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We demonstrate that the dispersion of surface plasmon polaritons in a periodically perforated gold film can be efficiently manipulated by femtosecond laser pulses with the wavelengths far from the intrinsic resonances of gold. Using a time-…

In this work, we present a novel technique to directly measure the phase shift of the optical signal scattered by single plasmonic nanoparticles in a diffraction-limited laser focus. We accomplish this by equipping an inverted confocal…

Femtosecond point-projection microscopy (fs-PPM) is an electron microscopy technique that possesses a combination of high spatio-temporal resolution and sensitivity to local electric fields. This allows it to visualize ultrafast charge…

The combination of nanodiamonds with plasmonic metal particles is being explored for synergic effects that can enhance biosensing and antibacterial treatments, energy harvesting, photocatalysis, and quantum centres. Here we systematically…

Single nanoparticle tracking using optical microscopy is a powerful technique with many applications in biology, chemistry and material sciences. Despite significant advances, localising objects with nanometric position accuracy in a…

Nanoscale phase-control is one of the most powerful approaches to specifically tailor electrical fields in modern nanophotonics. Especially the precise sub-wavelength assembly of many individual nano-building-blocks has given rise to…

光学 · 物理学 2021-05-26 Lisa Saemisch , Niek F. van Hulst , Matz Liebel

Femtosecond electron microscopy produces real-space images of matter in a series of ultrafast snapshots. Pulses of electrons self-disperse under space-charge broadening, so without compression, the ideal operation mode is a single electron…

加速器物理 · 物理学 2016-04-21 A. R. Bainbridge , C. W. Barlow-Myers , W. A. Bryan

Specialized applications of nanoparticles often call for particular, well-characterized particle size distributions in solution. But, this property can prove difficult to measure. High-throughput methods, such as dynamic light scattering,…

介观与纳米尺度物理 · 物理学 2021-09-24 Luke Melo , Angus Hui , Matt Kowal , Eric Boateng , Zahra Poursorkh , Edène Rocheron , Jake Wong , Ashton Christy , Edward Grant

Pan-microbial inactivation technologies that do not require high temperatures, reactive chemical compounds, or UV radiation could address gaps in current infection control strategies and provide efficient sterilization of biologics in the…

Understanding light-matter interaction at the nanoscale requires probing the optical properties of matter at the individual nano-absorber level. To this end, we have developed a nanomechanical photothermal sensing platform that can be used…

光学 · 物理学 2024-06-07 Kostas Kanellopulos , Robert G. West , Silvan Schmid

Surface Plasmon Resonance sensors are a well-established class of sensors which includes a very large variety of materials and detection schemes. However, the development of portable devices is still challenging as due to the intrinsic…

Current advances in ultrafast electron microscopy make it possible to combine optical pumping of a nanostructure and electron beam probing with sub{\aa}ngstrom and femtosecond spatiotemporal resolution. We present a theory predicting that…

We measure the transient absorption of single gold particles with a common-path interferometer. The prompt electronic part of the signal provides high-contrast images for diameters as small as 10 nm. Mechanical vibrations of single…

其他凝聚态物理 · 物理学 2007-05-23 Meindert A. van Dijk , Markus Lippitz , Michel Orrit

Watching the motion of electrons on their natural nanometre length- and femtosecond time scales is a fundamental goal and an open challenge of contemporary ultrafast science. Optical techniques and electron microscopy currently mostly…

光学 · 物理学 2018-01-23 Jan Vogelsang , Germann Hergert , Dong Wang , Petra Groß , Christoph Lienau

The photothermal heterodyne imaging technique enabled studies of individual weakly absorbing nano-objects in various environments. It uses a photo-induced change in the refractive index of the environment. Taking advantage of the dramatic…

Current optical detection schemes for single molecules require light absorption, either to produce fluorescence or direct absorption signals. This severely limits the range of molecules that can be detected, because most molecules are…

化学物理 · 物理学 2012-07-06 Peter Zijlstra , Pedro M. R. Paulo , Michel Orrit

Efficiency is a critical factor limiting the applications of nonlinear plasmonic devices. We show by theory and experiments that high efficiency four-wave mixing (FWM) is achieved in nanometer size plasmonic hotspots, which open up…

光学 · 物理学 2020-06-16 Hui Yi , Xiaodan Wang , Tian Yang

Plasmonic metal nanostructures are an integral part of nanophotonic device applications owing to their ability to generate strong localized electromagnetic fields when illuminated from the far-field. These nanostructures can be prepared in…

介观与纳米尺度物理 · 物理学 2018-02-05 Sunil Kumar , A. K. Sood

We report the investigation of the generation and detection of GHz coherent acoustic phonons in plasmonic gold nanoparticles superlattices (NPS). The experiments have been performed from an optical femtosecond pump-probe scheme across the…

材料科学 · 物理学 2015-12-09 P. Ruello , A. Ayouch , G. Vaudel , T. Pezeril , N. Delorme , S. Sato , K. Kimura , V. Gusev

We use frequency entangled photons, generated via spontaneous parametric down conversion, to measure the broadband spectral response of an array of gold nanoparticles exhibiting Fano-type plasmon resonance. Refractive index sensing of a…

量子物理 · 物理学 2014-03-27 Dmitry A. Kalashnikov , Zhenying Pan , Arseniy I. Kuznetsov , Leonid A. Krivitsky
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