvements of the thermoelectric figure of merit, ZT, have been recently reported for nanostructures compared to the raw materials' ZT values. It has also been suggested that low…

介观与纳米尺度物理 · 物理学 2011-04-11 Neophytos Neophytou , Hans Kosina

It has been proposed for a long time now that the reduction of the thermal conductivity by reducing the phonon mean free path is one of the best way to improve the current performance of thermoelectrics. By measuring the thermal conductance…

Thermoelectrics (TE) materials manifest themselves in direct conversion of temperature differences to electric power and vice versa. Despite remarkable advances have been achieved in the past decades for various TE systems, the energy…

材料科学 · 物理学 2017-07-11 Yanguang Zhou , Xiaojing Gong , Ben Xu , Ming Hu

Nanoporous materials are of broad interest for various applications, in particular advanced thermoelectric materials. The introduction of nanoscale porosity, even at modest levels, has been known to drastically reduce a materials thermal…

介观与纳米尺度物理 · 物理学 2019-07-31 Laura de Sousa Oliveira , Neophytos Neophytou

Nano-engineering crystalline materials can be used to tailor their thermal properties. By adding new nanoscale phonon scattering centers and controlling their size, one can effectively decrease the phonon mean free path and hence the…

Periodic hole array phononic crystals (PnC) can strongly modify the phonon dispersion relations, and have been shown to influence thermal conductance coherently, especially at low temperatures where scattering is suppressed. One very…

介观与纳米尺度物理 · 物理学 2019-07-10 Yaolan Tian , Tuomas A. Puurtinen , Zhuoran Geng , Ilari J. Maasilta

Boundary-engineering in nanostructures has the potential to dramatically impact the development of materials for high-efficiency conversion of thermal energy directly into electricity. In particular, nanostructuring of semiconductors can…

材料科学 · 物理学 2016-10-04 Giuseppe Romano , Alexie M. Kolpak

Herein, we report the use of nanostructured crystalline Si as a thermoelectric material and its integration into thermoelectric harvesters. The proof-of-concept relies on the partial suppression of lattice thermal transport by introducing…

Nanoporous materials are a promising platform for thermoelectrics in that they offer high thermal conductivity tunability while preserving good electrical properties, a crucial requirement for high- effciency thermal energy conversion.…

材料科学 · 物理学 2017-09-20 Giuseppe Romano , Jeffrey C. Grossman
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