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Infrared spectroscopy in the spectral fingerprint region from 6-12 um accesses the largest molecular absorption cross-sections, permitting sensitive, quantitative and species-specific measurements. Here, we show how dual-comb…

光学 · 物理学 2023-06-26 O. Kara , L. Maidment , T. Gardiner , P. G. Schunemann , D. T. Reid

We demonstrate dual-comb spectroscopy based on difference frequency generation of frequency-agile near-infrared frequency combs, produced with the help of electro-optic modulators. The combs have a remarkably flat intensity distribution and…

Broadband and high-resolution spectroscopy in the visible and ultraviolet is central to advances in multiple fields, including fundamental quantum physics, biology, atmospheric science and astronomy. Traditionally, these measurements are…

Dual-comb spectroscopy has emerged as an indispensable analytical technique in applications that require high resolution and broadband coverage within short acquisition times. Its experimental realization, however, remains hampered by…

仪器与探测器 · 物理学 2019-12-02 Łukasz A. Sterczewski , Aleksandra Przewłoka , Wawrzyniec Kaszub , Jarosław Sotor

Ultrabroadband electro-optic sampling with few-cycle optical pulses is known to be an extremely sensitive technique to detect electric field amplitudes. By combining this method with dual-comb spectroscopy and with a new class of ultrafast…

Dual-comb spectroscopy allows for the rapid, multiplexed acquisition of high-resolution spectra without the need for moving parts or low-resolution dispersive optics. This method of broadband spectroscopy is most often accomplished via…

With the advent of laser frequency combs, coherent light sources that offer equally-spaced sharp lines over a broad spectral bandwidth have become available. One decade after revolutionizing optical frequency metrology, frequency combs hold…

Historically, there has been a trade-off in spectroscopic measurements between high spectral resolution, broadband coverage, and acquisition time. Optical frequency combs, initially envisioned for precision spectroscopy of the hydrogen atom…

光学 · 物理学 2020-06-04 A. V. Muraviev , D. Konnov , K. L. Vodopyanov

Time-resolved near-infrared absorption spectroscopy of single non-repeatable transient events is performed at high spectral resolution with a dual-comb interferometer using a continuous-wave laser followed by a single electro-optic…

A fieldable dual-comb spectrometer is described based on a "bootstrapped" frequency referencing scheme in which short-term optical phase coherence between combs is attained by referencing each to a free-running diode laser, whilst high…

We propose a new approach to near-infrared molecular spectroscopy, harnessing advanced concepts of optical telecommunications and supercontinuum photonics. We generate, without mode-locked lasers, two frequency combs of slightly different…

We present quasi-real-time dual-comb spectroscopy (DCS) using two Yb:fiber combs with ~750 MHz repetition rates. A computational coherent averaging technique is employed to correct timing and phase fluctuations of the measured dual-comb…

In this paper, we introduce an all-fibered dual-comb spectrometer based on a new design of highly nonlinear fiber to efficiently convert frequency combs from 1.55 micron to 2 micron We show that our spectrometer can be used to measure…

We demonstrate the use of dual-comb spectroscopy for isotope ratio measurements. We show that the analysis spectral range of a free-running near-infrared dual-comb spectrometer can be extended to the mid-infrared by difference frequency…

仪器与探测器 · 物理学 2022-05-10 Alexandre Parriaux , Kamal Hammani , Christophe Thomazo , Olivier Musset , Guy Millot

We have carried out dual-comb spectroscopy and observed in a simultaneous acquisition a 140-THz-wide spectrum from 1.0 to 1.9 {\mu}m using two fiber-based frequency combs phase-locked to each other. This ultra-broad wavelength bandwidth is…

The femtosecond laser frequency comb has enabled the 21st century revolution in optical synthesis and metrology. A particularly compelling technique that relies on the broadband coherence of two laser frequency combs is dual-comb…

光学 · 物理学 2023-07-19 Vicente Duran , Santiago Tainta , Victor Torres-Company

We radically simplify coherently averaged dual-comb spectroscopy by introducing a real-time self-correction system: a radio frequency system-on-chip computes each incoming dual-comb interferogram's phase, frequency, and arrival time;…

Dual-comb spectroscopy in the ultraviolet (UV) and visible would enable broad bandwidth electronic spectroscopy with unprecedented frequency resolution. However, there are significant challenges in generation, detection and processing of…

Dual-comb spectroscopy utilizes two sets of comb lines with slightly different comb-tooth-spacings, and optical spectral information is acquired by measuring the radio-frequency beat notes between the sets of comb lines. It holds the…

光学 · 物理学 2016-09-13 Xin Zhao , Guoqing Hu , Bofeng Zhao , Cui Li , Yingling Pan , Ya Liu , Takeshi Yasui , Zheng Zheng

Dual-comb spectroscopy has been proven a powerful tool in molecular characterization, which remains challenging to implement in the mid-infrared region due to difficulties in the realization of two mutually locked comb sources and efficient…

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