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Cooperative Jahn-Teller ordering is well-known to drive the cubic $Fd\overline{3}m$ to tetragonal $I$4$_1$/$amd$ structural distortion in Mn$_3$O$_4$ at 1170 $^{\circ}$C. Further structural distortion occurs in Mn$_3$O$_4$ upon magnetic…

材料科学 · 物理学 2014-08-26 Moureen C. Kemei , Jaye K. Harada , Ram Seshadri , Matthew R. Suchomel

We present temperature-, magnetic-field-, and pressure-dependent Raman scattering studies of single crystal Mn3O4, combined with temperature- and field-dependent x-ray diffraction studies, revealing the novel magnetostructural phases in…

强关联电子 · 物理学 2015-05-28 M. Kim , X. M. Chen , X. Wang , C. S. Nelson , R. Budakian , P. Abbamonte , S. L. Cooper

We report the magnetic properties of $A$-site spinel compound MnSc$_2$Se$_4$. The macroscopic magnetic measurements uncovers successive magnetic transitions at $T_{\rm{N1}}$= 2.04 K, followed by two further transitions at $T_{\rm{N2}}$=1.8…

强关联电子 · 物理学 2022-06-01 K. Guratinder , V. Tsurkan , L. Prodan , L. Keller , J. P. Embs , F. Juranyi , M. Medarde , Ch. Rüegg , O. Zaharko

Two magnetic ordering transitions are found in InMnO3, the paramagnetic to antiferromagnetic transition near ~118 K and a lower possible spin rotation transition near ~42 K. Multiple length scale structural measurements reveal enhanced…

材料科学 · 物理学 2015-06-22 T. Yu , T. A. Tyson , P. Gao , T. Wu , X. Hong , S. Ghose , Y. -S. Chen

The structural, magnetic, and electronic properties of NdFe$_{0.5}$Mn$_{0.5}$O$_3$ have been studied in detail using bulk magnetization, neutron/x-ray diffraction and first principles density functional theory calculations. The material…

强关联电子 · 物理学 2017-10-25 Ankita Singh , A. Jain , Avijeet Ray , B. Padmanabhan , S. M. Yusuf , T. Maitra , V. K. Malik

Neutron and X-ray diffraction, magnetic susceptibility, and specific heat measurements have been used to investigate the magnetic and structural phase transitions of the spinel system Fe1+xCr2-xO4(0.0<=x<=1.0). The temperature versus Fe…

We present temperature-dependent x-ray diffraction and temperature- and field-dependent Raman scattering studies of single crystal Mn3O4, which reveal the novel magnetostructural phases that evolve in the spinels due to the interplay…

强关联电子 · 物理学 2015-05-14 M. Kim , X. M. Chen , E. Fradkin , P. Abbamonte , S. L. Cooper

MnAs exhibits a first-order phase transition from a ferromagnetic, high-spin metal NiAs-type hexagonal phase to a paramagnetic, lower-spin insulator MnP-type orthorhombic phase at T_C = 313 K. Here, we report the results of neutron…

材料科学 · 物理学 2009-11-07 J. Mira , F. Rivadulla , J. Rivas , A. Fondado , R. Caciuffo , F. Carsughi , T. Guidi , J. B. Goodenough

The magnetic structures and the magnetic phase transitions in the Mn-doped orthoferrite TbFeO$_3$ studied using neutron powder diffraction are reported. Magnetic phase transitions are identified at $T^\mathrm{Fe/Mn}_N \approx$ 295~K where a…

The structural and magnetic properties of the hexagonal four-layer form of SrMnO$_3$ have been investigated by combining magnetization measurements, electron diffraction and high-resolution synchrotron X-ray and neutron powder diffraction.…

强关联电子 · 物理学 2007-05-23 A. Daoud-Aladine , C. Martin , L. C. Chapon , M. Hervieu , K. S. Knight , M. Brunelli , P. G. Radaelli

Spin wave dispersion in the metallic antiferromagnet Mn$_3$Pt was investigated just above the order-order transition temperature by using the inelastic neutron scattering technique. The spin wave dispersion at $T = 400$ K along [100], [110]…

The crystal and magnetic structures of the spinel compounds ZnCr$_2$S$_4$ and ZnCr$_2$Se$_4$ were investigated by high resolution powder synchrotron and neutron diffraction. ZnCr$_2$Se$_4$ exhibits a first order phase transition at $T_N=21$…

Magnetization, neutron diffraction and X-ray diffraction of Zn doped MnV2O4 as a function of temperature have been measured and the critical exponents and magnetocaloric effect of this system have been estimated. It is observed, that with…

A variable temperature neutron and synchrotron diffraction study have been performed on the giant magnetoresistant oxypnictides LnMnAsO (Ln = La, Nd). The low temperature magnetic structures have been studied and results show a spin…

强关联电子 · 物理学 2012-07-05 N. Emery , E. J. Wildman , J. M. S. Skakle , R. I. Smith , A. N. Fitch , A. C. Mclaughlin

Cubic spinel GeNi2O4 exhibits intriguing magnetic properties with two successive antiferromagnetic phase transitions (TN1 12.1 and TN2 11.4 K) with the absence of any structural transition. We have performed detailed heat capacity and…

强关联电子 · 物理学 2020-12-02 T. Basu , T. Zou , Z. Dun , C. Q. Xu , C. R. Dela Cruz , Tao Hong , H. B. Cao , K. M. Taddei , H. D. Zhou , X. Ke

The crystal structure and the magnetism of BaMn$_2$O$_3$ have been studied by thermodynamic and by diffraction techniques using large single crystals and powders. BaMn$_2$O$_3$ is a realization of a $S = 5/2$ spin ladder as the magnetic…

强关联电子 · 物理学 2015-05-20 M. Valldor , O. Heyer , A. C. Komarek , A. Senyshyn , M. Braden , T. Lorenz

By means of powder neutron diffraction we investigate changes in the magnetic structure of the coplanar non-collinear antiferromagnet Mn$_3$Ge caused by an application of hydrostatic pressure up to 5\phantom{ }GPa. At ambient conditions the…

The high-pressure synthesized quasi-one-dimensional compounds NaMn$_2$O$_4$ and Li$_{0.92}$Mn$_2$O$_4$ are both antiferromagnetic insulators, and here their atomic and magnetic structures were investigated using neutron powder diffraction.…

Co10Ge3O16 crystallizes in an intergrowth structure featuring alternating layers of spinel and rock salt. Variable-temperature powder synchrotron X-ray and neutron diffraction, magnetometry, and heat capacity experiments reveal a…

材料科学 · 物理学 2013-07-12 Phillip T. Barton , Ram Seshadri , Anna Llobet , Matthew R. Suchomel

The fascinating multiple magnetic states observed in the Ni-Mn-Sn based metamagnetic shape memory alloy are addressed through a combined muon spin relaxation (muSR) and neutron powder diffraction studies. The material used in the present…

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