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The electrical control of magnons opens up new ways to transport and process information for logic devices. In magnetoelectrical multiferroics, the Dzyaloshinskii-Moriya (DM) interaction directly allow for such a control and, hence, is of…

材料科学 · 物理学 2023-07-19 Sebastian Meyer , Bin Xu , Matthieu Verstraete , Laurent Bellaiche , Bertrand Dupé

Low-energy magnon excitations in multiferroic BiFeO$_3$ were measured in detail as a function of temperature around several Brillouin zone centers by inelastic neutron scattering experiments on single crystals. Unique features around 1 meV…

First-principles calculations, in combination with the four-state energy mapping method, are performed to extract the magnetic interaction parameters of multiferroic BiFeO$_3$. Such parameters include the symmetric exchange (SE) couplings…

材料科学 · 物理学 2019-03-20 Changsong Xu , Bin Xu , Bertrand Dupé , L. Bellaiche

We present a terahertz spectroscopic study of magnetic excitations in ferroelectric antiferromagnet BiFeO3. We interpret the observed spectrum of long-wavelength magnetic resonance modes in terms of the normal modes of the material's…

材料科学 · 物理学 2015-05-27 D. Talbayev , S. A. Trugman , Seongsu Lee , Hee Taek Yi , S. -W. Cheong , A. J. Taylor

High resolution inelastic neutron scattering reveals that the elementary magnetic excitations in multiferroic MnWO4 consist of low energy dispersive electromagnons in addition to the well-known spin-wave excitations. The latter can well be…

强关联电子 · 物理学 2016-06-30 Y. Xiao , C. M. N. Kumar , S. Nandi , Y. Su , W. T. Jin , Z. Fu , E. Faulhaber , A. Schneidewind , Th. Brueckel

Magnetic, dielectric and calorimetric studies on 0.9BiFeO3-0.1BaTiO3 indicate strong magnetoelectric coupling. XRD studies reveal a very remarkable change in the rhombohedral distortion angle and a significant shift in the atomic positions…

材料科学 · 物理学 2009-11-13 Anar Singh , Vibhav Pandey , R. K. Kotnala , Dhananjai Pandey

We report local probe investigations of the magnetic interaction between BiFeO3 films and a ferromagnetic Co0.9Fe0.1 layer. Within the constraints of intralayer exchange coupling in the Co0.9Fe0.1, the multiferroic imprint in the…

The link between the crystal distortions of the perovskite structure and the magnetic exchange interaction, the single-ion anisotropy (SIA) and the Dzyaloshinsky-Moriya (DM) interaction are investigated by means of density-functional…

材料科学 · 物理学 2015-06-05 Carlo Weingart , Nicola Spaldin , Eric Bousquet

We present data on the magnetic and magneto-elastic coupling in the hexagonal multiferroic manganite LuMnO3 from inelastic neutron scattering, magnetization and thermal expansion measurements. We measured the magnon dispersion along the…

强关联电子 · 物理学 2010-12-01 H. J. Lewtas , A. T. Boothroyd , M. Rotter , D. Prabhakaran , H. Mueller , M. D. Le , B. Roessli , J. Gavilano , P. Bourges

Ab initio calculations show that the Dzyaloshinskii-Moriya interaction(DMI)and net magnetization per unit cell in BiFeO3 are reduced when U is increasing from 0 to 2.9 eV, and independent of $J$. Interestingly, the DMI is even destroyed as…

材料科学 · 物理学 2012-12-20 Hong-Jian Feng

Magnetic order and excitations in multiferroic DyMnO3 were studied by neutron scattering experiments using a single crystal prepared with enriched 162Dy isotope. The ordering of Mn moments exhibits pronounced hysteresis arising from the…

强关联电子 · 物理学 2015-06-23 T. Finger , K. Binder , Y. Sidis , A. Maljuk , D. N. Argyriou , M. Braden

We performed inelastic neutron scattering measurements on single crystals of NdFe$_{3}$($^{11}$BO$_{3}$)$_{4}$ to explore the magnetic excitations, to establish the underlying Hamiltonian, and to reveal the detailed nature of hybridization…

强关联电子 · 物理学 2015-07-23 S. Hayashida , M. Soda , S. Itoh , T. Yokoo , K. Ohgushi , D. Kawana , H. M. Rønnow , T. Masuda

We apply degenerate perturbation theory to investigate the effects of magnetic anisotropy in the magnetic molecule V15. Magnetic anisotropy is introduced via Dzyaloshinskii-Moriya (DM) interaction in the full Hilbert space of the system.…

介观与纳米尺度物理 · 物理学 2009-11-07 N. P. Konstantinidis , D. Coffey

We have identified three of the four magnetoelectric modes of multiferroic BiFeO$_3$ measured using THz spectroscopy. Excellent agreement with the observed peaks is obtained by including the effects of easy-axis anisotropy along the…

强关联电子 · 物理学 2015-06-11 Randy S. Fishman , Nobuo Furukawa , Jason T. Haraldsen , Masaaki Matsuda , Shin Miyahara

The spectroscopic modes of multiferroic BiFeO$_3$ provide detailed information about the very small anisotropy and Dzyaloshinskii-Moriya (DM) interactions responsible for the long-wavelength, distorted cycloid below $\TN = 640$ K. A…

材料科学 · 物理学 2015-06-15 Randy S. Fishman

In this article we review and discuss a mechanism for coupling between electric polarization and magnetization that can ultimately lead to electric-field switchable magnetization. The basic idea is that a ferroelectric distortion in an…

材料科学 · 物理学 2009-11-13 Claude Ederer , Craig J. Fennie

We analyze the coupling between the ferroelectric and magnetic order parameters in the magnetoelectric multiferroic BiFeO_3 using density functional theory within the local spin density approximation and the LSDA+U method. We show that weak…

材料科学 · 物理学 2007-05-23 Claude Ederer , Nicola A. Spaldin

A microscopic model for the room-temperature multiferroic BiFeO$_3$ that includes two Dzyaloshinskii-Moriya interactions and single-ion anisotropy along the ferroelectric polarization predicts both the zero-field spectroscopic modes as well…

We present a first-principles scheme for computing the magnetoelectric response of multiferroics. We apply our method to BiFeO3 (BFO) and related compounds in which Fe is substituted by other magnetic species. We show that under certain…

材料科学 · 物理学 2012-04-17 Jacek C. Wojdel , Jorge Iniguez

We investigated the static and dynamic magnetic properties of the polar ferrimagnet Mn$_2$Mo$_3$O$_8$ in three magnetically ordered phases via magnetization, magnetic torque, and THz absorption spectroscopy measurements. The observed…

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