相关论文: Introduction to attosecond time-delays in photoion…
We investigate dynamics of atomic and molecular systems exposed to intense, shaped chaotic fields and a weak femtosecond laser pulse theoretically. As a prototype example, the photoionization of a hydrogen atom is considered in detail. The…
The initial insight into time delay in Mn photoionization in the region of the $3p \to 3d$ giant autoionization resonance is gained in the framework of the "spin-polarized" random phase approximation with exchange. The dramatic effect of…
The double-slit interference in single-photon ionization of the diatomic molecular ion $\mathrm{H}_2^+$ is theoretically studied beyond the dipole approximation. Via simulating and comparing the interactions of the prealigned…
A novel and universal interference structure is found in the photoelectron momentum distribution of atoms in intense infrared laser field. Theoretical analysis shows that this structure can be attributed to a new form of…
We present experimental measurements and theoretical calculations of photoionization time delays from the $3s$ and $3p$ shells in Ar in the photon energy range of 32-42 eV. The experimental measurements are performed by interferometry using…
We investigate theoretically electron dynamics under a VUV attosecond pulse train which has a controlled phase delay with respect to an additional strong infrared laser field. Using the strong field approximation and the fact that the…
First time-resolved photoemission experiments employing attosecond streaking of electrons emitted by an XUV pump pulse and probed by a few-cycle NIR pulse found a time delay of about 100 attoseconds between photoelectrons from the…
Attosecond angular streaking measurements have revealed deep insights into the timing of tunnel ionization processes of atoms in intense laser fields. So far experiments of this type have been performed only with a cold-target recoil-ion…
The photoionization of the CO molecule from the C$-1s$ orbital does not obey the Franck-Condon approximation, as a consequence of the nuclear recoil that accompanies the direct emission and intra-molecular scattering of the photoelectron.…
We use the soft photon approximation to extract the Wigner time delay from atomic two-color photoionization experiments. Unlike the strong field approximation, the present method does not require introduction of the Coulomb-laser coupling…
We propose a protocol to probe the ultrafast evolution and dephasing of coherent electronic excitation in molecules in the time domain by the intrinsic streaking field generated by the molecule itself. Coherent electronic motion in the…
In molecular systems, the ultrafast motion of electrons initiates the process of chemical change. Tracking this electronic motion across molecules requires coupling attosecond time resolution to atomic-scale spatial sensitivity. In this…
The birth of attosecond light sources is expected to inspire a breakthrough in ultrafast optics, which may extend human real-time measurement and control techniques into atomic-scale electronic dynamics. For applications, it is essential to…
Light-phase-sensitive techniques, such as coherent multidimensional spectroscopy, are well-established in a broad spectral range, already spanning from radio-frequencies in nuclear magnetic resonance spectroscopy to visible and ultraviolet…
We investigate the laser-assisted single XUV photon double ionization of ground state helium. By solving full six-dimensional time-dependent schr{\"o}dinger equation, we study the correlation and angular distribution. The discussion in…
The dissociation dynamics of diatomic molecules interacting with (near) optical laser pulses of different duration is investigated by an elaborate discussion of the electric field of the laser and by a direct solution of the time-dependent…
We theoretically investigate the scattering of an attosecond electron wave packet launched by an attosecond pulse under the influence of an infrared laser field. As the electron scatters inside a spatially extended system, the dressing…
The electron motion in atoms and molecules is at the heart of all phenomena in nature that occur outside the nucleus. Recently, ultrafast electron and X-ray imaging tools have been developed to image the ultrafast dynamics of matter in real…
We introduce and experimentally demonstrate a method, where the two intrinsic time scales of a molecule, the slow nuclear motion and the fast electronic motion, are simultaneously measured in a photo-electron photo-ion coincidence…
We discuss the concept of an all-optical and ionizing matter-wave interferometer in the time domain. The proposed setup aims at testing the wave nature of highly massive clusters and molecules, and it will enable new precision experiments…