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Using ultrafast optical pump-probe spectroscopy, we study the relaxation dynamics of hot optical phonons in few-layer and multi-layer graphene films grown by epitaxy on silicon carbide substrates and by chemical vapor deposition on nickel…

The energy relaxation of carriers in reduced graphene oxide thin films is studied using optical pump-probe spectroscopy with two probes of different colors. We measure the time difference between peaks of the carrier density at each probing…

介观与纳米尺度物理 · 物理学 2015-05-27 Brian A. Ruzicka , Nardeep Kumar , Shuai Wang , Kian Ping Loh , Hui Zhao

We report ultrafast response of femtosecond photoexcited carriers in single layer reduced graphene oxide flakes suspended in water as well as few layer thick film deposited on indium tin oxide coated glass plate using pump-probe…

材料科学 · 物理学 2011-06-30 Sunil Kumar , N. Kamaraju , K. S. Vasu , A. K. Sood

We report the ultrafast dynamics of the 47.4 THz coherent phonons of graphite interacting with a photoinduced non-equilibrium electron-hole plasma. Unlike conventional materials, upon photoexcitation the phonon frequency of graphite…

其他凝聚态物理 · 物理学 2008-03-13 Kunie Ishioka , Muneaki Hase , Masahiro Kitajima , Ludger Wirtz , Angel Rubio , Hrvoje Petek

We study, by means of a Monte Carlo simulator, the hot phonon effect on the relaxation dynamics in photoexcited graphene and its quantitative impact as compared to considering an equilibrium phonon distribution. Our multi-particle approach…

介观与纳米尺度物理 · 物理学 2016-02-02 José M. Iglesias , María J. Martín , Elena Pascual , Raúl Rengel

Radio-frequency compressed ultrafast electron diffraction has been used to probe the coherent and incoherent coupling of impulsive electronic excitation at 1.55 eV (800 nm) to optical and acoustic phonon modes directly from the perspective…

Ultrafast optical pump-probe spectroscopy is used to track carrier dynamics in the large magnetoresistance material WTe$_{2}$. Our experiments reveal a fast relaxation process occurring on a sub-picosecond time scale that is caused by…

Using ultrafast optical pump-probe spectroscopy, we have measured carrier relaxation times in epitaxial graphene layers grown on SiC wafers. We find two distinct time scales associated with the relaxation of nonequilibrium photogenerated…

Ultrafast electron-phonon relaxation dynamics in graphene hides many distinct phenomena, such as hot phonon generation, dynamical Kohn anomalies, and phonon decoupling, yet still remains largely unexplored. Here, we unravel intricate…

材料科学 · 物理学 2023-09-19 Nina Girotto , Dino Novko

Using optical-pump terahertz-probe spectroscopy, we study the relaxation dynamics of photoexcited carriers in graphene at different temperatures. We find that at lower temperatures the tail of the relaxation transients as measured by the…

介观与纳米尺度物理 · 物理学 2015-05-30 Jared H. Strait , Haining Wang , Shriram Shivaraman , Virgil B. Shields , Michael G. Spencer , Farhan Rana

The broadband and ultrafast photoresponse of graphene has been extensively studied in recent years, although the photoexcited carrier dynamics is still far from being completely understood. Different experimental approaches imply either one…

介观与纳米尺度物理 · 物理学 2017-08-22 Sergey Menabde , Hyunwoo Cho , Namkyoo Park

The dynamics of photocarriers in reduced graphene oxide thin films is studied by using ultrafast pump-probe spectroscopy. Time dependent differential transmissions are measured with sample temperatures ranging from 9 to 300 K. At each…

介观与纳米尺度物理 · 物理学 2015-05-18 Brian A. Ruzicka , Lalani K. Werake , Hui Zhao , Shuai Wang , Kian Ping Loh

Time-domain femtosecond laser spectroscopic measurements of the ultrafast lattice dynamics in 2H-MoTe2 bulk crystals were carried out to understand the carrier-phonon interactions that govern electronic transport properties. An unusually…

Fast carrier cooling is important for high power graphene based devices. Strongly Coupled Optical Phonons (SCOPs) play a major role in the relaxation of photoexcited carriers in graphene. Heterostructures of graphene and hexagonal boron…

介观与纳米尺度物理 · 物理学 2017-04-21 Dheeraj Golla , Alexandra Brasington , Brian J. LeRoy , Arvinder Sandhu

For most optoelectronic applications of graphene a thorough understanding of the processes that govern energy relaxation of photoexcited carriers is essential. The ultrafast energy relaxation in graphene occurs through two competing…

Understanding and controlling hot-carrier relaxation in graphene is crucial for advancing ultrafast optoelectronic and terahertz technologies. Here, we investigate carrier cooling dynamics in monolayer and bilayer graphene using…

介观与纳米尺度物理 · 物理学 2026-05-21 Sachin Sharm , Elliott Walker , Rachael Myers-Ward , Jenifer Hajzus , Yijing Liu , Paola Barbara , Ioannis Chatzakis

We perform a femtosecond-THz optical pump-probe spectroscopy to investigate the cooling dynamics of hot carriers in quasi-free standing bilayer epitaxial graphene. We observed longer decay time constants, in the range of 2.6 to 6.4 ps,…

介观与纳米尺度物理 · 物理学 2023-02-03 Sachin Sharma , Rachael L. Myers-Ward , David Kurt Gaskill , Ioannis Chatzakis

The ultrafast relaxation and recombination dynamics of photogenerated electrons and holes in epitaxial graphene are studied using optical-pump Terahertz-probe spectroscopy. The conductivity in graphene at Terahertz frequencies depends on…

介观与纳米尺度物理 · 物理学 2015-05-13 Paul A. George , Jared Strait , Jahan Dawlaty , Shriram Shivaraman , Mvs Chandrashekhar , Farhan Rana , Michael G. Spencer

We investigate carrier and collective mode dynamics in 2H-NbSe$_2$ using time-resolved optical pump-probe spectroscopy and compare the results with first-principle calculations. Broadband ultrafast reflectivity studies of 2H-NbSe$_2$ in a…

强关联电子 · 物理学 2020-12-30 A. Anikin , R. D. Schaller , G. P. Wiederrecht , E. R. Margine , I. I. Mazin , G. Karapetrov

The transient response of Ba(Fe(1-x)Co(x))2As2, x=0.08 was studied by pump-probe optical reflectivity. After ultrafast photoexcitation, hot electrons were found to relax with two different characteristic times, indicating the presence of…

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