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Electron-positron interactions have been utilized in various fields of science. Here we develop time-dependent multi-component density functional theory to study the coupled electron-positron dynamics from first principles. We prove that…

化学物理 · 物理学 2018-10-03 Yasumitsu Suzuki , Satoshi Hagiwara , Kazuyuki Watanabe

Many-body correlation plays a crucial role in the low-energy positron-molecule scattering dynamics. In the present work, we have integrated a recent model correlation potential, developed by Swann and Gribakin, with the single-center…

原子与分子团簇 · 物理学 2025-09-22 Snigdha Sharma , Dhanoj Gupta

The recent theoretical and experimental activities in positronium (Ps) scattering by atoms and molecules are reviewed with special emphasis at low energies. We critically compare the results of different groups $-$ theoretical and…

化学物理 · 物理学 2009-11-07 Sadhan K. Adhikari

Using a complex model potential, we have calculated the total, integrated elastic, momentum transfer, absorption, and differential cross sections for positrons scattered from molecular hydrogen. The widely available software package…

原子物理 · 物理学 2009-11-10 David D. Reid , William B. Klann , J. M. Wadehra

A many-body theory approach is developed for the problem of positron-atom scattering and annihilation. Strong electron-positron correlations are included non-perturbatively through the calculation of the electron-positron vertex function.…

原子物理 · 物理学 2007-05-23 G. F. Gribakin , J. Ludlow

Positron binding energies and Dyson orbitals for five-membered heterocycles with N, O, S and NH substituents are predicted \emph{ab initio} via many-body theory. The positron-molecule correlation potential (self energy) is calculated via…

化学物理 · 物理学 2026-05-11 S. K. Gregg , D. G. Green

The scattering of ortho-positronium (Ps) by hydrogen atoms has been investigated in a five-state coupled-channel model allowing for Ps(1s)H(2s,2p) and Ps(2s,2p)H(1s) excitations using a recently proposed electron-exchange model potential.…

原子与分子团簇 · 物理学 2008-12-18 Sadhan K. Adhikari , P. K. Biswas

The many-body system comprising a He nucleus, three electrons, and a positron has been studied using the exact diagonalization technique. The purpose has been to clarify to which extent the system can be considered as a distinguishable…

原子与分子团簇 · 物理学 2013-05-31 A. Zubiaga , F. Tuomisto , M. J. Puska

Different computational methods are employed to evaluate elastic (rotationally summed) integral and differential cross sections for low energy (below about 10 eV) positron scattering off gas-phase C$_2$H$_2$ molecules. The computations are…

We investigate the modeling of positronium (Ps) states and their pick-off annihilation trapped at open volumes pockets in condensed molecular matter. Our starting point is the interacting many-body system of Ps and a He atom because it is…

原子与分子团簇 · 物理学 2014-10-20 A. Zubiaga , F. Tuomisto , M. Puska

The production of a Bose-Einstein condensate made of positronium may be feasible in the near future. Below the condensation temperature, the positronium collision process is modified by the presence of the condensate. This makes the…

量子物理 · 物理学 2016-05-04 O. Morandi , P. -A. Hervieux , G. Manfredi

We calculate the `exact' potential corresponding to a one-dimensional interacting system of two electrons with a specific, tailored density. We use one-dimensional density-functional theory with a local-density approximation (LDA) on the…

其他凝聚态物理 · 物理学 2015-05-13 J. P. Coe , I. D'Amico

We present the positron coupled cluster singles and doubles (POS-CCSD) method to calculate positron binding energies in molecules. This framework treats electrons and positrons on an equal footing and includes up to simultaneous…

化学物理 · 物理学 2026-03-23 Rosario R. Riso , Jan Haakon M. Trabski , Federico Rossi , Dermot Green , Henrik Koch

The positron-hydrogen atom scattering system is considered within the S-wave model. Convergence in the elastic scattering, excitation, ionization, and positronium formation channels is studied as a function of the number and type of states…

原子物理 · 物理学 2009-10-31 Alisher S. Kadyrov , Igor Bray

Positron scattering and annihilation on noble gas atoms below the positronium formation threshold is studied ab initio using many-body theory methods. The many-body theory provides a near-complete understanding of the…

原子物理 · 物理学 2014-09-12 D. G. Green , J. A. Ludlow , G. F. Gribakin

New results are presented for Ps(1s) scattering by H(1s), He(1$^1$S) and Li(2s). Calculations have been performed in a coupled state framework, usually employing pseudostates, and allowing for excitation of both the Ps and the atom. In the…

原子物理 · 物理学 2015-06-26 H R J Walters , A C H Yu , S Sahoo , Sharon Gilmore

Calculations of the relaxation energy, contact pair-correlation function, and annihilating-pair momentum density for a single positron immersed in a homogeneous electron gas are presented. We achieve an accurate description of the…

介观与纳米尺度物理 · 物理学 2011-01-20 N. D. Drummond , P. Lopez Rios , C. J. Pickard , R. J. Needs

We present a new method to calculate the total ion-ion interaction potential in terms of building blocks which we refer to as "single-particle interaction potentials". This allows also to compose the separate contributions from neutrons and…

核理论 · 物理学 2012-01-06 A. S. Umar , V. E. Oberacker , J. A. Maruhn , P. -G. Reinhard

Self-interactions (SIs) are a major problem in density functional approximations and the source of serious divergence from experimental results. Here, we propose to optimize density functional total energies in terms of the effective local…

其他凝聚态物理 · 物理学 2012-06-20 Nikitas I. Gidopoulos , Nektarios N. Lathiotakis

The scattering of ortho positronium (Ps) by H$_2$ has been investigated using a three-Ps-state [Ps(1s,2s,2p)H$_2($X $^1\Sigma_g^+$)] coupled-channel model and using Born approximation for higher excitations and ionization of Ps and B…

原子与分子团簇 · 物理学 2009-11-06 P. K. Biswas , Sadhan K. Adhikari
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