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To exploit the high intensity of laser radiation, we propose to select frequencies at which single-photon absorption is of too low energy and two or more photons are needed to produce states of an atom that can undergo interatomic Coulombic…

原子与分子团簇 · 物理学 2012-01-04 Philipp V. Demekhin , Spas D. Stoychev , Alexander I. Kuleff , Lorenz S. Cederbaum

It is shown that well collimated mono-energetic ion beams with a large particle number can be generated in the hole-boring radiation pressure acceleration regime by using an elliptically polarized laser pulse with appropriate theoretically…

等离子体物理 · 物理学 2015-06-12 Dong Wu , C. Y. Zheng , C. T. Zhou , X. Q. Yan , M. Y. Yu , X. T. He

There are two types of two-photon transitions in molecular aggregates, that is, non-local excitations of two monomers and local double excitations to some higher excited intra-monomer electronic state. As a consequence of the inter-monomer…

量子物理 · 物理学 2015-06-04 Yun-an Yan , Oliver Kühn

We characterize the coherent dynamics of a two-level quantum emitter driven by a pair of symmetrically-detuned phase-locked pulses. The promise of dichromatic excitation is to spectrally isolate the excitation laser from the quantum…

To greatly enhance output of nuclear fusion produced neutrons in a laser-initiated Coulomb explosion of Deuterium clusters, we propose to accelerate the resulting ions by a quasi-$dc$ electrical pulse to the energies where the $D^+ + D$…

原子与分子团簇 · 物理学 2018-05-08 A. E. Kaplan

Reaching high cavity population with a coherent pump in the strong-coupling regime of a single-atom laser is impossible due to the photon blockade effect. In this work, we experimentally demonstrate that in a single-atom maser based on a…

量子物理 · 物理学 2023-04-05 A. A. Sokolova , D. A. Kalacheva , G. P. Fedorov , O. V. Astafiev

Laser excitation of nanometer-sized atomic and molecular clusters offers various opportunities to explore and control ultrafast many-particle dynamics. Whereas weak laser fields allow the analysis of photoionization, excited-state…

原子与分子团簇 · 物理学 2010-06-15 Th. Fennel , K. -H. Meiwes-Broer , J. Tiggesbaumker , P. -G. Reinhard , P. M. Dinh , E. Suraud

An ultrafast mechanism belonging to the family of interatomic Coulombic decay (ICD) phenomena is proposed. When two excited species are present, an ultrafast energy transfer can take place bringing one of them to its ground state and…

Effectiveness of using laser field to produce entanglement between two dipole-interacting identical two-level atoms is considered in detail. The entanglement is achieved by driving the system with a carefully designed laser pulse…

量子物理 · 物理学 2017-04-26 I. V. Bargatin , B. A. Grishanin , V. N. Zadkov

To greatly enhance output of fusion-produced neutrons in a laser-initiated Coulomb explosion of $D$ clusters, we propose to accelerate $D^+$ ions by an electrical pulse to the energies where the $D^+ + D$ collision cross-section is the…

原子与分子团簇 · 物理学 2019-02-20 A. E. Kaplan

We present a novel method to construct particle accelerators targeting light atoms and nuclei using high-power femtosecond laser pulses. Initially, we confine light atoms within the laser pulse envelope due to longitudinal polarization…

光学 · 物理学 2024-11-18 L. M. Kovachev , E. Iordanova , G. Yankov , I. P. Angelov

Optimal control techniques combined with femtosecond laser pulse shaping are applied to steer and enhance the strong-field induced emission of highly charged atomic ions from silver clusters embedded in helium nanodroplets. With light…

Calculating the energy absorption of atomic clusters as a function of the laser pulse length $T$ we find a maximum for a critical $T^*$. We show that $T^*$ can be linked to an optimal cluster radius $R^*$. The existence of this radius can…

原子与分子团簇 · 物理学 2009-11-07 Christian Siedschlag , Jan M. Rost

We study the dissociation of H$_2$$^+$ in uv laser pulses by solving the non-Born-Oppenheimer time-dependent Schr\"{o}dinger equation as a function of the photon energy $\omega$ of the pulse. Significant enhancements of the dissociation…

原子与分子团簇 · 物理学 2014-07-22 Kunlong Liu , Qianguang Li , Pengfei Lan , Peixiang Lu

The expansion of laser-irradiated clusters or nanodroplets depends strongly on the amount of energy delivered to the electrons and can be controlled by using appropriately shaped laser pulses. In this paper, a self-consistent kinetic model…

等离子体物理 · 物理学 2009-11-13 F. Peano , J. L. Martins , R. A. Fonseca , F. Peinetti , R. Mulas , G. Coppa , I. Last , J. Jortner , L. O. Silva

Intense few-to-sub-femtosecond soft x-ray pulses can produce neutral, two-site excited double-core-hole states by promoting two core electrons to the same unoccupied molecular orbital. We theoretically investigate double nitrogen K-edge…

化学物理 · 物理学 2023-06-28 Adam E. A. Fouda , Dimitris Koulentianos , Linda Young , Gilles Doumy , Phay J. Ho

An ensemble of Rubidum atoms can be excited with lasers such that it evolves into an entangled state with just one collective excitation within the Rydberg blockade radius. The decay of this state leads to the emission of a single,…

We propose a novel scheme for the population and depletion of nuclear isomers. The scheme combines the $\gamma$-photons with energies $\gtrsim 10$ keV emitted during the interaction of a contemporary high-intensity laser pulse with a plasma…

核理论 · 物理学 2025-07-25 C. -J. Yang , K. M. Spohr , M. Cernaianu , D. Doria , P. Ghenuche , V. Horny

The absorption-ablation-excitation mechanism in laser-cluster interactions is investigated by measuring Rayleigh scattering of aerosol clusters along with atomic emission from phase-selective laser-induced breakdown spectroscopy (PS-LIBS).…

原子与分子团簇 · 物理学 2015-06-23 Yihua Ren , Shuiqing Li , Yiyang Zhang , Stephen D. Tse , Marshall B. Long

We show that induced dipole-dipole interactions allow for photon blockade in subwavelength ensembles of two-level, ground-state neutral atoms. Our protocol relies on the energy shift of the single-excitation, superradiant state of $N$…

量子气体 · 物理学 2020-08-19 A. Cidrim , T. S. do Espirito Santo , J. Schachenmayer , R. Kaiser , R. Bachelard
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