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Mid-infrared optical frequency combs are of significant interest for molecular spectroscopy due to the large absorption of molecular vibrational modes on one hand, and the ability to implement superior comb-based spectroscopic modalities…

We demonstrate an octave-spanning frequency comb with a spectrum covering wavelengths from 1,540 nm up to 3,200 nm. The supercontinuum is generated by pumping a 1-cm long dispersion engineered silicon wire waveguide by 70 fs pulses with an…

We demonstrate efficient generation of mid-infrared frequency combs based on continuous-wave-seeded femtosecond optical parametric generation in nonlinear waveguides. Conversion of the near-infrared pump to signal and idler light takes…

光学 · 物理学 2021-09-01 Mikhail Roiz , Jui-Yu Lai , Juho Karhu , Markku Vainio

We describe a coherent mid-infrared continuum source with 700 cm-1 usable bandwidth, readily tuned within 600 - 2500 cm-1 (4 - 17 \mum) and thus covering much of the infrared "fingerprint" molecular vibration region. It is based on…

量子物理 · 物理学 2015-06-04 Fritz Keilmann , Sergiu Amarie

We experimentally demonstrate a simple configuration for mid-infrared (MIR) frequency comb generation in quasi-phase-matched lithium niobate waveguides using the cascaded-$\chi^{(2)}$ nonlinearity. With nanojoule-scale pulses from an…

Optical frequency combs represent a revolutionary technology for high precision spectroscopy due to their narrow linewidths and precise frequency spacing. Generation of such combs in the mid-infrared (IR) spectral region (2-20 um) is of…

We present a simple method for fully-stabilized mid-infrared optical frequency comb generation based on single-pass femtosecond optical parametric generation that is seeded by a continuous-wave laser. We have implemented the method in a…

光学 · 物理学 2024-06-12 Mikhail Roiz , Krishna Kumar , Juho Karhu , Markku Vainio

The potential of frequency comb spectroscopy has aroused great interest in generating mid-infrared frequency combs in the integrated photonic setting. However, despite remarkable progress in microresonators and quantum cascade lasers, the…

Nanophotonic waveguides with sub-wavelength mode confinement and engineered dispersion profiles are an excellent platform for application-tailored nonlinear optical interactions at low pulse energies. Here, we present fully air clad…

Mid-infrared (mid-IR) spectroscopy provides a way to study structures and dynamics of complicated molecules in condensed phases. Therefore, developing compact and broadband mid-IR spectrometer has been a long-standing challenge. Here, we…

光学 · 物理学 2020-01-16 Noh Soo Han , JunWoo Kim , Tai Hyun Yoon , Minhaeng Cho

A fully stabilized mid-infrared optical frequency comb spanning from 2.9 to 3.4 um is described. The comb is based on half-harmonic generation in a femtosecond optical parametric oscillator, which transfers the high phase coherence of a…

光学 · 物理学 2017-04-05 Markku Vainio , Juho Karhu

We present numerical results of supercontinuum (SC) generation in the mid-IR spectral region, specifically addressing the molecular fingerprint window ranging from 2.5 to 25 um. By solving the Generalized Nonlinear Schr\"odinger Equation…

光学 · 物理学 2016-05-11 Santiago M. Hernandez , Pablo I. Fierens , Juan Bonetti , Diego F. Grosz

Mid-infrared femtosecond optical frequency combs were produced by difference frequency generation of the spectral components of a near-infrared comb in a 3-mm-long MgO:PPLN crystal. We observe strong pump depletion and 9.3 dB parametric…

High resolution and fast detection of molecular vibrational absorption is important for organic synthesis, pharmaceutical process and environmental monitoring, and is enabled by mid-infrared (mid-IR) laser frequency combs via dual-comb…

Mid-infrared frequency comb spectroscopy enables measurement of molecular at megahertz spectral resolution, sub-hertz frequency accuracy and microsecond acquisition speed. However, the widespread adoption of this technique has been hindered…

We demonstrate the generation of a low-noise, octave-spanning mid-infrared supercontinuum from 1700 to 4800 nm by injecting femtosecond pulses into the normal dispersion regime of a multimode step-index chalcogenide fiber with 100 $\mu$m…

光学 · 物理学 2020-06-24 Zahra Eslami , Piotr Ryczkowski , Lauri Salmela , Goëry Genty

Infrared spectroscopy is a powerful tool for basic and applied science. The molecular spectral fingerprints in the 3 um to 20 um region provide a means to uniquely identify molecular structure for fundamental spectroscopy, atmospheric…

The mid-infrared (mid-IR) regime (typically the wavelength regime of $\lambda \sim 2.5-20 \ \mathrm{\mu m}$) is an important spectral range for spectroscopy as many molecules have their fundamental rotational-vibrational absorption in this…

For the growing demand of frequency combs in mid-infrared (mid-IR), known as the "molecular fingerprint" region of the spectrum [1], down conversion of near-IR frequency combs through half- harmonic generation offers numerous benefits…

光学 · 物理学 2015-10-14 Alireza Marandi , Kirk A. Ingold , Marc Jankowski , Robert L. Byer

Supercontinuum generation (SCG) is an important nonlinear optical process enabling broadband light sources for many applications, for which silicon nitride(Si3N4) has emerged as a leading on-chip platform.To achieve suitable group velocity…

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