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The eigenvalue of a Hamiltonian, $\mathcal{H}$, can be estimated through the phase estimation algorithm given the matrix exponential of the Hamiltonian, $exp(-i\mathcal{H})$. The difficulty of this exponentiation impedes the applications of…

量子物理 · 物理学 2018-11-01 Ammar Daskin , Sabre Kais

Path integral implementation of the quantum instanton approximation currently belongs among the most accurate methods for computing quantum rate constants and kinetic isotope effects, but its use has been limited due to the rather high…

化学物理 · 物理学 2017-05-10 Konstantin Karandashev , Jiri Vanicek

A new scheme to study the properties of finite nuclei is proposed based on the Dirac-Brueckner-Hartree-Fock (DBHF) approach starting from a bare nucleon-nucleon interaction. The relativistic structure of the nucleon self-energies in nuclear…

In this article, a fast algorithm based on time two-mesh (TT-M) finite element (FE) scheme, which aims at solving nonlinear problems quickly, is considered to numerically solve the nonlinear space fractional Allen-Cahn equations with smooth…

数值分析 · 数学 2019-01-30 Baoli Yin , Yang Liu , Hong Li , Siriguleng He

We examine the problem of particle acceleration at a relativistic shocks assuming pitch-angle scattering and using a Hartree-Fock method to approximate the associated eigenfunctions. This leads to a simple transcendental equation…

天体物理学 · 物理学 2009-11-13 Paul Dempsey , John G. Kirk

In this manuscript we propose and analyze an implicit two-point type method (or inertial method) for obtaining stable approximate solutions to linear ill-posed operator equations. The method is based on the iterated Tikhonov (iT) scheme. We…

数值分析 · 数学 2024-01-30 Joel C. Rabelo , Antonio Leitão , Alexandre L. Madureira

The multiconfiguration Dirac-Hartree-Fock (MCDHF) method has been employed to calculate atomic electric dipole moments (EDM) of 225^Ra, 199^Hg, and 171^Yb. For the calculations of the matrix elements we extended the relativistic atomic…

原子物理 · 物理学 2013-12-24 Laima Radziute , Gediminas Gaigalas , Per Jonsson , Jacek Biero

Time-dependent density functional theory (TDDFT) is a widely used method to investigate electron dynamics under various external perturbations such as laser fields. In this work, we present a novel approach to accelerate real time TDDFT…

材料科学 · 物理学 2024-07-29 Karan Shah , Attila Cangi

Inertial navigation computation is to acquire the attitude, velocity and position information of a moving body by integrating inertial measurements from gyroscopes and accelerometers. Over half a century has witnessed great efforts in…

机器人学 · 计算机科学 2021-09-21 Yuanxin Wu

Repeated computations on the same molecular system, but with different geometries, are often performed in quantum chemistry, for instance, in ab-initio molecular dynamics simulations or geometry optimizations. While many efficient…

化学物理 · 物理学 2020-12-02 E. Polack , A. Mikhalev , Geneviève Dusson , B. Stamm , F. Lipparini

We propose a high precision algorithm for solving the Gelfand-Levitan-Marchenko equation. The algorithm is based on the block version of the Toeplitz Inner-Bordering algorithm of Levinson's type. To approximate integrals, we use the…

数值分析 · 数学 2024-05-02 Sergey Medvedev , Irina Vaseva , Mikhail Fedoruk

Computing excited states of many-body quantum Hamiltonians is a fundamental challenge in computational physics and chemistry, with state-of-the-art methods broadly classified into variational (critical point search) and linear response…

化学物理 · 物理学 2026-02-27 Laura Grazioli , Yukuan Hu , Eric Cancès

We consider here variational solutions in the Hartree-Fock approximation upon breaking time reversal and axial symmetries. When decomposed on axial harmonic oscillator functions, the corresponding single particle triaxial eigenstates as…

核理论 · 物理学 2009-10-31 D. Samsoen , P. Quentin , J. Bartel

We consider the problem of estimating parameters in large-scale weakly nonlinear inverse problems for which the underlying governing equations is a linear, time-dependent, parabolic partial differential equation. A major challenge in…

数值分析 · 数学 2016-05-04 Tania Bakhos , Arvind K. Saibaba , Peter K. Kitanidis

Ultra-fast electronic phenomena originating from finite temperature, such as nonlinear optical excitation, can be simulated with high fidelity via real-time time dependent density functional theory (rt-TDDFT) calculations with hybrid…

材料科学 · 物理学 2025-01-07 Rongrong Liu , Zhuoqiang Guo , Qiuchen Sha , Tong Zhao , Haibo Li , Wei Hu , Lijun Liu , Guangming Tan , Weile Jia

The structure of approximate two electron wavefunction is deeply investigated, both theoretically and numerically, in the strong-field driven ionization dynamics. Theoretical analyses clarify that for two electron singlet systems, the…

原子物理 · 物理学 2014-11-13 Takeshi Sato , Kenichi L Ishikawa

We compute the leading-order inertial corrections to the instantaneous force acting on a rigid body moving with a time-dependent slip velocity in a linear flow field, assuming that the variation of the undisturbed flow at the body scale is…

流体动力学 · 物理学 2025-10-01 Fabien Candelier , Bernhard Mehlig , Jacques Magnaudet

We describe the inclusion of electrodynamic fields in Time-Dependent Density Functional Theory (TDDFT) by incorporating both the induced scalar and vector potentials within the time-dependent Kohn-Sham equation. The Hamiltonian is described…

化学物理 · 物理学 2020-07-01 Dor Gabay , Ali Yilmaz , Vitaliy Lomakin , Amir Boag , Amir Natan

We apply the approximate dynamics derived from the Gaussian time-dependent variational principle to the Hamiltonian $ \hat H= {1/2}(\hat p_x ^2+ \hat p_y ^2)+ {1/2}\hat x^2\hat y^2$, which is strongly chaotic in the classical limit. We are…

chao-dyn · 物理学 2016-08-31 Arjendu Pattanayak , William Schieve

Neural network force field (NNFF) is a method for performing regression on atomic structure-force relationships, bypassing expensive quantum mechanics calculation which prevents the execution of long ab-initio quality molecular dynamics…