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相关论文: Mechanism of enhanced optical second-harmonic gene…

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The synergy of strong spin-orbit coupling and electron-electron interactions gives rise to unconventional topological states, such as topological Mott insulator, Weyl semimetal, and quantum spin liquid. In this study, we have grown single…

强关联电子 · 物理学 2024-07-18 Harish Kumar , M. Köpf , P. Telang , N. Bura , A. Jesche , P. Gegenwart , C. A. Kuntscher

Ir-based materials have drawn much attention due to the observation of insulating phase believed to be driven by spin-orbit coupling while Ir 5$d$ states are expected to be weakly correlated due to their large orbital extensions. IrO$_2$, a…

Electrons in the pyrochore iridates experience a large interaction energy in addition to a strong spin-orbit interaction. Both features make the iridates promising for realizing novel states such as the Topological Mott Insulator. The…

强关联电子 · 物理学 2017-09-21 Tian Liang , Timothy H. Hsieh , Jun J. Ishikawa , Satoru Nakatsuji , Liang Fu , N. P. Ong

Material systems with lone-pair electrons have long been a treasure trove in the search for large second harmonic generation effects. Revealing the origin of second harmonic generation in nonlinear optical materials can provide theoretical…

材料科学 · 物理学 2025-05-13 Fuming Li , Shilie Pan , Zhihua Yang

The 5d-transition metal pyrochlore oxide Cd2Re2O7, which was recently suggested to be a prototype of the spin-orbit-coupled metal [Phys. Rev. Lett. 115, 026401 (2015)], exhibits an inversion-symmetry breaking (ISB) transition at 200 K and a…

Second harmonic generation is a powerful tool directly connected to the symmetry of materials. Phase transitions, lattice rotations or electromagnetic coupling in multiferroic compounds can be revealed by using second harmonic…

光学 · 物理学 2010-01-11 Pablo Molina , Mariola O Ramirez , Basilio J. Garcia , Luisa E. Bausa

We report magnetic, transport, neutron diffraction, and muon spin rotation data showing that Pb$_2$CoOsO$_6$, a newly synthesized metallic double-perovskite with a centrosymmetric space group at room temperature, exhibits a continuous…

Optical conductivity spectra of cubic pyrochlore $Y_{2-x} Bi_x Ru_2 O_7$ (0.0$\leq ${\it x}$\leq $2.0) compounds are investigated. As a metal-insulator transition (MIT) occurs around {\it x}$=$0.8, large spectral changes are observed. With…

强关联电子 · 物理学 2009-11-11 J. S. Lee , S. J. Moon , T. W. Noh , T. Takeda , R. Kanno , S. Yoshii , M. Sato

We present a model that explains two phenomena, recently observed in high-mobility Si-MOS structures: (i) the strong enhancement of metallic conduction at low temperatures, T<2 K, and (ii) the occurrence of the metal-insulator transition in…

强关联电子 · 物理学 2009-10-30 V. M. Pudalov

Polar metals and noncentrosymmetric superconductors are exceptionally rare, yet their broken inversion symmetry can give rise to emergent electronic phenomena including mixed singlet-triplet superconducting pairing. As only a few such…

We report on the epitaxial growth, structural and electrical properties of metallic pyrochlore bismuth ruthenate heterostructures grown along both the [001] and [111] directions. Ordered pyrochlore thin films were obtained with highly…

The pyrochlore oxide Pb2Re2O7-{\delta} (PRO) is a candidate spin-orbit-coupled metal (SOCM) that exhibits a structural phase transition with inversion symmetry breaking. In this study, we report the results of detailed X-ray diffraction…

Second harmonic generation (SHG) on the pyrochlore metal Cd2Re2O7 indicates the presence of three order parameters setting in below an inversion breaking transition. Here, we explore a possible structural explanation and relate it not only…

强关联电子 · 物理学 2020-01-15 M. R. Norman

Geometrical frustration and spin-orbit coupling effect together play vital role to influence properties in pyrochlore based iridium oxides. Here we have investigated detailed structural, magnetic, thermodynamic and transport properties of…

强关联电子 · 物理学 2017-02-06 Harish Kumar , A. K. Pramanik

The $f$-$d$ magnetic exchange interaction is considered to be a key ingredient for many exotic topological phases in pyrochlore iridates. Here, we have investigated the evolution of structural, magnetic and electronic properties in doped…

强关联电子 · 物理学 2020-02-07 Harish Kumar , K. C. Kharkwal , Kranti Kumar , K. Asokan , A. Banerjee , A. K. Pramanik

In 5d transition metal oxides such as the iridates, novel properties arise from the interplay of electron correlations and spin-orbit interactions. We investigate the electronic structure of the pyrochlore iridates, (such as…

强关联电子 · 物理学 2015-05-19 Xiangang Wan , Ari Turner , Ashvin Vishwanath , Sergey Y. Savrasov

The dc-current-induced optical second-harmonic generation is observed at the surface of centrosymmetric single crystal of Si. Surface dc-current with density up to $\textit{j}_{max} \sim 10^{3}$ A/cm$^{2}$ results in break of inversion…

光学 · 物理学 2007-05-23 O. A. Aktsipetrov , V. O. Bessonov , A. A. Fedyanin , A. I. Maidykovsky

Metal-insulator transitions in pyrochlore iridates (A2Ir2O7) are believed to occur due to subtle interplay of spin-orbit coupling, geometric frustration, and electron interactions. In particular, the nature of magnetic ordering of iridium…

强关联电子 · 物理学 2014-07-29 Eric Kin-Ho Lee , Subhro Bhattacharjee , Yong Baek Kim

We report the systematic study of structural, magnetic and electrical transport properties of $Y_{2-x}Bi_xIr_2O_7$ (x = 0.0, 0.1, 0.2, 0.3) pyrochlore iridates. The chemical doping enhances electrical conductivity and antiferromagnetic…

材料科学 · 物理学 2020-01-08 Vinod Kumar Dwivedi , Soumik Mukhopadhyay

Non-Fermi liquid behavior in some fermionic systems have attracted significant interest in last few decades. Certain pyrochlore iridates with stronger spin-orbit coupling strength have recently been added to the list. Here, we provide…

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