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Bimetallic rod-shaped nanomotors swim autonomously in hydrogen peroxide solutions. Here we present a scaling analysis, computational simulations, and experimental data that show that the nanomotor locomotion is driven by fluid slip around…

流体动力学 · 物理学 2010-07-12 J. L. Moran , P. M. Wheat , J. D. Posner

Gold-capped Janus particles immersed in a near-critical binary mixture can be propelled using illumination. We employ a non-isothermal diffuse interface approach to investigate the self-propulsion mechanism of a single colloid. We attribute…

软凝聚态物质 · 物理学 2015-11-04 Sela Samin , René van Roij

Self-propulsion of catalytic Janus swimmers in electrolyte solutions is induced by inhomogeneous ion release from their surface. Here, we consider the experimentally relevant cases of particles which emit only one type of ions (type I) or…

软凝聚态物质 · 物理学 2023-10-19 Evgeny S. Asmolov , Olga I. Vinogradova

In this work, we numerically investigate the dynamics of a self-propelling autophoretic Janus particle in a weakly viscoelastic fluid. The self-propulsion is achieved by an asymmetry in the properties of the surface of the Janus particle…

流体动力学 · 物理学 2018-01-17 Giovanniantonio Natale , Charu Datt , Savvas G. Hatzikiriakos , Gwynn J. Elfring

Most available theoretical predictions for the self-diffusiophoretic motion of colloidal particles are based on the hydrodynamic thin boundary layer approximation in combination with a solvent body force due to a self-generated local solute…

软凝聚态物质 · 物理学 2019-06-19 Thomas Speck

A small, bimetallic particle in a hydrogen peroxide solution can propel itself by means of an electrocatalytic reaction. The swimming is driven by a flux of ions around the particle. We model this process for the presence of a monovalent…

软凝聚态物质 · 物理学 2015-06-04 Benedikt Sabass , Udo Seifert

We report simulations of a spherical Janus particle undergoing exothermic surface reactions around one pole only. Our model excludes self-phoretic transport by design. Nevertheless, net motion occurs from direct momentum transfer between…

软凝聚态物质 · 物理学 2020-05-13 Shaltiel Eloul , Wilson C K Poon , Oded Farago , Daan Frenkel

We present a detailed theoretical study which demonstrates that electrokinetic effects can also play a role in the motion of metallic-insulator spherical Janus particles. Essential to our analysis is the identification of the fact that the…

软凝聚态物质 · 物理学 2017-10-09 Yahaya Ibrahim , Ramin Golestanian , Tanniemola B. Liverpool

Catalytically active Janus particles suspended in solution create gradients in the chemical composition of the solution along their surfaces, as well as along any nearby container walls. The former leads to self-phoresis, while the latter…

软凝聚态物质 · 物理学 2016-09-22 W. E. Uspal , M. N. Popescu , S. Dietrich , M. Tasinkevych

Catalytic Janus swimmers demonstrate a diffusio-phoretic motion by self-generating the gradients of concentrations and electric potential. Recent work has focused on simplified cases, such as a release of solely one type of ions or low…

软凝聚态物质 · 物理学 2022-04-06 Evgeny S. Asmolov , Tatiana V. Nizkaya , Olga I. Vinogradova

We numerically study the escape kinetics of a self-propelled Janus particle, carrying a cargo, from a meta-stable state. We assume that the cargo is attached to the Janus particle by a flexible harmonic spring. We take into account the…

软凝聚态物质 · 物理学 2018-12-31 Tanwi Debnath , Pulak Kumar Ghosh

We theoretically study the active motion of self-diffusiophoretic Janus particles (JPs) using the Onsager-Casimir reciprocal relations. The linear and angular velocity of a single JP are shown to respectively result from a coupling of…

软凝聚态物质 · 物理学 2019-10-30 Jérôme Burelbach , Holger Stark

Charged colloidal particles propel themselves through asymmetric fluxes of chemically generated ions on their surface. We show that asymmetry in the surface charge distribution introduces a new mode of self-phoretic motion for chemically…

软凝聚态物质 · 物理学 2023-05-03 Ahis Shrestha , Monica Olvera de la Cruz

The dynamics of self-propelled colloidal particles are strongly influenced by their environment through hydrodynamic and, in many cases, chemical interactions. We develop a theoretical framework to describe the motion of confined active…

流体动力学 · 物理学 2025-08-29 Günther Turk , Rajesh Singh , Howard A. Stone

Suspended colloidal particles interacting chemically with a solute are able to self-propel by autophoretic motion when they are asymmetrically patterned (Janus colloids). Here we demonstrate that the chemical anisotropy is not a necessary…

软凝聚态物质 · 物理学 2013-06-28 Sebastien Michelin , Eric Lauga , Denis Bartolo

Self-phoretic Janus particles move by inducing -- via non-equilibrium chemical reactions occurring on their surfaces -- changes in the chemical composition of the solution in which they are immersed. This process leads to gradients in…

软凝聚态物质 · 物理学 2018-01-30 W. E. Uspal , M. N. Popescu , M. Tasinkevych , S. Dietrich

Catalytic microswimmers typically swim close to walls due to hydrodynamic and/or phoretic effects. The walls in turn are known to affect their propulsion, making it difficult to single out the contributions that stem from particle-based…

We experimentally investigate active motion of spherical Janus colloidal particles in a viscoelastic fluid. Self-propulsion is achieved by a local concentration gradient of a critical polymer mixture which is imposed by laser illumination.…

软凝聚态物质 · 物理学 2016-03-31 Juan Ruben Gomez-Solano , Alex Blokhuis , Clemens Bechinger

Recent findings of possible applications of bio-friendly synthetic self-phoretic swimmers, have motivated the researchers in investigating the various motion-generating mechanisms to optimize the operating characteristics of the same. In…

流体动力学 · 物理学 2019-05-09 Antarip Poddar , Aditya Bandopadhyay , Suman Chakraborty

A locally heated Janus colloid can achieve motion in a fluid through the coupling of dissolved ions and the medium's polarizibility to an imposed temperature gradient, an effect known as self-thermo(di)electrophoresis. We numerically study…

软凝聚态物质 · 物理学 2019-05-02 Joost de Graaf , Sela Samin
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